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Interfacial engineering of the layered oxide cathode materials for sodium-ion battery

Nano Research 2024年第3期17卷 1441-1464页

作者： Quanqing Zhao Ruru Wang Ming Gao Faheem KButt Jianfeng Jia Haishun Wu Youqi Zhu Key Laboratory of Magnetic Molecules and Magnetic Information Materials of Ministry of Education School of Chemistry and Materials ScienceShanxi Normal UniversityTaiyuan 030032China Metals and Chemistry Research Institute China Academy of Railway Sciences Corporation LimitedBeijing 100081China Department of Physics Division of Science and TechnologyUniversity of EducationLahore 54770Pakistan Research Center of Materials Science Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green ApplicationsBeijing Institute of TechnologyBeijing 100081China

The layered metal oxides are reviewed as the hopeful cathode materials for high-performance sodium-ion batteries(SIBs)due to their large theoretical capacity,favorable two-dimensional(2D)ion diffusion channel,and simple ***,their cycling stability,rate capability,and thermal stability are still significantly concerned and highlighted before further practical *** chemical,mechanical and electrochemical stability of the cathode–electrolyte interfaces upon cycling is of great ***,the unique structural and electrochemical properties of the layered oxide cathode materials for SIB are *** mechanism of bulk/surface degradation induced by oxygen evolution,phase transition,microcrack,and electrolyte decomposition is thoroughly ***,the interfacial engineering to construct stable interface through various effective methods is fully *** future outlook and challenges for interfacial engineering in this filed are also *** review should shed light on the rational design and construct of robust interface for applications of superior layered oxide cathodes in SIB and may suggest future research directions.

关键词： interfacial engineering sodium-ion battery layered oxide electrolyte interface

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Ultrahigh rate binder-free Na_3V_2(PO_4)_3/carbon cathode for sodium-ion battery

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Journal of Energy Chemistry 2018年第5期27卷 1439-1445页

作者： Le Yang Wei Wang Mingxiang Hu Jiaojing Shao Ruitao Lv State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and Engineering Tsinghua University Beijing 100084 China School of Materials and Metallurgy Guizhou University Guiyang 550025 Guizhou China Key Laboratory of Advanced Materials (MOE) School of Materials Science and Engineering Tsinghua University Beijing 100084 China

sodium ion batteries （SIBs） are very promising for large-scale energy storage in virtue of its high energy density, abundant sodium resources and low environmental impact, etc. However, it is still a big chal- lenge to develop high-performance and durable cathode materials for SIBs. Among different candidate materials, Na_3V_2（PO_4）_3 has attracted great attentions due to its high theoretical capacity （117 mAh/g）, stable framework structure and excellent ionic conductivity. However, Na_3V_2（PO_4）_3 delivers inferior rate capability and cycling stability due to its poor electronic conductivity. In this work, free-standing Na_3V_2（PO_4）_3/carbon nanofiber membranes are synthesized by an electrospinning-sintering mute. The sample could deliver excellent cycling capability with specific capacity of 112 mAh/g at 1 C after 250 cycles and ultrahigh rate capability with 76.9 mAh/g even at 100 C, which is superior to many state-of- the-art SIB cathode materials. This can be attributed to the hierarchically distributed Na_3V_2（PO_4）_3 crystals in carbon nanofiber network, which possesses outstanding electronicfionic conductivity and thus leads to an ultrahigh rate capabilitY.

关键词： sodium-ion battery Free-standing cathode Na_3V_2(PO_4)_3 Carbon nanofiber Electrospinning

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Hollow Bio-derived Polymer Nanospheres with Ordered Mesopores for sodium-ion battery

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Nano-Micro Letters 2020年第3期12卷 1-11页

作者： Yan Ai Yuxiu You Facai Wei Xiaolin Jiang Zhuolei Han Jing Cui Hao Luo Yucen Li Zhixin Xu Shunqi Xu Jun Yang Qinye Bao Chengbin Jing Jianwei Fu Jiangong Cheng Shaohua Liu State Key Laboratory of Precision Spectroscopy and Department of Materials School of Physics and Electronic ScienceEast China Normal UniversityShanghai 200241People’s Republic of China Department of Physics and Astronomy Shanghai Jiao Tong UniversityShanghai 200240People’s Republic of China School of Chemistry and Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240People’s Republic of China Center for Advancing Electronics Dresden(cfaed)and Department of Chemistry and Food Chemistry Technische Universität Dresden01062 DresdenGermany School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450052People’s Republic of China State Key Lab of Transducer Technology Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050People’s Republic of China

Bio-inspired hierarchical self-assembly provides elegant and powerful bottom-up strategies for the creation of complex ***,the current self-assembly approaches for natural bio-compounds often result in materials with limited diversity and complexity in architecture as well as ***,we develop a novel coordination polymerization-driven hierarchical assembly of micelle strategy,using phytic acid-based natural compounds as an example,for the spatially controlled fabrication of metal coordination bio-derived *** resultant ferric phytate polymer nanospheres feature hollow architecture,ordered meso-channels of^12 nm,high surface area of 401 m2 g−1,and large pore volume of 0.53 cm3 g−*** an advanced anode material,this bio-derivative polymer delivers a remarkable reversible capacity of 540 mAh g−1 at 50 mA g−1,good rate capability,and cycling stability for sodium-ion *** study holds great potential of the design of new complex bio-materials with supramolecular chemistry.

