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An insight into aggregation kinetics of polystyrene nanoplastics interaction with metal cations

Chinese Chemical Letters 2022年第12期33卷 5213-5217页

作者： Yucheng Zhang Xiaotong Su Nora FYTam Xiaolan Lao Meiling Zhong Qihang Wu Huifang Lei Zihui Chen Zhang Li Jie Fu Key Laboratory for Water Quality and Conservation of the Pearl Stream Delta Ministry of EducationSchool of Environmental Science and EngineeringGuangzhou UniversityGuangzhou 510006China State Key Laboratory of Marine Pollution and Department of Chemistry City University of Hong KongHong KongChina School of Science and Technology Open University of Hong KongHong KongChina School of Environmental Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China

Once inevitably released into the aquatic environment,polystyrene nanoplastics(PS-NPs)will present complicated environmental behaviors,of which the aggregation is a key process determining their environmental fate and *** this study,the aggregation kinetics of different sizes(30 nm and 100 nm)of PS-NPs with metal cations(Na^(+),K^(+),Ca^(2+),Mg^(2+)and Pb^(2+))at different solution pH(3,6 and 8)were *** results showed that the aggregation of PS-NPs increased with cation *** Pb^(2+)as an example,the adsorption behavior of cations onto PS-NPs was determined by transmission electron microscopy(TEM)and energy dispersive X-ray(EDX)spectroscopy,which demonstrated Pb^(2+)could be adhered onto the surface of PS-NPs with the effect of charge *** critical coagulation concentrations(CCC)of smaller PS-NPs were higher than that of larger PS-NPs for monovalent cations,whereas a different pattern is observed for divalent *** was suggested that there were other factors that DLVO theory does not consider affect the stability of NPs with different particle *** addition,it should be noted that PS-NPs had the capacity of adsorbing large amounts of heavy metal cations and carried them transport to a long distance,and the corresponding ecological risks need to further elucidate.

关键词： Polystyrene nanoplastics lead cation Aggregation kinetics Critical coagulation concentration Size effect

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Reversible Disassembly and Intercalation of 2-Ureido-4[1 H]- Pyrimidinone Quadruple Hydrogen-bonded Supramolecular Assembly by Fluoride and lead Ions

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Chinese Journal of Chemistry 2011年第12期29卷 2684-2688页

作者：俞茂林赵春常冯科陈彬佟振合吴骊珠 Key Laboratory of Photochemical Conversion and Optoelectronic Materials Technical Institute of Physics and Chemistry ＆ Graduate University Chinese Academy of Sciences Beijing 100190 China

2-Ureido-4[1H]-pyrimidinone quadruple hydrogen-bonded assembly 1,1 containing N,N-dimethylaminophenyl moiety exhibits a sensitive response to fluoride anion and lead cation. Spectroscopic studies reveal that the presence of small amount of fluoride anions and lead cations can easily disassemble and intercalate 2-ureido- 4[ 1H]-pyri mi di none hydrogen-bonded supramolecular architectures.

关键词： 2-ureido-4[1H]-pyrimidinone assembly hydrogen bonds fluoride anion lead cation self-assembly

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