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Molecular design of an ultra-strong tissue adhesive hydrogel with tunable multifunctionality

Bioactive Materials 2023年第11期29卷 214-229页

作者： Yuting Zheng Avijit Baidya Nasim Annabi Department of Chemical and Biomolecular Engineering University of Californi1Los AngelesLos AngelesCA90095United States Department of Bioengineering University of Californi1Los AngelesLos AngelesCA90095United States

Designing adhesive hydrogels with optimal properties for the treatment of injured tissues is challenging due to the tradeoff between material stiffness and toughness while maintaining adherence to wet tissue surfaces. In most cases, bioadhesives with improved mechanical strength often lack an appropriate elastic compliance, hindering their application for sealing soft, elastic, and dynamic tissues. Here, we present a novel strategy for engineering tissue adhesives in which molecular building blocks are manipulated to allow for precise control and optimization of the various aforementioned properties without any tradeoffs. To introduce tunable mechanical properties and robust tissue adhesion, the hydrogel network presents different modes of covalent and noncovalent interactions using N-hydroxysuccinimide ester (NHS) conjugated alginate (Alg-NHS), poly (ethylene glycol) diacrylate (PEGDA), tannic acid (TA), and Fe^(3+) ions. Through combining and tuning different molecular interactions and a variety of crosslinking mechanisms, we were able to design an extremely elastic (924%) and tough (4697 kJ/m3) multifunctional hydrogel that could quickly adhere to wet tissue surfaces within 5 s of gentle pressing and deform to support physiological tissue function over time under wet conditions. While Alg-NHS provides covalent bonding with the tissue surfaces, the catechol moieties of TA molecules synergistically adopt a mussel-inspired adhesive mechanism to establish robust adherence to the wet tissue. The strong adhesion of the engineered bioadhesive patch is showcased by its application to rabbit conjunctiva and porcine cornea. Meanwhile, the engineered bioadhesive demonstrated painless detachable characteristics and in vitro biocompatibility. Additionally, due to the molecular interactions between TA and Fe3+, antioxidant and antibacterial properties required to support the wound healing pathways were also highlighted. Overall, by tuning various molecular interactions, we were able to develop a single-hydrogel platform wit

关键词： Molecular engineering Tough hydrogel Bioadhesive multifunctionality

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Tree-based ecosystem services supply and multifunctionality of church forests and their agricultural matrix near Lake Tana,Ethiopia

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Forest Ecosystems 2023年第6期10卷 656-667页

作者： Ferehiwot Mequanint Tobias Fremout Diederik Strubbe Alemayehu Wassie Shimelis Aynalem Enyew Adgo Jan Nyssen Amaury Frankl Luc Lens Bart Muys Department of Wildlife and Ecotourism Management Bahir Dar UniversityBahir DarEthiopia Terrestrial Ecology Unit Ghent UniversityGhentBelgium Division Forest Natureand LandscapeKU LeuvenLeuvenBelgium Alliance Biodiversity International–CIAT LimaPeru Organization for Rehabilitation and Development in Amhara Bahir DarEthiopia Department of Natural Resource Management Bahir Dar UniversityBahir DarEthiopia Department of Geography Ghent UniversityGhentBelgium INRAE AMAPIRDCIRADCNRSUniversity MontpellierBld de La Lironde34398Montpellier Cedex 5France

Ecosystem services(ES)are the connection between nature and society,and are essential for the well-being of local communities that depend on them.In Ethiopia,church forests and the surrounding agricultural matrix supply numerous ES.However,the ES delivered by both land use types have not yet been assessed simultaneously.Here we surveyed both church forests and their agricultural matrices,aiming to quantify,compare and unravel the drivers underlying tree-based ES supply,density and multifunctionality.We found that almost all church forests and half of the agricultural matrices provided high ES densities.ES multifunctionality was higher in the agricultural matrices,suggesting that people deliberately conserve or plant multifunctional tree species.Furthermore,the supply of all categories of ES was positively correlated with church forest age(p-valuemultifunctionality,and to prioritize restoration efforts at sites with low levels thereof.

