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2-D Modeling and Calculations of Stratospheric ozone and Influences of Convection, Diffusion, and Time

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Atmospheric and Climate Sciences 2024年第2期14卷 250-276页

作者： Ibraheem Alelmi Laurie Wei Sen Nieh Department of Mechanical Engineering The Catholic University of America Washington DC USA School of Engineering The Catholic University of America Washington DC USA College of Engineering Yuan Ze University Taoyuan

An engineering system approach of 2-D cylindrical model of transient mass balance calculations of ozone and other concerned chemicals along with fourteen photolysis, ozone-generating and ozone-depleting chemical reaction equations was developed, validated, and used for studying the ozone concentrations, distribution and peak of the layer, ozone depletion and total ozone abundance in the stratosphere. The calculated ozone concentrations and profile at both the Equator and a 60˚N location were found to follow closely with the measured data. The calculated average ozone concentration was within 1% of the measured average, and the deviation of ozone profiles was within 14%. The monthly evolution of stratospheric ozone concentrations and distribution above the Equator was studied with results discussed in details. The influences of slow air movement in both altitudinal and radial directions on ozone concentrations and profile in the stratosphere were explored and discussed. Parametric studies of the influences of gas diffusivities of ozone DO3 and active atomic oxygen DO on ozone concentrations and distributions were also studied and delineated. Having both influences through physical diffusion and chemical reactions, the diffusivity (and diffusion) of atomic oxygen DO was found to be more sensitive and important than that of ozone DO3 on ozone concentrations and distribution. The 2-D ozone model present in this paper for stratospheric ozone and its layer and depletion is shown to be robust, convenient, efficient, and executable for analyzing the complex ozone phenomena in the stratosphere. .

关键词： Stratospheric ozone 2-D Model ozone Layer ozone depletion Convection Diffusion

Simulation and Causes of Eastern Antarctica Surface Cooling Related to ozone depletion during Austral Summer in FGOALS-s2

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Advances in Atmospheric Sciences 2014年第5期31卷 1147-1156页

作者： YANG Jing BAO Qing JI Duoying GONG Daoyi MAO Rui ZHANG Ziyin Seong-Joong KIM State Key Laboratory of Earth Surface Processes and Resource Ecology Beijing Normal University State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics Institute of Atmospheric Physics Chinese Academy of Sciences College of Global Change and Earth System Science Beijing Normal University Beijing Meteorological Bureau Korea Polar Research Institute Incheon 406-130 Korea

Two parallel sets of numerical experiments （an ozone-hole simulation and a non-ozone-hole simulation） were performed to investigate the effect of ozone depletion on surface temperature change using the second spectral version of the Flexible Global Ocean-Atmosphere-Land System model （FGOALS-s2）, focusing on the eastern Antarctica （EA） continent in austral summer. First, we evaluated the ability of the model to simulate the EA surface cooling, and found the model can successfully reproduce the cooling trend of the EA surface, as well as the circulation change circling the South Pole in the past 30 years. Second, we compared the two experiments and discovered that the ozone depletion causes the cooling trend and strengthens the circumpolar westerly flow. We further investigated the causes of the EA surface cooling associated with the ozone hole and found two major contributors. The first is the ozone-hole direct radiation effect （DRE） upon the surface that happens because the decrease of the downward longwave （LW） radiation overcomes the increase of the downward shortwave （SW） radiation under clear sky. The second is the cloud radiation effect （CRE） induced by ozone depletion, which happens because the decreased downward SW radiation overcomes the increased downward LW radiation in the case of increased cloud. Although the CRE is theoretically opposite to the DRE, their final net effect makes comparable contributions to the EA surface cooling. Compared with the surface radiation budget, the surface heat flux budgets have a much smaller contribution. We additionally note that the CRE is basically ascribed to the circulation change.

关键词： ozone depletion eastern Antarctica surface cooling numerical simulation

Air Temperature Changes over the Tibetan Plateau and Other Regions in the Same Latitudes and the Role of ozone depletion

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Acta meteorologica Sinica 2009年第3期23卷 290-299页

作者：张人禾周顺武 State Key Laboratory of Severe Weather (LaSW) Chinese Academy of Meteorological Sciences Jiangsu Key Laboratory of Metrological Disaster Nanjing University of Information Sciences and Technology

Using radiosonde and satellite observations, we investigated the trends of air temperature changes over the Tibetan Plateau （TP） in comparison with those over other regions in the same latitudes from 1979 to 2002. It is shown that Over the TP, the trends of air temperature changes in the upper troposphere to lower stratosphere were out of phase with those in the lower to middle troposphere. Air temperature decreased and a decreasing trend appeared in the upper troposphere to lower stratosphere. The amplitude of the annual or seasonal mean temperature decreases over the TP was larger than that over the whole globe. In the lower to middle troposphere over the TP, temperature increased, and the increasing trend was stronger than that over the non-plateau regions in the same latitudes in the eastern part of China. Meanwhile, an analysis of the satellite observed ozone data in the same period of 1979-2002 shows that over the TP, the total ozone amount declined in all seasons, and the ozone depleted the most compared with the situations in other regions in the same latitudes. It is proposed that the difference between the ozone depletion over the TP and that over other regions in the same latitudes may lead to the difference in air temperature changes. Because of the aggravated depletion of ozone over the TP, less （more） ultraviolet radiation was absorbed in the upper troposphere to lower stratosphere （lower to middle troposphere） over the TP, which favored a stronger cooling in the upper troposphere to lower stratosphere, and an intenser heating in the lower to middle troposphere over the TP. Therefore, the comparatively more depletion of ozone over the TP is possibly a reason for the difference between the air temperature changes over the TP and those over other regions in the same latitudes.

