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Enhanced pyrocatalysis of the pyroelectric BiFeO_(3)/g-C_(3)N_(4) heterostructure for dye decomposition driven by cold–hot temperature alternation

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Journal of Advanced Ceramics 2021年第2期10卷 338-346页

作者： Mingzi Chen Yanmin Jia Huamei Li Zheng Wu Tianyin Huang Hongfang Zhang College of Physics and Electronic Information Engineering Zhejiang Normal UniversityJinhua321004China School of Science Xi’an University of Posts and TelecommunicationsXi’an710121China College of Environmental and Chemical Engineering Xi’an Polytechnic UniversityXi’an710048China Jiangsu Key Laboratory of Micro and Nano Heat Fluid Flow Technology and Energy Application School of Physical Science and Technology and School of Environmental Science and EngineeringSuzhou University of Science and TechnologySuzhou215009China

The BiFeO_(3)/g-C_(3)N_(4) heterostructure,which is fabricated via a simple mixing–calcining method,benefits the significant enhancement of the pyrocatalytic *** the growth of g-C_(3)N_(4) content in the heterostructure pyrocatalysts from 0 to 25%,the decomposition ratio of Rhodamine B(RhB)dye after 18 cold-hot temperature fluctuation(25-65℃)cycles increases at first and then decreases,reaching a maximum value of~94.2%at 10%while that of the pure BiFeO_(3) is~67.7%.The enhanced dye decomposition may be due to the generation of the internal electric field which strengthens the separation of the positive and negative carriers and further accelerates their *** intermediate products in the pyrocatalytic reaction also have been detected and confirmed,which proves the key role of the pyroelectric effect in realizing the dye decomposition using BiFeO_(3)/g-C_(3)N_(4) heterostructure *** pyroelectric BiFeO_(3)/g-C_(3)N_(4) heterostructure shows the potential application in pyrocatalytically degrading dye wastewater.

关键词： pyroelectric material BiFeO_(3) g-C_(3)N_(4) heterostructure pyrocatalysis

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氨基酸系列改性TGS晶体研究

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人工晶体学报 2000年第S1期29卷 106-页

作者：苏根博贺友平姚宏志史子康中国科学院福建物质结构研究所福州350002

TGS (triglycine sulfate) is a pyroelectric crystal material which has an excllent *** LATGS,a kind of doped TGS crystal,in which L α alanine (LA) substitues for glycine partially and induces an internal bias in TGS resulting in permanently poled single domain crystal,becomes the comprehensively used pyroelectric material. Based on the study which was about the locked polarization in LATGS,we select many kinds of aminoacids which have a strong polarity group and a unsymmetry atom to dope into TGS *** aninoacids are LB (L asparagine),LL (L lysine),LH (L histidine) and LG (L glutamid acid).The saturated solutions for above four crystals growth are prepared by TGS doped with different aminoacids in water. Transparent crystals up to several centinetres in size have been grown by circling plate method and the reversible rotation rate of the platform with the crystal was about 90 r/*** was a prefered growth in the b axis direction,with a growth rate of the b axis of about 1.0-1.2mm/*** concentrations of aminoacids doped in TGS crystals were determined by a liquid chromatography,the concentrations of different aminoacids are about 10 -3 . It shows that the lattice parameters ( a,b and V )of TGS doped with aminoacids are significant longer than that of pure TGS crystal. We conclude that the pyroelectic cofficient,pyroelectric merit and the locked polarization of four TGS crystals,especially,the internal bield ( E b ) of LLTGS is larger than the LATGS,so that the LLTGS crystal is a promising pyroelectrc material for infrared detector.

关键词： TGS crystal pyroelectric material crystal growth from solution

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