关键词： Church forest Remnant forest Provisioning service Regulating service Cultural service multifunctionality Key informant interview Agricultural matrix

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Fungal diversity rather than bacterial diversity drives the ecosystem multifunctionality of vineyards in a semi-arid region

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International Journal of Agricultural and Biological Engineering 2021年第6期14卷 126-136页

作者： Bingbing Duan Yizhao Ren Leqi Zhang Chenxing Suzhou Guoqiao Chen Ping Cui Yusong Zhangyang Wei Liu Hasmik Merkeryan Xu Liu College of Enology Northwest A&F UniversityYangling 712100ShaanxiChina Penglai Wine College Yantai Institute of Science and TechnologyYantai 265600ShandongChina Grape Industrial Park Management Committee of the Eastern Foot of Helan Mountain in Ningxia Yinchuan 750004China Horticulture Research Institute Sichuan Academy of Agricultural SciencesChengdu 610066China Ningxia Helan Mountain’s East Foothill Wine Experiment and Demonstration Station of Northwest A&F University Yongning 750104NingxiaChina

The presence of multiple ecosystem functions and services(i.e.,ecosystem multifunctionality)has been proven to be maintained by biodiversity in natural terrestrial ecosystems.However,the mechanisms by which microbial diversity drives ecosystem functions in vineyards and the effects of ecosystem functions on wine quality remain unknown.Here,fifteen vineyards from five wine sub-regions(Shizuishan,Yinchuan,Yuquanying,Qingtongxia,and Hongsipu)in Ningxia were selected to assess the microbial community structure,ecosystem multifunctionality,and wine quality.Overall,each index differed among the vineyards from these five wine sub-regions in Ningxia.High-throughput sequencing revealed that bacterial and fungal communities varied among these vineyards.Bacterial communities were dominated by Actinobacteria,Proteobacteria,Chloroflexi,and Acidobacteria.Ascomycota was the dominant fungal phylum,followed by Basidiomycota and Mortierellomycota.In addition,fungal Shannon diversity rather than bacterial Shannon diversity showed a positive relationship with ecosystem multifunctionality.Correlation analysis revealed that ecosystem multifunctionality was positively correlated with wine acidity and negatively correlated with pH value and residual sugar content of wine.Soil chemical functions exhibited relationships with wine quality being similar to those of ecosystem multifunctionality;i.e.,positively related to wine acidity but negatively related to wine pH and residual sugar content.However,soil physical functions were negatively correlated with the alcohol and anthocyanin content of wine.The research results show that the ecosystem functions maintained by fungal diversity could be attributed to wine quality of vineyards.

关键词： microbial diversity multifunctionality terroir wine quality wine sub-regions

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Functional group richness increases multifunctionality in intensively managed grasslands

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Grassland Research 2023年第3期2卷 225-240页

作者： Laura Argens Caroline Brophy Wolfgang W.Weisser Sebastian Meyer Terrestrial Ecology Research Group Department for Life Science SystemsSchool of Life SciencesTechnical University of MunichFreisingGermany School of Computer Science and Statistics Trinity College DublinDublinIreland

Background:Agricultural yields have increased continuously over the last few decades.However,a focus solely on production can harm the environment.Diversification of agriculture has been suggested to increase production and sustainability.Biodiversity experiments showed positive effects on ecosystems and productivity.However,application of these results to intensively managed grasslands has been questioned due to differences in plant species and management regimes.Research on whether diversity can benefit multifunctionality,that is,an integrated index of multiple ecosystem functions,under intensive management,is still scarce.Methods:To address this,we manipulated plant species richness from one to six species spanning three functional groups(legumes,herbs,and grasses)in intensively managed multispecies grassland leys and examined seven ecosystem functions.Results:We found that multifunctionality increased with functional group and species richness.Legume+herb mixtures showed high multifunctionality,while grass monocultures and mixtures with high proportions of grasses had low multifunctionality.Different plant species and plant communities drove different ecosystem functions.Legumes and herbs improved productivity and water availability,while grasses enhanced invasion resistance.These results indicate that multifunctionality and individual ecosystem functions can be promoted through targeted combinations of plants with complementary ecological traits.Conclusions:Plant diversity can improve multifunctionality also under intensive management,potentially benefitting agroeconomics and sustainability.