关键词： Self-assembly Biomimetic synthesis Mesoporous polymer Ferric phytate sodium-ion battery

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Ultra‑Stable sodium‑ion battery Enabled by All‑Solid‑State Ferroelectric‑Engineered Composite Electrolytes

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Nano-Micro Letters 2024年第11期16卷 704-717页

作者： Yumei Wang Zhongting Wang Xiaoyu Xu Sam Jin An Oh Jianguo Sun Feng Zheng Xiao Lu Chaohe Xu Binggong Yan Guangsheng Huang Li Lu College of Aerospace Engineering Chongqing UniversityChongqing 400044People’s Republic of China National University of Singapore(Chongqing)Research Institute Chongqing 401123People’s Republic of China College of Materials Science and Engineering Chongqing UniversityChongqing 400044People’s Republic of China Department of Mechanical Engineering National University of Singapore9 Engineering Drive 1Singapore 117575Singapore Fujian Key Laboratory of Special Energy Manufacturing Xiamen Key Laboratory of Digital Vision MeasurementHuaqiao UniversityXiamen 361021People’s Republic of China

Symmetric Na-ion cells using the NASICON-structured electrodes could simplify the manufacturing process,reduce the cost,facilitate the recycling post-process,and thus attractive in the field of large-scale stationary energy ***,the long-term cycling performance of such batteries is usually *** investigation reveals the unavoidable side reactions between the NASICON-type Na_(3)V_(2)(PO_(4))_(3)(NVP)anode and the commercial liquid electrolyte,leading to serious capacity fading in the symmetric NVP//NVP *** resolve this issue,an all-solid-state composite electrolyte is used to replace the liquid electrolyte so that to overcome the side reaction and achieve high anode/electrolyte interfacial *** ferroelectric engineering could further improve the interfacial ion conduction,effectively reducing the electrode/electrolyte interfacial *** NVP//NVP cell using the ferroelectric-engineered composite electrolyte can achieve a capacity retention of 86.4%after 650 ***,the electrolyte can also be used to match the Prussianblue cathode NaxFeyFe(CN)_(6−z)·nH_(2)O(NFFCN).Outstanding long-term cycling stability has been obtained in the all-solid-state NVP//NFFCN cell over 9000 cycles at a current density of 500 mA g^(-1),with a fading rate as low as 0.005%per cycle.

关键词： sodium-ion battery NVP anode All-solid-state Cyclic stability Ferroelectric

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Ultra-stable carbon-coated sodium vanadium phosphate as cathode material for sodium-ion battery

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Rare Metals 2022年第1期41卷 115-124页

作者： Di Wang Peng Cai Guo-Qiang Zou Hong-Shuai Hou Xiao-Bo Ji Ye Tian Zhen Long Tianjin Key Laboratory of Functional Crystal Materials Institute of Functional CrystalTianjin University of TechnologyTianjin 300384China College of Chemistry and Chemical Engineering Central South UniversityChangsha 410083China

Based on the excellent sodium ion mobility of sodium superionic conductor structures,Na_(3)V_(2)(PO_(4))_(3)materials have become promising cathode materials in sodium-ion batteries(SIBs).However,inadequate electronic transport of Na_(3)V_(2)(PO_(4))_(3)limits the cycling stability and rate performances in *** this work,high-performance conductive carbon-coated Na_(3)V_(2)(PO_(4))_(3)materials are obtained via a simple and facile ball-milling assisted solid-state method by utilizing citric acid as carbon *** carbon-coated composite electrodes display a high initial specific capacity of 111.6 mAh·g^(-1),and the specific capacity could retention reach 92.83%after 100 cycles at 1C with the high coulombic efficiency(99.95%).More importantly,the capacity of conductive carbon-coated nano-sized Na_(3)V_(2)(PO_(4))_(3)can remain 48.5 mAh·g^(-1) at 10℃after 3000 cycles(initial capacity of 101.2 mAh·g^(-1)).At the same time,high coulombic efficiency(near 100%)has little decay even at a high rate of 20℃during 1000 cycles,demonstrating the excellent cycling stability and remarkable rate performances,and showing potential in largescale productions and applications.

