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Aggregate 2023年第2期4卷 156-162页

作者： Xiao-Yan Wang Junyi Gong Hang Zou Sheng Hua Liu Jing Zhang Key Laboratory of Pesticide and Chemical Biology Ministry of EducationCollege of ChemistryCentral China Normal UniversityWuhanHubeiChina Department of Laboratory Medicine Nanfang HospitalSouthern Medical UniversityGuangzhouGuangdongChina College of Chemical Engineering Shijiazhuang UniversityShijiazhuangP.R.China School of Science and Engineering Shenzhen Institute of Aggregate Science and TechnologyThe Chinese University of Hong KongShenzhenGuangdongChina

Long-lived luminescent materials possess wide application prospects in various areas,but their constructions still face a huge challenge,especially the achievement in *** aggregate is an effective method to attain intriguing luminescence,thus it is expected to build long-lived materials in *** this work,a series of new gold(I)complexes were developed by employing unique carbazole and phosphine as the ligands,and these resulting systems exhibited rare long lifetimes of milliseconds in the aggregate *** was well unveiled that these complexes emitted blue thermally activated delayed fluorescence(TADF)with the lifetimes of several microseconds in dilute solution;while orange-red phosphorescence with much longer lifetimes of several milliseconds were achieved in the aggregate *** our knowledge,this is the first implementation of aggregation-induced conversion from TADF to *** on their excellent luminescent properties,we successfully applied these complexes in cell imaging and inhibition of cancer cells.

关键词： aggregation-induced conversion carbazole gold(I)complexes long-lived luminescence millisecond lifetime

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