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Blackening failure of poly-α-olefin impregnated porous polymide due to the splitting of lubrication oil catalyzed by iron

引用

Friction 2024年第9期12卷 1969-1979页

作者： Pengfei SHI Yang YIN Shaohua ZHANG Diankai ZHANG Yuanyuan JIANG Yang WANG Ningning ZHOU Tao QING Jintao WU Linmao QIAN Jiyang ZHANG Lei CHEN Tribology Research Institute State Key Laboratory of Rail Transit Vehicle SystemSchool of Mechanical EngineeringSouthwest Jiaotong UniversityChengdu 610031China Beijing Key Laboratory of Long-life Technology of Precise Rotation and Transmission Mechanisms Beijing Institute of Control EngineeringBeijing 100094China Technology and Equipment of Rail Transit Operation and Maintenance Key Laboratory of Sichuan Province School of Mechanical EngineeringSouthwest Jiaotong UniversityChengdu 610031China

Lubrication failure accompanying with blackening phenomenon significantly reduces the long-running operational reliability of porous polymide(PPI)lubricated with poly-α-olefin(PAO)***,the effects of lubrication condition and counter-surface chemistry on the blackening failure of PAO impregnated PPI were studied through the comparison of the tribological tests against GCr15 steel ball and Al_(2)O_(3)ceramic ball with and without PAO oil *** products were found to be formed on the PAO impregnated PPI surface slid against steel ball or Al_(2)O_(3)ball added with iron nano-particles,but be absent under the conditions without iron or PAO *** analysis indicated that the iron-catalyzed splitting of PAO oil into small molecule alkanes and following the formation of black organic matter should be mainly responsible for the blackening *** dynamic(MD)simulations demonstrated that the iron facilitated the separation of hydrogen atom and the following broken of C–C bonds in PAO molecules,final resulting in the splitting of PAO oil.

关键词： porous polyimide poly-α-olefin oil friction-induced blackening phenomenon tribological performance ReaxFF MD simulation

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