关键词： Na_(3)V_(2)(PO_(4))_(3) sodium superionic conductor structures Ball-milling Cathode sodium-ion battery

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Fluorophosphates and fluorosulfates cathode materials: Progress towards high energy density sodium-ion battery

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Nano Research 2024年第3期17卷 1427-1440页

作者： Mohammed Hadouchi Jingrong Hou Toshinari Koketsu Abdelilah Lahmar Jiwei Ma Laboratoire de Chimie Appliquée des Matériaux Centre des Sciences des MatériauxFaculty of ScienceMohammed V University in RabatAvenue Ibn BattoutaBP 1014RabatMorocco Shanghai Key Laboratory for R&D and Application of Metallic Functional Materials Institute of New Energy for VehiclesSchool of Materials Science and EngineeringTongji UniversityShanghai 201804China battery Materials Development Section Business Creation Sector R&D CenterMitsui Mining&Smelting Co.Ltd.362-0021 SaitamaJapan Laboratoiry of Condensed Matter Physics University of Picardie Jules Verne33 Rue Saint-Leu 80039AmiensFrance

The rapid diffusion of renewable energy boosts the wide deployment of large-scale energy storage *** the low cost and high crustal abundance,sodium-ion battery(SIB)technology is expected to become a dominant technology in that area in the *** the practical application,novel cathode materials are urged to develop that show high energy density without sacrificing their cost and benignity to the *** the years of many studies,this still remains a huge challenge to battery *** this review,we discuss recent breakthroughs in SIB cathode materials with high energy density,namely fluorphosphates and *** design of materials,the crystal structure,the electrochemical performance,and the underlaying intercalation mechanism are systematically *** strategies and research directions are also provided to advance future high-energy,low-cost,and ecofriendly cathode materials for next generation SIB.

关键词： fluorophosphates fluorosulfates crystal structure intercalation mechanism high energy density sodium-ion battery

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Surface engineering based on in situ electro-polymerization to boost the initial Coulombic efficiency of hard carbon anode for sodium-ion battery

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Rare Metals 2022年第5期41卷 1616-1625页

作者： Cheng-Xin Yu Yu Li Zhao-Hua Wang Xin-Ran Wang Ying Bai Chuan Wu Beijing Key Laboratory of Environmental Science and Engineering School of Materials Science&EngineeringBeijing Institute of TechnologyBeijing 100081China Yangtze Delta Region Academy of Beijing Institute of Technology Jiaxing 314019China

Hard carbon(HC) is considered as a commercial candidate for anode materials of sodium-ion batteries due to its low cost and excellent capacity. However, the problem of low initial Coulombic efficiency is still urgently needed to be solved to promote the industrialization of *** this paper, 2,2-dimethylvinyl boric acid(DEBA) is used to modify the surface of HC to prepare HC-DEBA materials. During the cycling, the C = C bonds of DEBA molecules will be in situ electro-polymerized to form a polymer network, which can act as the passive protecting layer to inhibit irreversible decomposition of electrolyte,and induce a thinner solid electrolyte interface with lower interface impedance. Therefore, HC-DEBA has higher initial Coulombic efficiency and better cycling stability. In ester-based electrolyte, the initial Coulombic efficiency of the optimized HC-DEBA-3% increases from 65.2% to77.2%. After 2000 cycles at 1 A·g^(-1), the capacity retention rate is 90.92%. Moreover, it can provide a high reversible capacity of 294.7 m Ah·g^(-1) at 50 mA·g^(-1). This simple surface modification method is ingenious and versatile,which can be extended to other energy storage materials.

关键词： sodium-ion battery Hard carbon Initial Coulombic efficiency Solid electrolyte interface Surface modification Ester electrolyte

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Enhanced interphasial stability of hard carbon for sodium-ion battery via film-forming electrolyte additive

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Nano Research 2023年第3期16卷 3823-3831页

作者： Wenguang Zhang Fanghong Zeng Huijuan Huang Yan Yu Mengqing Xu Lidan Xing Weishan Li Engineering Research Center of MTEES(Ministry of Education) Research Center of BMET(Guangdong Province)Engineering Lab.of OFMHEB(Guangdong Province)Key Lab.of ETESPG(GHEI)and Innovative Platform for ITBMD(Guangzhou Municipality)School of ChemistrySouth China Normal UniversityGuangzhou 510006China Hefei National Laboratory for Physical Sciences at the Microscale Department of Materials Science and EngineeringCAS Key Laboratory of Materials for Energy ConversionUniversity of Science and Technology of ChinaHefei 230026China

Although the operating mechanism of sodium-ion battery(SIB)resembles that of lithium-ion battery,common film-forming additive for lithium-ion battery does not play its role in ***,it is essential to tailor new additives for *** carbon(HC),as the most used anode material of SIB,has the disadvantage of interphasial instability,especially under the condition of long-term *** incessant accumulation of electrolyte decomposition products leads to a significant increase in interphasial impedance and a sharp decline in discharge *** this work,N-phenyl-bis(trifluoromethanesulfonimide)(PTFSI)was proposed as a novel film-forming electrolyte additive,which effectively enhances the long-term cycling performance for HC anode in *** passivation film generated from the preferential reduction of PTFSI improves the capacity retention of HC/Na half-cell from 0%to 68%after 500 ***,the enhanced interphasial stability of HC anode results in a 52%increase in capacity retention of HC/Na_(3)V_(2)(PO_(4))_(3)full-cells after 100 cycles.

