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Recent progress in intermetallic nanocrystals for electrocatalysis:From binary to ternary to high-entropy intermetallics

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SmartMat 2023年第4期4卷 145-177页

作者： Jiawei Liu Carmen Lee Yue Hu Zhishan Liang Rong Ji Xiang Yun Debbie Soo Qiang Zhu Qingyu Yan School of Materials Science and Engineering Nanyang Technological UniversitySingaporeSingapore Institute of Materials Research and Engineering(IMRE) Agency for ScienceTechnology and Research(A*STAR)SingaporeSingapore

Developing sustainable and clean energy-conversion techniques is one of the strategies to simultaneously meet the global energy demand,save fossil fuels and protect the environment,in which nanocatalysts with high activity,selectivity and durability are of great *** nanocrystals,featuring their ordered atomic arrangements and predictable electronic structures,have been recognized as a type of active and durable catalysts in energy-related *** this minireview,the very recent progress in the syntheses and electrocatalytic applications of noble metal-based intermetallic nanocrystals is *** synthetic strategies,including the conventional thermal annealing approach and its diverse modifications,as well as the wet-chemical synthesis,for the construction of binary,ternary and high-entropy intermetallic nanocrystals have been discussed with representative examples,highlighting their strengths and ***,their electrocatalytic applications toward oxygen reduction reaction,small molecule oxidation reactions,hydrogen evolution reaction,CO_(2)/CO reduction reactions,and nitrogen reduction reaction are discussed,with the emphasis on how the ordered intermetallic structures contribute to the enhanced *** conclude the minireview by addressing the current challenges and opportunities of intermetallic nanocrystals in terms of syntheses and electrocatalytic applications.

关键词： binary intermetallic electrocatalysis high-entropy intermetallic intermetallic nanocrystals ternary intermetallic

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