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Sulphite measurement and its influence on Hg behaviour in wet-limestone flue-gas desulphurization

Clean Energy 2020年第4期4卷 360-371页

作者： Ida Masoomi Sophia Bruttel Marc Oliver Schmid Günter Scheffknecht Univ.-Prof.Dr.techn.Günter Scheffknecht University of StuttgartInstitute of Combustion and Power Plant Technology—IFKPfaffenwaldring 23D-70569 StuttgartGermany

The most abundant and typical reducing agent for oxidized mercury in the slurry of wet flue-gas desulphurization(FGD)is the absorbed sulphur dioxide(SO_(2)),which is present as different species of bisulphite or sulphite,depending on the pH of the *** this study,two different measurement principles for continuous sulphite measurement in the slurry of lab-scale FGD were investigated to check their feasibility to be implemented in a wet *** first method is based on light absorbance at the characteristic wavelength of sulphite measurement using a spectrophotometer and,in the second method,sulphite is measured as sulphur dioxide using a gas *** addition,the correlation of sulphite concentration and mercury(Hg)in the slurry can be shown by measuring sulphite *** was concluded that using a spectrophotometer leads to distorted *** contrast,measuring sulphite as SO2 in the gas phase proved to be more *** implementation of the measurement technique in the lab-scale FGD showed promising results for sulphite ***,the correlation of Hg and sulphite concentration could be shown at different synthetic slurries containing different *** a slurry without halides demonstrated the ambivalent influence of sulphite in reactions involving Hg,in which sulphite acts as a ligand for Hg complexes as well as a reducing agent,depending on the existing ***,in the presence of halides,the role of sulphite was less significant.

关键词： flue-gas cleaning flue-gas desulphurization mercury re-emission sulphite measurement

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