关键词： hard carbon anode interphasial stability N-phenyl-bis(trifluoromethanesulfonimide) sodium-ion battery

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Bi_2Se_3/C Nanocomposite as a New sodium-ion battery Anode Material

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Nano-Micro Letters 2018年第3期10卷 135-143页

作者： Lixin Xie Ze Yang Jingying Sun Haiqing Zhou Xiaowei Chi Hailong Chen ANDy X.Li Yan Yao Shuo Chen Department of Physics and TcSUH University of Houston Department of Electrical and Computer Engineering and Materials Science and Engineering Program University of Houston The Woodruff School of Mechanical Engineering Georgia Institute of Technology Clements High School

Bi_2Se_3 was studied as a novel sodium-ion battery anode material because of its high theoretical capacity and high intrinsic conductivity. Integrated with carbon,Bi_2Se_3/C composite shows excellent cyclic performance and rate capability. For instance, the Bi_2Se_3/C anode delivers an initial capacity of 527 mAh g^(-10) at 0.1 A g^(-1) and maintains 89% of this capacity over 100 cycles. The phase change and sodium storage mechanism are also carefully investigated.

关键词： Bi2Se3 sodium-ion battery High-energy ball milling sodium storage mechanism

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Moisture stable and ultrahigh-rate Ni/Mn-based sodium-ion battery cathodes via K^(+)decoration

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Nano Research 2023年第5期16卷 6890-6902页

作者： Tao Yuan Yuanyuan Sun Siqing Li Haiying Che Qinfeng Zheng Yongjian Ni Yixiao Zhang Jie Zou Xiaoxian Zang Shi-Hao Wei Yuepeng Pang Shuixin Xia Shiyou Zheng Liwei Chen Zi-Feng Ma School of Materials and Chemistry University of Shanghai for Science and TechnologyShanghai 200093China Zhejiang Natrium Energy Co. Ltd.Shaoxing 312000China In-situ Center for Physical Sciences Shanghai Electrochemical Energy Device Research CenterFrontiers Science Center for Transformative MoleculesSchool of Chemistry and Chemical EngineeringShanghai Jiao Tong UniversityShanghai 200240China Faculty of Electrical Engineering and Computer Science Ningbo UniversityNingbo 315000China Key Laboratory of Solar Energy Utilization&Energy Saving Technology of Zhejiang Province Zhejiang Energy R&D Institute Co.Ltd.Hangzhou 311121China

As one of the most promising cathodes for sodium-ion batteries(SIBs),the layered transition metal oxides have attracted great attentions due to their high specific capacities and facile ***,their applications are still hindered by the problems of poor moisture stability and sluggish Na^(+)diffusion caused by intrinsic structural Jahn–Teller ***,we demonstrate a new approach to settle the above issues through introducing K^(+)into the structures of Ni/Mn-based *** physicochemical characterizations reveal that K^(+)induces atomic surface reorganization to form the birnessite-type K_(2)Mn_(4)O_(8).Combining with the phosphate,the mixed coating layer protects the cathodes from moisture and hinders metal dissolution into the electrolyte ***,K^(+)substitution at Na site in the bulk structure can not only widen the lattice-spacing for favoring Na^(+)diffusion,but also work as the rivet to restrain the grain crack upon *** as achieved K^(+)-decorated P2-Na_(0.67)Mn_(0.75)Ni_(0.2)5O_(2)(NKMNO@KM/KP)cathodes are tested in both coin cell and pouch cell configurations using Na metal or hard carbon(HC)as ***,the NKMNO@KM/KP||Na half-cell demonstrates a high rate performance of 50 C and outstanding cycling performance of 90.1%capacity retention after 100 cycles at 5 ***,the NKMNO@KM/KP||HC fullcell performed a promising energy density of 213.9 Wh·kg^(−1).This performance significantly outperforms most reported state-ofthe-art ***,by adopting this strategy on O3-NaMn_(0.5)Ni_(0.5)O_(2),we further proved the universality of this method on layered cathodes for SIBs.

关键词： sodium-ion battery cathode layered oxide material K^(+)decoration

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