关键词： biodiversity ecosystem functions intensively managed grassland Legacy Network(LegacyNet) multifunctionality

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An Environment‑Tolerant Ion‑Conducting Double‑Network Composite Hydrogel for High‑Performance Flexible Electronic Devices

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Nano-Micro Letters 2024年第5期16卷 352-369页

作者： Wenchao Zhao Haifeng Zhou Wenkang Li Manlin Chen Min Zhou Long Zhao State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074People’s Republic of China

High-performance ion-conducting hydrogels(ICHs)are vital for developing flexible electronic devices.However,the robustness and ion-conducting behavior of ICHs deteriorate at extreme tempera-tures,hampering their use in soft electronics.To resolve these issues,a method involving freeze–thawing and ionizing radiation technology is reported herein for synthesizing a novel double-network(DN)ICH based on a poly(ionic liquid)/MXene/poly(vinyl alcohol)(PMP DN ICH)system.The well-designed ICH exhibits outstanding ionic conductivity(63.89 mS cm^(-1) at 25℃),excellent temperature resistance(-60–80℃),prolonged stability(30 d at ambient temperature),high oxidation resist-ance,remarkable antibacterial activity,decent mechanical performance,and adhesion.Additionally,the ICH performs effectively in a flexible wireless strain sensor,thermal sensor,all-solid-state supercapacitor,and single-electrode triboelectric nanogenerator,thereby highlighting its viability in constructing soft electronic devices.The highly integrated gel structure endows these flexible electronic devices with stable,reliable signal output performance.In particular,the all-solid-state supercapacitor containing the PMP DN ICH electrolyte exhibits a high areal specific capacitance of 253.38 mF cm^(-2)(current density,1 mA cm^(-2))and excellent environmental adaptability.This study paves the way for the design and fabrication of high-performance mul-tifunctional/flexible ICHs for wearable sensing,energy-storage,and energy-harvesting applications.

关键词： Ionic liquids Double-network hydrogels Temperature tolerance multifunctionality Flexible electronic devices

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Vertically Aligned Silicon Carbide Nanowires/Boron Nitride Cellulose Aerogel Networks Enhanced Thermal Conductivity and Electromagnetic Absorbing of Epoxy Composites

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Nano-Micro Letters 2022年第7期14卷 209-227页

作者： Duo Pan Gui Yang Hala MAbo-Dief Jingwen Dong Fengmei Su Chuntai Liu Yifan Li Ben Bin Xu Vignesh Murugadoss Nithesh Naik Salah MEl-Bahy Zeinhom MEl-Bahy Minan Huang Zhanhu Guo Key Laboratory of Materials Processing and Mold(Zhengzhou University) Ministry of EducationNational Engineering Research Center for Advanced Polymer Processing TechnologyZhengzhou UniversityZhengzhou 450002People’s Republic of China Department of Chemistry College of ScienceTaif UniversityP.O.Box 11099Taif 21944Saudi Arabia Mechanical and Construction Engineering Faculty of Engineering and EnvironmentNorthumbria UniversityNewcastle upon Tyne NE18STUK Integrated Composites Laboratory(ICL) Department of Chemical and Biomolecular EngineeringUniversity of TennesseeKnoxvilleTN 37996USA Advanced Materials Division Engineered Multifunctional Composites(EMC)Nanotech LLCKnoxvilleTN 37934USA College of Materials Science and Engineering Taiyuan University of Science and TechnologyTaiyuan 030024People’s Republic of China Department of Mechanical and Manufacturing Engineering Manipal Institute of TechnologyManipal Academy of Higher EducationManipalKarnataka 576104India Department of Chemistry Turabah University CollegeTaif UniversityP.O.Box 11099Taif 21944Saudi Arabia Department of Chemistry Al-Azhar UniversityNasr CityCairo 11884Egypt

With the innovation of microelectronics technology, the heat dissipation problem inside the device will face a severe test. In this work, cellulose aerogel(CA) with highly enhanced thermal conductivity(TC) in vertical planes was successfully obtained by constructing a vertically aligned silicon carbide nanowires(SiC NWs)/boron nitride(BN) network via the ice template-assisted strategy. The unique network structure of SiC NWs connected to BN ensures that the TC of the composite in the vertical direction reaches 2.21 W m^(-1) K^(-1) at a low hybrid filler loading of 16.69 wt%, which was increased by 890% compared to pure epoxy(EP). In addition, relying on unique porous network structure of CA, EP-based composite also showed higher TC than other comparative samples in the horizontal direction. Meanwhile, the composite exhibits good electrically insulating with a volume electrical resistivity about 2.35 × 10^(11) Ω cm and displays excellent electromagnetic wave absorption performance with a minimum reflection loss of-21.5 dB and a wide effective absorption bandwidth(<-10 dB) from 8.8 to 11.6 GHz. Therefore, this work provides a new strategy for manufacturing polymer-based composites with excellent multifunctional performances in microelectronic packaging applications.

