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Sorting semiconducting single-walled carbon nanotubes by Water-Soluble Polyfluorene Assisted Electrophoresis and Its Application in Field-effect Transistors

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Chinese Journal of Chemistry 2015年第7期33卷 756-764页

作者： Haoyun Zhu Weizhi Wang State Key Laboratory of Molecular Engineering of Polymers Collaborative Innovation Center of Polymers and Polymer Composite Materials Department of Maeromoleeular Science Fudan University Shanghai 200433 China

We report a considerably promising method based on agarose gel electrophoresis （AGE） to separate single-walled carbon nanotubes by adding a water-soluble polyfluorene （w-PFO） as surfactant into the agarose gel. In this effective method, the AGE/w-PFO gel network will trap more semiconducting single-walled carbon nanotubes （SWNTs） with the assistance ofw-PFO, for the strong interaction between w-PFO and semiconducting species. The optical absorbance, photoluminescence emission and resonant Raman scattering characterization were used to ver- ify the separation effect. The purity of separated semiconducting species is as high as （98±1）%. The demonstrated field effect transistors give the on/off ratio and mobility about 27000 and 10.2 cm^2·V^-1·s^-1, respectively.

关键词： agarose gel electrophoresis field effect transistors semiconducting single-walled carbon nanotubes water-soluble polyfluorene

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Air-stable synaptic devices based on bismuth triiodide and carbon nanotubes

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Nano Research 2022年第6期15卷 5435-5442页

作者： Dandan Hao Junyao Zhang Li Li Ben Yang Pu Guo Shiqi Zhang Jia Huang Interdisciplinary Materials Research Center School of Materials Science and EngineeringFrontiers Science Center for Intelligent Autonomous SystemsTongji UniversityShanghai 201804China Translational Research Institute of Brain and Brain-Like Intelligence Shanghai Fourth People’s Hospital Affiliated to Tongji UniversitySchool of Materials Science and EngineeringTongji UniversityShanghai 200434China

Artificial synaptic devices with the functions of emulating important biological synaptic behaviors are playing an increasingly important role in the development of neuromorphic computing systems.single-walled carbon nanotubes(SWCNTs)with excellent electrical properties and high stability have been studied as active materials for synaptic devices.However,the performance of optical synaptic devices(OSDs)based on pure SWCNTs is limited by the weak light absorption property.Herein,bismuth triiodide(BiI_(3)),an environmentally stable and friendly optoelectronic material,is firstly combined with SWCNTs to fabricate OSDs with decent properties of perceiving and memorizing optical information.The OSDs can exhibit typical synaptic behaviors including excitatory postsynaptic current,paired-pulse facilitation,and short/long-term memory.Distinctively,the photoresponse of the OSD is independent of pulse light wavelength in the range of 365 to 650 nm,different from most of the previously reported OSDs,which usually have wavelength-dependent photo-response.Temperature-dependent photo-response behaviors of the devices are investigated.Importantly,the OSD without encapsulation holds good excitatory post-synaptic current(EPSC)behavior after being stored in the ambient environment for 170 days,indicating reliable environmental stability.Furthermore,an OSD array with nine synaptic devices is employed to mimic the human visual perception and memory functions.These results suggest the feasibility of BiI3/SWCNTs-based OSDs for the simulation of human visual memory.

关键词： semiconducting single-walled carbon nanotubes bismuth triiodide optical synaptic devices stability human visual memory

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