关键词： the Tibetan Plateau air temperature changes ozone depletion

Causes of ozone Layer depletion and Its Effects on Human: Review

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Atmospheric and Climate Sciences 2016年第1期6卷 129-134页

作者： Fakhra Anwar Fahad Nazir Chaudhry Saiqa Nazeer Noshila Zaman Saba Azam Department of Zoology University of Gujrat Hafiz Hayat Campus Gujrat Pakistan

This study was conducted at University of Gujrat during 2014-2015 as a term paper for Master of Philosophy. The data regarding effect of ozone depletion on human was reviewed and compiled as a review paper from various published articles of international reputed journals, annual/environmental reports of recognized organization and e-books. The causes, mechanism and bio-effects of ozone layer depletion on humans were addressed. It is revealed that introduction of Chloroflourocarbons (CFCs) in the environment is the most rated cause of said depiction. ozone depletion is allowing the UV radiation to earth surface. The exposure to these radiations is severely affecting all life forms on earth, especially the humans. Permanent or temporary blindness, skin cancer and immunity suppression are the main effects of these radiations reported by various researchers on humans. The prospects of ozone recovery are still undiscovered. The current situation of ozone depiction demands urgent remedial measures to protect lives on this earth.

关键词： ozone ozone depletion Chloroflourocarbons (CFCs) Ultra Violet (UV) Radiations Bio-Effects

Middle Stratospheric Polar Vortex ozone Budget during the Warming Arctic Winter, 2002-2003

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Advances in Atmospheric Sciences 2011年第5期28卷 985-996页

作者：刘毅刘传熙铁学熙高守亭 Key Laboratory of Middle Atmosphere and Global Environment Observation Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029 Graduate University of Chinese Academy of Sciences Beijing 100049 National Center for Atmospheric Research BoulderColoradoUSA Laboratory of Cloud Precipitation Physicsand Severe Storms Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029

The ozone budget inside the middle stratospheric polar vortex （24-36 km） during the 2002-2003 Arctic winter is studied by analyzing Michelson Interferometer for Passive Atmospheric Sounding （MIPAS） satellite data.A comprehensive global chemical transport model （Model for ozone and Related Chemical Tracers,MOZART-3） is used to analyze the observed variation in polar vortex ozone during the stratospheric sudden warming （SSW） events.Both MIPAS measurement and MOZART-3 calculation show that a pronounced increase （26-28 DU） in the polar vortex ozone due to the SSW events.Due to the weakening of the polar vortex,the exchange of ozone mass across the edge of the polar vortex increases substantially and amounts to about 3.0 × 10 7 kg according to MOZART-3 calculation.The enhanced downward transport offsets about 80% of polar vortex ozone mass increase by horizontal transport.A ＂passive ozone＂ experiment shows that only ～55% of the vertical ozone mass flux in February and March can be attributed to the variation in vertical transport.It is also shown that the enhanced downward ozone above ～32 km should be attributed to the springtime photochemical ozone production.Due to the increase of air temperature,the NO x reaction rate increases by 40%-80% during the SSW events.As a result,NO x catalytic cycle causes another 44% decrease in polar vortex ozone compared to the net ozone changes due to dynamical transport.It is also shown that the largest change in polar vortex ozone is due to horizontal advection by planetary waves in January 2003.

关键词： stratospheric sudden warming planetary wave MIPAS MOZART-3 model ozone depletion

Quantifying the Response Strength of the Southern Stratospheric Polar Vortex to Indian Ocean Warming in Austral Summer

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Advances in Atmospheric Sciences 2014年第2期31卷 492-503页

作者： LI Shuanglin CHEN Xiaoting Climate Change Research Center and Nansen-Zhu International Research Centre Institute of Atmospheric PhysicsChinese Academy of Sciences State Key Laboratory of Severe Weather Chinese Academy of Meteorological Sciences Shaanxi Provincial Meteorological Observatory

A previous multiple-AGCM study suggested that Indian Ocean Warming （IOW） tends to warm and weaken the southern polar vortex.Such an impact is robust because of a qualitative consistency among the five AGCMs used.However,a significant difference exists in the modeled strengths,particularly in the stratosphere,with those in three of the AGCMs （CCM3,CAM3,and GFS） being four to five times as strong as those in the two other models （GFDL AM2,ECHAM5）.As to which case reflects reality is an important issue not only for quantifying the role of tropical ocean warming in the recent modest recovery of the ozone hole over the Antarctic,but also for projecting its future trend.This issue is addressed in the present study through comparing the models＇ climatological mean states and intrinsic variability,particularly those influencing tropospheric signals to propagate upward and reach the stratosphere.The results suggest that differences in intrinsic variability of model atmospheres provide implications for the difference.Based on a comparison with observations,it is speculated that the impact in the real world may be closer to the modest one simulated by GFDL AM2 and ECHAM5,rather than the strong one simulated by the three other models （CCM3,CAM3 and GFS）.In particular,IOW during the past 50 years may have dynamically induced a 1.0℃ warming in the polar lower stratosphere （～100 hPa）,which canceled a fraction of radiative cooling due to ozone depletion.