关键词： Epoxy Ice template Vertical alignment Thermal conductivity multifunctionality

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Recent progress on multifunctional electromagnetic interference shielding polymer composites

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Journal of Materials Science & Technology 2023年第3期134卷 106-131页

作者： Ke Tian Danrong Hu Quan Wei Qiang Fu Hua Deng College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu 610065China Rehabilitation Medicine Center and Institute of Rehabilitation Medicine Key Laboratory of Rehabilitation Medicine in Sichuan ProvinceWest China HospitalSichuan UniversityChengdu 610041China

The explosive development of electronic devices and wireless communication technology gives rise to the issue of electromagnetic pollution,known as electromagnetic interference(EMI).The accumulation of undesirable electromagnetic radiation in space disturbs the normal function of unshielded electronic appliances and poses seriously threat to human health.Thus,the development of EMI shielding materials have emerged to solve the grim problem.Considering the complex application contexts,EMI shielding materials have evolved from traditional single-function to multi-functions to meet the ever-increasing application requirements in recent few years.This paper provides detailed insight into the current re-search status and future challenges in the advancement of polymer-based EMI shielding materials with various functions.First,the basic theory of EMI shielding,factors influencing results and the dominating characterization technologies for EMI shielding properties are summarized.Then,the comprehensive descriptions of the seven types of multifunctional EMI shields are provided with respect to their structures,fabrication methods and specific functions.Meanwhile,the corresponding critical scientific and technical issues are proposed.Based on our comprehensive analysis,the main challenges in the development of multifunctional EMI shielding materials are presented.This review aims to provide some guidance and inspire more efforts toward functional EMI shielding material research to satisfy the growing requirements for next-generation electronic systems.

关键词： Polymer-based composites Electromagnetic interference shielding Multiple losses multifunctionality

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A comprehensive study on the processing of Co:ZnO nanostructured ceramics:Defect chemistry engineering and grain growth kinetics

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Journal of Materials Science & Technology 2023年第7期138卷 221-232页

作者： R.T.da Silva J.M.Morbec G.Rahman H.B.de Carvalho Universidade Federal de Ouro Preto-UFOP Ouro PretoMG 35400-000Brazil School of Chemical and Physical Sciences Keele UniversityKeele ST55BGUnited Kingdom Department of Physics Quaid-i-Azam UniversityIslamabad 45320Pakistan Universidade Federal de Alfenas-UNIFAL Alfenas 37130-000Brazi

In this report,we present a systematic study on the preparation of Co:ZnO ceramics via a standard solid-state route from different Co precursors(Co_(3)O_(4),CoO,and metallic Co)and atmospheres(O_(2)and Ar).Particular emphasis is given to defect chemistry engineering and the sintering growth kinetics.First-principles calculations based on density functional theory are employed to determine the formation en-ergy of the main point defects in ZnO and Co:ZnO systems.Based on the theoretical results,a set of chemical reactions is proposed.Detailed microstructural characterization is also performed to determine the degree of Co incorporation into the ZnO lattice.The samples prepared in Ar atmosphere and metal-lic Co present the highest Co solubility limit(lower apparent Co incorporation activation energy)due to the incongruent ZnO decomposition.Determination of the parameters of the sintering growth kinetics reveals that Co_(3)O_(4)is the best sintering additive to achieve larger grain sizes,and possible higher densi-ties,in both sintering atmospheres,while metallic Co is the best to achieve the smallest grain size with higher Co concentration and homogeneous spatial distribution for a subsequent reduction of dimension-ality.The results show that the sintering in O_(2)effectively promotes zinc vacancies in the ZnO structure,while the sintering in Ar promotes zinc interstitial defects.Our findings contribute to understanding the preparation of Co-doped ZnO ceramics and the sintering growth kinetics,which may improve the state of the art in processing the material at both bulk and nanometric scales.

