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Achieving high-performance sodium metal anodes: From structural design to reaction kinetic improvement

Nano Research 2024年第3期17卷 1288-1312页

作者： Jing Xu Jianhao Yang Yashuang Qiu Yang Jin Tianyi Wang Bing Sun Guoxiu Wang Research Center of Grid Energy Storage and Battery Application School of Electrical and Information EngineeringZhengzhou UniversityZhengzhou 450001China College of Chemistry and Chemical Engineering Yangzhou University Yangzhou 225009China Centre for Clean Energy Technology School of Mathematical and Physical SciencesFaculty of ScienceUniversity of Technology SydneyUltimoNSW 2007Australia

sodium metal is one of the ideal anodes for high-performance rechargeable batteries because of its high specific capacity(~1166 mAh·g^(-1)),low reduction potential(-2.71 V compared to standard hydrogen electrodes),and low ***,the unstable solid electrolyte interphase,uncontrolled dendrite growth,and inevitable volume expansion hinder the practical application of sodium metal *** present,many strategies have been developed to achieve stable sodium metal ***,we systematically summarize the latest strategies adopted in interface engineering,current collector design,and the emerging methods to improve the reaction kinetics of sodium deposition ***,the strategies of constructing protective layers are reviewed,including inorganic,organic,and mixed protective layers through electrolyte additives or ***,the classification of metal-based,carbon-based,and composite porous frames is discussed,including their function in reducing local deposition current density and the effect of introducing sodiophilic ***,the recent progress of alloys,nanoparticles,and single atoms in improving Na deposition kinetics is systematically ***,the future research direction and the prospect of high-performance sodium metal batteries are proposed.

关键词： sodium metal anodes interface engineering current collector design reaction kinetics sodium deposition processes

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High‑Energy Room‑Temperature sodium–Sulfur and sodium–Selenium Batteries for Sustainable Energy Storage

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Electrochemical Energy Reviews 2023年第1期6卷 87-147页

作者： Zefu Huang Pauline Jaumaux Bing Sun Xin Guo Dong Zhou Devaraj Shanmukaraj Michel Armand Teofilo Rojo Guoxiu Wang Centre for Clean Energy Technology School of Mathematical and Physical SciencesFaculty of ScienceUniversity of Technology SydneyUltimoNSW 2007Australia Centre for Cooperative Research on Alternative Energies(CIC energiGUNE) Basque Research and Technology Alliance(BRTA)Alava Technology ParkAlbert Einstein 4801510 Vitoria-GasteizSpain Inorganic Chemistry Department University of the Basque Country UPV/EHUP.O.Box.64448080 BilbaoSpain

Rechargeable room-temperature sodium–sulfur(Na–S)and sodium–selenium(Na–Se)batteries are gaining extensive attention for potential large-scale energy storage applications owing to their low cost and high theoretical energy *** of electrode materials and investigation of mechanisms are essential to achieve high energy density and long-term cycling stability of Na–S(Se)***,we provide a comprehensive review of the recent progress in Na–S(Se)*** elucidate the Na storage mechanisms and improvement strategies for battery *** particular,we discuss the advances in the development of battery components,including high-performance sulfur cathodes,optimized electrolytes,advanced Na metal anodes and modified *** with current research achievements,this review outlines remaining challenges and clear research directions for the future development of practical high-performance Na–S(Se)batteries.

关键词： sodium-sulfur batteries sodium-selenium batteries Sulfur cathodes Electrolyte engineering Solid-state electrolytes sodium metal anodes

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