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MoS_(2)core-shell nanoparticles prepared through liquid-phase ablation and light exfoliation of femtosecond laser for chemical sensing

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Science China(Technological Sciences) 2023年第3期66卷 853-862页

作者： ZUO Pei JIANG Lan LI Xin TIAN MengYao YUAN YongJiu HAN WeiNa MA Le HU LiFei HE ZhiCong LI Fang School of Mechanical and Electrical Engineering Hubei Key Laboratory of Optical Information and Pattern RecognitionSchool of Optical Information and Energy EngineeringWuhan Institute of TechnologyWuhan 430073China Laser Micro/Nano Fabrication Laboratory School of Mechanical EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing Institute of Technology Chongqing Innovation Center Chongqing 401120China

Molybdenum disulfide(MoS_(2))-based nanostructures are highly desirable for applications such as chemical and biological sensing,photo/electrochemical catalysis,and energy storage due to their unique physical and chemical properties.In this work,MoS_(2)core-shell nanoparticles were first prepared through the liquid-phase processing of bulk MoS2by a femtosecond laser.The core of prepared nanoparticles was incompletely and weakly crystalline MoS_(2);the shell of prepared nanoparticles was highly crystalline MoS_(2),which wrapped around the core layer by layer.The femtosecond laser simultaneously achieved liquid-phase ablation and light exfoliation.The formation mechanism of the core-shell nanoparticles is to prepare the nanonuclei first by laser liquid-phase ablation and then the nanosheets by light exfoliation;the nanosheets will wrap the nanonuclei layer by layer through van der Waals forces to form core-shell nanoparticles.The MoS_(2)core-shell nanoparticles,because of Mo-S bond breakage and recombination,have high chemical activity for chemical catalysis.Afterward,the nanoparticles were used as a reducing agent to directly prepare three-dimensional(3D)Au-MoS_(2)micro/nanostructures,which were applied as surface-enhanced Raman spectroscopy(SERS)substrates to explore chemical sensing activity.The ultrahigh enhancement factor(1.06×10^(11)),ultralow detection limit(10-13M),and good SERS adaptability demonstrate highly sensitive SERS activity,great ability of ultralow concentration detection,and ability to detect diverse analytes,respectively.This work reveals the tremendous potential of 3D Au-MoS_(2)composite structures as excellent SERS substrates for chemical and biological sensing.

关键词： MoS_(2)core-shell nanoparticle femtosecond laser liquid-phase ablation light exfoliation 3D Au-MoS_(2)composite structure chemical sensing

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