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Simulation Modelling Study of Self-Assembled nanoparticle Coatings for Retinal Implants

Journal of Bionic Engineering 2013年第1期10卷 65-76页

作者： TomasMaul Andrzej Bargiela Yuying Yan Nan Gao Alexander Foss School of Computer Science University of Nottingham Malaysia Campus Jalan Broga 43500 Semenyih Malaysia School of Computer Science University of Nottingham Jubilee Campus Wollaton Road Nottingham NG8 1BB UK Faculty of Engineering University of Nottingham Nottingham NG7 2RD UK Department of Ophthalmology Queen's Medical Centre Nottingham NG7 2UH UK

The electrode resolution of current retinal prostheses is still far from matching the densities of retinal neurons. Decreasing electrode diameter increases impedance levels thus deterring effective stimulation of neurons. One solution is to increase the surface roughness of electrodes, which can be done via nanoparticle coatings. This paper explores a Lattice Gas Model of the drying-mediated self-assembly of nanoparticle mixtures. The model includes representations for different types of nanoparti- cles, solvent, vapour, substrate and the energetic relationships between these elements. The dynamical aspect of the model is determined by energy minimization, stochastic fluctuations and physical constraints. The model attempts to unravel the rela- tionships between different experimental conditions （e.g. evaporation rate, substrate characteristics and solvent viscosity） and the surface roughness of resulting assemblies. Some of the main results include the facts that the assemblies formed by nanoparticles of different sizes can boost roughness in specific circumstances and that the optimized assemblies can exhibit walled or stalagmite structures. This study provides a set of simulation modelling experiments that if confirmed in the laboratory may result in new and useful materials.

关键词： nanoparticle assemblies simulation modelling Lattice Gas Models retinal prostheses

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Flexible synthesis of high-purity plasmonic assemblies

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Nano Research 2021年第3期14卷 635-645页

作者： Laurent Lermusiaux Anum Nisar Alison M.Funston ARC Centre of Excellence in Exciton Science and School of Chemistry Monash UniversityClaytonVIC3800Australia

The self-assembly of nanoparticles has attracted a vast amount of attention due to the ability of the nanostructure to control light at the sub-wavelength scale,along with consequent strong electromagnetic field ***,most approaches developed for the formation of discrete assemblies are limited to a single and homogeneous system,and incorporation of larger or asymmetrical nanoparticles into assemblies with high purity remains a key ***,a simple and versatile approach to assemble nanoparticles of different sizes,shapes,and materials into various discrete homo-or hetero-structures using only two complementary deoxyribonucleic acid(DNA)strands is ***,surface functionalisation using DNA and alkyl-polyethylene glycol(PEG)enables transformation of as-synthesised nanoparticles into readily usable plasmonic building blocks for *** of the DNA coverage enables the production of different assembly types,such as homo-and hetero-dimers,trimers and tetramers and core-satellite structures,which are produced in high purity using electrophoresis *** approach is extended from purely plasmonic structures to incorporate(luminescent)semiconductor nanoparticles for formation of hybrid *** deposited assemblies form a high yield of specific geometrical arrangements,attributed to the van der Waals attraction between *** method will enable the development of new complex colloidal nanoassemblies for biological and optical applications.

关键词： deoxyribonucleic acid(DNA)self-assembly electrophoretic purification nanoparticle assemblies colloidal stability

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