关键词： southern hemispheric polar vortex SST atmospheric general circulation models ozone depletion

Preliminary Investigation of Total ozone Column and Its Relationship with Atmospheric Variables

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Atmospheric and Climate Sciences 2023年第2期13卷 225-239页

作者： Moses Owoicho Audu Ejembi Emmanuel Otor Daniel Abi Daniel Audu Ogbe Chibuoke Kingsley Arinze Department of Physics Joseph Sarwuan Tarka University (Federal University of Agriculture) Makurdi Nigeria Department of Natural and Applies Sciences Namibia University of Science and Technology Windhoek Namibia Department of Chemical Science Yaba College of Technology Lagos Nigeria

This study attempts to investigate the interaction between lower and upper atmosphere, employing daily data of Total ozone Column (TOC) and atmospheric parameter (cloud cover) over Nigeria from 1998-2012;in order to study the dynamic effect of ozone on climate and vice versa. This is due to the fact that ozone and climate influence each other and the understanding of the dynamic effect of the interconnectivity is still an open research area. Monthly mean daily TOC and cloud cover data were obtained from the Earth Probe Total ozone Mass Spectroscopy (EPTOMS) and the International Satellite Cloud Climatology Project (ISCCP)-D2 datasets respectively. Bivariate analysis and Mann Kendall trend tests were used in data analysis. MATLAB and ArcGIS software were employed in analyzing the data. Results reveal that TOC increased spatially from the coastal region to the north eastern region of the country. Seasonally, the highest value of TOC was observed at the peak of rainy season when cloud activity is very high, while the lowest value was recorded in dry season. These variations were attributed to rain producing mechanisms and atmospheric phenomena which influence the transport and distribution of ozone. Furthermore, the statistical analysis reveals significant relationship between TOC and low and middle cloud covers in contrast to high cloud cover. This relationship is consistent with previous studies using other atmospheric variables. This study has given scientific insight which is useful in understanding the coupling of the lower and upper atmosphere.

关键词： Total ozone Column Cloud Cover ozone depletion Atmospheric Variables EPTOMS Nigeria

Global methyl halide emissions from biomass burning during 2003-2021

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Environmental Science and Ecotechnology 2023年第2期14卷 79-86页

作者： Xiaoyi Hu Di Chen Liting Hu Bowei Li Xinhe Li Xuekun Fang College of Environmental&Resource Sciences Zhejiang UniversityHangzhouZhejiang310058PR China State Key Joint Laboratory for Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing100871PR China Center for Global Change Science Massachusetts Institute of TechnologyCambridgeMA02139USA

Methyl halides(CH3Cl,CH3Br,and CH3I)are ozone-depleting substances.Biomass burning(BB)is an important source of methyl halides.The temporal variations and global spatial distribution of BB methyl halide emissions are unclear.Thus,global methyl halide emissions from BB during 2003e2021 were estimated based on satellite data.A significant decreasing trend(p<0.01)in global methyl halide emissions from BB was found between 2003 and 2021,with CH3Cl emissions decreasing from 302 to 220 Gg yr^(-1),CH3Br emissions decreasing from 16.5 to 11.7 Gg yr^(-1),and CH3I emissions decreasing from 8.9 to 6.1 Gg yr^(-1).From a latitudinal perspective,the northern high-latitude region(60e90N)was the only latitude zone with significant increases in BB methyl halide emissions(p<0.01).Based on an analysis of the drivers of BB methyl halide emissions,emissions from cropland,grassland,and shrubland fires were more correlated with the burned area,while BB emissions from forest fires were more correlated with the emissions per unit burned area.The non-BB emissions of CH3Cl increased from 4749 Gg yr^(-1)in 2003 to 4882 Gg yr^(-1)in 2020,while those of CH3Br decreased from 136 Gg yr^(-1)in 2003 to 118 Gg yr^(-1)in 2020(global total CH3I emissions are not available).The finding indicates that global CH3Cl and CH3Br emissions from sources besides BB increased and decreased during 2003e2020.Based on our findings,not only searching for unknown sources is important,but also re-evaluating known sources is necessary for addressing methyl halide emissions.

关键词： Methyl halides Biomass burning Emission inventory Global budget ozone depletion

Opposite decadal atmospheric trends in the Southern Hemisphere between winter and summer

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Opposite decadal atmospheric trends in the Southern Hemisphe...