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Quantitative effect of kerogen type on the hydrocarbon generation potential of Paleogene lacustrine source rocks,Liaohe Western Depression,China

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Petroleum Science 2024年第1期21卷 14-30页

作者： Sha-Sha Hui Xiong-Qi Pang Fu-Jie Jiang Chen-Xi Wang Shu-Xing Mei Tao Hu Hong Pang Min Li Xiao-Long Zhou Kan-Yuan Shi State Key Laboratory of Petroleum Resources and Prospecting China University of Petroleum(Beijing)Beijing102249China College of Geosciences China University of Petroleum(Beijing)Beijing102249China Exploration and Development Research Institute PetroChina Liaohe Oilfield CompanyPanjin 124010LiaoningChina

Kerogen types exert a decisive effect on the onset and capacity of hydrocarbon generation of source *** source rocks in the Liaohe Western Depression are characterized by thick deposition,high total organic carbon(TOC)content,various kerogen types,and a wide range of thermal ***,their hydrocarbon generation potential and resource estimation can be *** this study,geochemical tests,numerical analysis,hydrocarbon generation kinetics,and basin modeling were integrated to investigate the differential effects of kerogen types on the hydrocarbon generation potential of lacustrine source *** hydrocarbon generation and expulsion(HGE)models of different kerogen types were established quantitatively upon abundant Rock-Eval/TOC/vitrinite reflectance(R_(o))*** sets of good-excellent source rocks deposited in the fourth(Es4),third(Es3),and first(Es1)members of Paleogene Shahejie Formation,are predominantly types I-II_(1),II_(1)-II_(2),and II-III,*** activation energy of types I-II_(2)kerogen is concentrated(180-230 kcal/mol),whereas that of type III kerogen is widely distributed(150-280 kcal/mol).The original hydrocarbon generation potentials of types I,II_(1),II_(2),and III kerogens are 790,510,270,and 85 mg/g TOC,*** Ro values of the hydrocarbon generation threshold for type I-III source rocks gradually increase from 0.42%to 0.74%,and Ro values of the hydrocarbon expulsion threshold increase from 0.49%to 0.87%.Types I and II_(1)source rocks are characterized by earlier hydrocarbon generation,more rapid hydrocarbon expulsion,and narrower hydrocarbon generation windows than types II_(2)and III source *** kerogen types also affect the HGE history and resource *** types(conventional,tight,and shale oil/gas)and three levels(realistic,expected,and prospective)of hydrocarbon resources of different members in the Liaohe Western Depression are *** suggest that t

关键词： Kerogen type Hydrocarbon generation potential lacustrine source rocks Liaohe western depression

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Application of C_(30)tetracyclic polyprenoids as effective biomarker in oil-to source rock correlation in the ZhuⅢdepression,Zhujiangkou Basin,northern South China

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Acta Oceanologica Sinica 2024年第8期43卷 37-46页

作者： Lei Lan Youchuan Li Shuchun Yang Yang Ouyang Wenjing Ding Qing Lin Shanshan Zhou CNOOC Research Institute Co. Ltd.Beijing 100028China

The northern South China Sea,including the Zhujiangkou Basin and the Beibuwan Basin,developed high-quality lacustrine source rocks during the Eocene rifting *** source rocks are vital for hydrocarbon generation in the northern South China *** ZhuⅠdepression in the Zhujiangkou Basin and the Beibuwan Basin typically exhibit high abundance of C_(30)4-methyl ***,shales in the Eocene Wenchang Formation in the ZhuⅢdepression of the Zhujiangkou Basin contains lower quantities of high-quality lacustrine source rocks with 4-methyl steranes,which often co-elute with some pentacyclic triterpanes in gas chromatography-mass spectrometry(GC-MS).Therefore,the single 4-methylsterane parameter based on GC-MS cannot accurately distinguish organic source in the deep to semi-deep water lacustrine source rocks of the Wenchang Formation from other source rocks,thus impeding the recognition of their contributions to petroleum *** this study,GC-MS of aliphatic hydrocarbons,palynofacies and algal identification,as well as stable carbon isotope data of organic matter were used to identify the algal species and construct the paleoclimate during deposition of the Wenchang Formation source rocks in the ZhuⅢdepression of the Zhujiangkou *** is suggested that during the Wenchang Formation period,freshwater green algae prevailed in the lake,which is likely account for the relatively low content of 4-methyl steranes in the high-quality lacustrine source *** by the algal species,it is proposed that the content of C_(30)tetracyclic polyprenoids(TPP)can better indicate the quality of the Wenchang source rocks than C_(30)4-methyl ***,a relationship between the TPP index and the quality of the lacustrine source rocks in the Wenchang Formation of the ZhuⅢdepression was established.A higher TPP index indicates higher organic matter abundance and hydrogen index of the lacustrine source *** applied to the origin analysis of oils

