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Designing Advanced Liquid electrolytes for Alkali Metal Batteries:Principles,Progress,and Perspectives

Energy & Environmental Materials 2023年第2期6卷 353-380页

作者： Wanming Teng Junxiong Wu Qinghua Liang Jiaojiao Deng Yu Xu Qiong Liu Biao Wang Ting Ma Ding Nan Jun Liu Baohua Li Qingsong Weng Xiaoliang Yu College of Chemistry and Chemical Engineering Inner Mongolia UniversityHohhot 010021China Inner Mongolia Key Laboratory of Graphite and Graphene for Energy Storage and Coating School of Materials Science and EngineeringInner Mongolia University of TechnologyHohhot 010051China Department of Mechanical Engineering Research Institute for Smart EnergyThe Hong Kong Polytechnic UniversityHong KongChina College of Environmental Science and Engineering Fujian Normal UniversityFuzhou 350007China Department of Chemical Engineering The University of MelbourneParkville VIC 3010Australia Shenzhen Key Laboratory on Power Battery Safety and Shenzhen Geim Graphene Center Tsinghua Shenzhen International Graduate School(SIGS)Shenzhen 518071China Inner Mongolia Enterprise Key Laboratory of High Voltage and Insulation Technology Inner Mongolia Electric Power(Group)Co.LtdHohhot 010020China

The ever-growing pursuit of high energy density batteries has triggered extensive efforts toward developing alkali metal(Li,Na,and K)battery(AMB)technologies owing to high theoretical capacities and low redox potentials of metallic ***,for new battery systems,the electrolyte design is critical for realizing the battery electrochemistry of *** electrolytes in alkali ion batteries are generally unsuitable for sustaining the stability owing to the hyper-reactivity and dendritic growth of alkali *** this review,we begin with the fundamentals of AMB *** advancements in concentrated and fluorinated electrolytes,as well as functional electrolyte additives for boosting the stability of Li metal batteries,are summarized and discussed with a special focus on structure-composition-performance *** then delve into the electrolyte formulations for Na-and K metal batteries,including those in which Na/K do not adhere to the Li-inherited ***,the challenges and the future research needs in advanced electrolytes for AMB are *** comprehensive review sheds light on the principles for the rational design of promising electrolytes and offers new inspirations for developing stable AMBs with high performance.

关键词： advanced liquid electrolytes alkali metal batteries concentrated and fluorinated electrolytes functional electrolyte additives

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