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Electrolyte design for rechargeable anion shuttle batteries

eScience 2022年第6期2卷 573-590页

作者： Yao Wang Xu Yang Zhijia Zhang Xia Hu Yuefeng Meng Xia Wang Dong Zhou Hao Liu Baohua Li Guoxiu Wang Tsinghua Shenzhen International Graduate School Tsinghua UniversityShenzhen 518055China Centre for Clean energy Technology School of Mathematical and Physical SciencesFaculty of ScienceUniversity of Technology SydneySydneyNSW 2007Australia Max-Planck-Institute for Chemical Physics of Solids Topological Catalysis GroupNöthnitzer Straße 4001187 DresdenGermany

As an emerging new type of battery chemistry,the anion shuttle battery(ASB),based on the shuttling and storage of anions,is considered a sustainable alternative to gigawatt-scale energy storage due to the associated resource abundance,low cost,high safety,and high energy *** significant progress has been achieved,practical applications of ASBs are still hindered by tough challenges,such as short lifetime,limited reversible capacity,and low Coulombic ***,it is very necessary to design and explore new electrolyte systems with high electrochemical/chemical stability,sufficient compatibility towards electrodes,and excellent kinetics/reversibility for anion electrochemical ***,we review the recent achievements and main challenges in developing electrolytes for ASBs,which include solid,non-aqueous,and aqueous *** mainly focus on the unique properties and basic principles of designing these electrolytes,and their various performance *** on design strategies for ASB electrolytes are also presented,which could facilitate the development of advanced ASBs for grid-scale energy storage.

关键词： Anion shuttle batteries Electrolytes Electrochemical stability Interfacial compatibility grid-scale energy storage

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Porous zinc metal anodes for aqueous zinc-ion batteries:Advances and prospectives

Energy Materials and Devices

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energy Materials and Devices 2024年第3期2卷 1-29页

作者： Yichen Ding Bingyue Ling Xin Zhao Xu Yang Yao Wang Dong Zhou Guoxiu Wang Tsinghua Shenzhen International Graduate School Tsinghua UniversityShenzhen 518055China Center for Clean energy Technology School of Mathematical and Physical SciencesFaculty of ScienceUniversity of Tech-nology SydneySydney 2007Australia

The intensifying challenges posed by climate change and the depletion of fossil fuels have spurred concerted global efforts to develop alternative energy storage *** zinc-ion batteries(AZIBs)have emerged as promising candidates for large-scale electrochemical energy storage systems because of their intrinsic safety,cost-effectiveness,and environmental ***,Zn dendrite growth consis-tently poses a remarkable challenge to the performance improvement and commercial viability of *** use of three-dimensional porous Zn anodes instead of planar Zn plates has been demonstrated as an effec-tive strategy to regulate the deposition/stripping behavior of Zn2+ions,thereby inhibiting the dendrite ***,the merits of porous Zn anodes were summarized,and a comprehensive overview of the recent advancements in the engineering of porous Zn metal anodes was provided,with a particular emphasis on the structural orderliness and critical role of porous structure modulation in enhancing battery ***,strategic insights into the design of porous Zn anodes were presented to facilitate the practical implementation of AZIBs for grid-scale energy storage applications.

关键词： aqueous zinc-ion battery porous zinc metal anode dendrite structural orderliness grid-scale energy storage

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