关键词： lacustrine source rocks C_(30)tetracyclic polyprenoids green algae Zhujiangkou Basin

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Organic geochemistry and petrology of source rocks from the Banqiao Sag, Bohai Bay Basin, China: Implications for petroleum exploration

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Petroleum Science 2022年第4期19卷 1505-1515页

作者： Xiang-Bai Liu Guang-Di Liu Wen-Ya Jiang Ze-Zhang Song Na Wang State Key Laboratory of Petroleum Resources and Prospecting China University of PetroleumBeijing102249China College of Geosciences China University of PetroleumBeijing102249China Exploration and Development Research Institute Dagang Oilfield CompanyPetroChinaTianjin300280China

The organic geochemistry and petrology of source rocks determine the hydrocarbon generation potential of the Banqiao Sag. In this study, organic geochemistry and petrology were used to determine the abundance of organic matter(OM), OM type, OM maturity, and sedimentary environments of the source rocks, collected from Cenozoic Shahejie Formation, Banqiao Sag, Bohai Bay Basin, China. Vitrinite and liptinite are the main maceral composition of the source rocks, and range from 18% to 81% and from 2% to82% on a mineral matter free(MMF) basis, respectively. The values of vitrinite reflectance(Ro)(0.36%-1.20%) and the Tmaxvalues(397-486.C) show that the thermal maturity range from low mature to peak-maturity. The abundance of OM varies between 0.22% and 4.37%, suggesting that the source rocks of the Shahejie(Es) Formation are mainly fair to good source rocks. The Rock-Eval pyrolysis results show that the source rocks have good petroleum generation potential. The amount of free hydrocarbons(S_1)and hydrocarbons generated from pyrolysis(S_(2)) range within 0.01-3.70 mg/g, and 0.04-29.17 mg/g. The hydrogen index(HI) varies between 18.18 and 741.13 mg HC/g TOC, with most of the samples appearing to be mainly Type II kerogen, and thereby exhibiting the ability to generate both oil and gas. The ratios of Pr/Ph, the cross plot of Pr/nC_(17)-Ph/nC_(18), the cross plot of C_(29)/C_(27)-Pr/Ph, and ternary of dibenzothiophene, dibenzofuran, and fluorene, indicate that the Shahejie Formation deposited in suboxic and weak reducing environments. The main biological source is from advanced plants. The maceral composition and rock pyrolysis data indicate the kerogen type is a humic type or mixed sapropelic-humic type. The source rocks of the Shahejie(Es) Formation occur in the oil window, and the abundant organic richness,humic kerogen demonstrate that these rocks are effective oil and gas source rocks. The mudstone rocks in the Shahejie Formation are the main source of oil and gas and re

关键词： lacustrine source rocks Petrology Biomarkers Depositional environment Banqiao Sag

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Maturity effects on steranes of source rocks in Lishu fault depression,Songliao Basin

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Acta Geochimica 2020年第4期39卷 561-573页

作者： Chuanjun Yi Min Zhang Li Teng College of Resources and Environment Yangtze UniversityWuhanPeople's Republic of China Key Laboratory of Exploration Technology for Oil and Gas Resource Ministry of EducationWuhanPeople's Republic of China

Geochemical analysis results of 30 source rock samples from Lishu fault depression in Songliao Basin show that samples are compositionally similar and represent a uniform organic *** distribution of steranes among the samples is due to rank,with vitrinite reflectances(Ro)ranging from 0.65 to 1.61%.In the maturity stage(Ro=0.65-1.20%),the absolute concentrations of steranes increase,which is affected by kerogen degradation,whereas the pyrolysis of high mature source(Ro=1.20-1.61%)show a decrease in the abundance of ***,the parameters of steranes vary greatly with *** of prognane/regular sterane value with the increase of maturity suggests that pregnane is not a product of regular steranes *** ratios of C27/C29regular sterane gradually increase,while the value of C29-20S/(20S+20R)and αββ/(αββ+ααα)decrease at high maturity stage,which is associated with the difference in the thermostability of steranes *** reversed trend can be used to determine the high-maturity stage of source *** the values of rearranged steranes/regular steranes in source rocks show an apparent positive correlation with maturity,it,therefore,appears to be particularly useful for maturity assessment at elevated levels.

关键词： Thermal effect Steranes Genetic mechanism lacustrine source rocks Maturity

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