关键词： multifunctionality Zinc oxide Defect engineering Growth kinetics

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Femtosecond laser direct writing of functional stimulus-responsive structures and applications

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International Journal of Extreme Manufacturing 2023年第4期5卷 375-414页

作者： Yuxuan Zhang Dong Wu Yachao Zhang Yucheng Bian Chaowei Wang Jiawen Li Jiaru Chu Yanlei Hu CAS Key Laboratory of Mechanical Behavior and Design of Materials Key Laboratory of Precision Scientific Instrumentation of Anhui Higher Education InstitutesDepartment of Precision Machinery and Precision InstrumentationUniversity of Science and Technology of ChinaHefei 230027People’s Republic of China

Diverse natural organisms possess stimulus-responsive structures to adapt to the surrounding environment.Inspired by nature,researchers have developed various smart stimulus-responsive structures with adjustable properties and functions to address the demands of ever-changing application environments that are becoming more intricate.Among many fabrication methods for stimulus-responsive structures,femtosecond laser direct writing(FsLDW)has received increasing attention because of its high precision,simplicity,true three-dimensional machining ability,and wide applicability to almost all materials.This paper systematically outlines state-of-the-art research on stimulus-responsive structures prepared by FsLDW.Based on the introduction of femtosecond laser-matter interaction and mainstream FsLDW-based manufacturing strategies,different stimulating factors that can trigger structural responses of prepared intelligent structures,such as magnetic field,light,temperature,pH,and humidity,are emphatically summarized.Various applications of functional structures with stimuli-responsive dynamic behaviors fabricated by FsLDW,as well as the present obstacles and forthcoming development opportunities,are discussed.

关键词： stimulus-responsive structures femtosecond laser direct writing laser–matter interaction multifunctionality

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Novel self-assembled two-dimensional layered oxide structure incorporated with Au nanoinclusions towards multifunctionalities

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Nano Research 2023年第1期16卷 1465-1472页

作者： Di Zhang Xingyao Gao Juanjuan Lu Ping Lu Julia Deitz Jianan Shen Hongyi Dou Zihao He Zhongxia Shang C.Austin Wade Xinghang Zhang Aiping Chen Haiyan Wang School of Materials Engineering Purdue UniversityWest LafayetteIN 47907USA Center for Integrated Nanotechnologies(CINT) Los Alamos National LaboratoryLos AlamosNM 87545USA Sandia National Laboratories AlbuquerqueNM 87185USA School of Electrical and Computer Engineering Purdue UniversityWest LafayetteIN 47907USA Thermo Fisher Scientific HillsboroOR 97124USA

Two-dimensional(2D)layered oxides have recently attracted wide attention owing to the strong coupling among charges,spins,lattice,and strain,which allows great flexibility and opportunities in structure designs as well as multifunctionality exploration.In parallel,plasmonic hybrid nanostructures exhibit exotic localized surface plasmon resonance(LSPR)providing a broad range of applications in nanophotonic devices and sensors.A hybrid material platform combining the unique multifunctional 2D layered oxides and plasmonic nanostructures brings optical tuning into the new level.In this work,a novel self-assembled Bi2MoO6(BMO)2D layered oxide incorporated with plasmonic Au nanoinclusions has been demonstrated via one-step pulsed laser deposition(PLD)technique.Comprehensive microstructural characterizations,including scanning transmission electron microscopy(STEM),differential phase contrast imaging(DPC),and STEM tomography,have demonstrated the high epitaxial quality and particle-in-matrix morphology of the BMO-Au nanocomposite film.DPC-STEM imaging clarifies the magnetic domain structures of BMO matrix.Three different BMO structures including layered supercell(LSC)and superlattices have been revealed which is attributed to the variable strain states throughout the BMO-Au film.Owing to the combination of plasmonic Au and layered structure of BMO,the nanocomposite film exhibits a typical LSPR in visible wavelength region and strong anisotropy in terms of its optical and ferromagnetic properties.This study opens a new avenue for developing novel 2D layered complex oxides incorporated with plasmonic metal or semiconductor phases showing great potential for applications in multifunctional nanoelectronics devices.

关键词： layered oxides plasmonic strain anisotropy multifunctionality

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