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perylene-diimide derived organic photovoltaic materials

Science China Chemistry 2022年第3期65卷 462-485页

作者： Ming Zhang Yang Bai Chenkai Sun Lingwei Xue Haiqiao Wang Zhi-Guo Zhang State Key Laboratory of Organic/Inorganic Composites Beijing Advanced Innovation Center for Soft Matter Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China College of Chemistry and Green Catalysis CenterZhengzhou UniversityZhengzhou 450001China School of Chemical and Environmental Engineering Pingdingshan UniversityPingdingshan 467000China Beijing Engineering Research Center for the Synthesis and Applications of Waterborne Polymers Beijing University of Chemical TechnologyBeijing 100029China

In organic solar cells(OSCs), the material design on photovoltaic layers and interlayers has significantly contributed to the rapid progress of the device performance. perylene-diimides(PDIs), owing to their distinct advantages of high electron affinity, high electron mobility and facial chemical modification, are being widely studied in OSCs, especially designed as photovoltaic acceptors and cathode interlayers. In this review, recent progress on those PDI derived photovoltaic materials is systematically summarized. Due to the different working mechanism in devices, the design strategies on modification of the parent PDI units towards their application as acceptors and cathode interlayers are explained. After disclosing the fundamental structure-property relationships, we disclose some common features in the design of those tailor-made PDI-based photovoltaic materials, and we also highlight the challenges and opportunities in improving their device performance in the future.

关键词： organic solar cells perylene-diimides photovoltaic acceptor cathode interlayer

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