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self-powered electrochemical system by combining Fenton reaction and active chlorine geheration for organic contaminant treatment

引用

Nano Research 2019年第11期12卷 2729-2735页

作者： Yawei Feng Kai Han Tao Jiang Zhenfeng Bian Xi Liang Xia Cao Hexing Li Zhong Lin Wang CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and SensorBejing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBejing 100083China School of Nanoscience and Technology University of Chinese Academy of Sciences Beijing 100049China Education Ministry Key and International Joint Lab of Resoure Chemistry and Shanghai Key Lab of Rare Earth Functional Materials Shanghai Normal UniversityShanghai 200234China School of Environmental and Chemical Engineering Shanghai Uriversity of Elecric PowerShanghai 200090China School of Material Science and Engineering Georgia Institute of Technology AtlantaGA 30332USA

Environmental deterioration,especially water pollution,is widely dispersed and could affect the quality of people's life at *** the sewage treatment plants are constructed to meet the demands of cities,distributed treatment units are still in request for the supplementary of centralized purification beyond the range of *** degradation can reduce organic pollution to some degree,but it has to be *** nanogenerator(TENG)is a newly-invented technology for low-frequency mechanical energy ***,by integrating a rotary TENG(R-TENG)as electric power source with an electrochemical cell containing a modified graphite felt cathode for hydrogen peroxide(H2O2)along with hydroxyl radical(·OH)generation by Fenton reaction and a platinum sheet anode for active chlorine generation,a self-powered electrochemical system(SPECS)was *** the driven of mechanical energy or wind flow,such SPECS can efficiently degrade dyes after power management in neutral condition without any O2 *** work not only provides a guideline for optimizing self-powered electrochemical reaction,but also displays a strategy based on the conversion from distributed mechanical energy to chemical energy for environmental remediation.

关键词： self-powered electrochemistry Fenton reaction active chlorine organic contaminant degradation

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