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Simulation-based environmental-impact assessment of glycerol-to-hydrogen conversion technologies

Clean Energy 2021年第3期5卷 387-402页

作者： Yehia F.Khalil Department of Chemical&Environmental Engineering Yale UniversityNew HavenCT 06520USA

This simulation-based comparative assessment aims to quantify the environmental and human-health impacts of greener hydrogen(H2)production via three glycerol-based technologies,including:supercritical water reforming(SCWR),aqueous-phase reforming(APR)and autothermal reforming(ATR).The GaBi(2018 edition)life-cycle assessment(LCA)platform is used to develop cradle-to-gate product system models for these technologies and the TRACI 2.1 methodology is used to quantify their midpoint impact *** HYSYS(v11)process-simulation software is used to generate the life-cycle inventory(LCI)primary data required to produce 1 kg of H2 via each of the indicated glycerol-reforming *** ISO 14040:2006 reporting requirements for the LCA results interpretation step,three base case(BC)scenarios and four sensitivity scenarios(SS)are developed and quantified to compare the effects of different process electricity sources(US grid mix versus wind power)and thermal energy sources(natural gas versus biogas)on the LCA *** high operating pressure(viz.240 bar)of SCWR enabled assessment of the impact of in situ electricity generation to offset some of electricity required for this *** major insights from this research are as follows:(i)per 1 kg of produced H2,APR reduces CO_(2) emissions by≈95%compared to ATR and by≈92%compared to SCWR,(ii)for BC scenarios,the primary energy consumption(in MJ/kg of produced H2)is in the following order from highest to lowest:ATR>SCWR>APR and(iii)H2 production via glycerol APR is more environmentally sustainable than SCWR and ATR,and thus offers a promising path for greener H2 *** environmental sustainability studies should focus on expanding the scope of this study to include H2 production via water electrolysis using renewable electricity sources and via solar and nuclear-driven thermochemical water splitting.

关键词： glycerol hydrogen impact categories reforming supercritical water valorization

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Cradle to Gate Life Cycle Assessment(LCA) of 3D Printing Houses

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Journal of Earth Science and Engineering 2021年第1期9卷 13-19页

作者： Elias Ali Department of Civil and Environmental Engineering The University of Alabama in HuntsvilleAL 35805USA

This paper presents a comparative“cradle to gate”life cycle assessment(LCA)of 3D printing houses and conventional buildings using SimaPro software,as a tool to model and compare the two *** study considered a terraced type of buildings with a floor area of 60 m^(2)(functional unit),which could occupy 2-3 *** results indicated that 3D printing houses have a smaller environmental impact than conventional buildings in all impact categories except in terrestrial ecotoxicity,in which both alternatives resulted in 172 kg 1,4-DB eq.3D printing houses exhibit a higher climate impact from Timber floorboards,window frames,and Portland cement which are responsible for 7.39×10^(4) kg CO_(2) eq,9.34 ×10^(4) kg CO_(2) eq,and 3.82×10^(4) kg CO_(2) eq respectively.

关键词： 3D printing LCA environmental impact impact categories

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