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Preparation of MXene-based hybrids and their application in neuromorphic devices

International Journal of Extreme Manufacturing 2024年第2期6卷 164-188页

作者： Zhuohao Xiao Xiaodong Xiao Ling Bing Kong Hongbo Dong Xiuying Li Bin He Shuangchen Ruan Jianpang Zhai Kun Zhou Qin Huang Liang Chu School of Materials Science and Engineering Jingdezhen Ceramic UniversityJingdezhen 333403JiangxiPeople’s Republic of China School of Mechanical and Vehicle Engineering Linyi UniversityLinyi 276000ShandongPeople’s Republic of China College of New Materials and New Energies Shenzhen Technology UniversityShenzhen 518118GuangdongPeople’s Republic of China School of Mechanical&Aerospace Engineering Nanyang Technological University50 Nanyang AvenueSingapore 639798Singapore Ningbo Institute of Materials Engineering and Technology Chinese Academy of ScienceNingbo 315201ZhejiangPeople’s Republic of China Institute of Carbon Neutrality and New Energy&School of Electronics and Information Hangzhou Dianzi UniversityHangzhou 310018ZhejiangPeople’s Republic of China

The traditional von Neumann computing architecture has relatively-low information processing speed and high power consumption,making it difficult to meet the computing needs of artificial intelligence(AI).Neuromorphic computing systems,with massively parallel computing capability and low power consumption,have been considered as an ideal option for data storage and AI computing in the future.Memristor,as the fourth basic electronic component besides resistance,capacitance and inductance,is one of the most competitive candidates for neuromorphic computing systems benefiting from the simple structure,continuously adjustable conductivity state,ultra-low power consumption,high switching speed and compatibility with existing CMOS technology.The memristors with applying MXene-based hybrids have attracted significant attention in recent years.Here,we introduce the latest progress in the synthesis of MXene-based hybrids and summarize their potential applications in memristor devices and neuromorphological intelligence.We explore the development trend of memristors constructed by combining MXenes with other functional materials and emphatically discuss the potential mechanism of MXenes-based memristor devices.Finally,the future prospects and directions of MXene-based memristors are briefly described.

关键词： MXene etching fabrication memristor neuromorphic

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MXenes/CNTs-based hybrids:fabrications,mechanisms,and modification strategies for energy and environmental applications

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Nano Research 2024年第5期17卷 3429-3454页

作者： Jizhou Jiang Fangyi Li Lei Ding Chengxun Zhang Arramel Xin Li School of Environmental Ecology and Biological Engineering School of Chemistry and Environmental EngineeringKey Laboratory of Green Chemical Engineering Process of Ministry of EducationEngineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationNovel Catalytic Materials of Hubei Engineering Research CenterWuhan Institute of TechnologyWuhan 430205China Nano Center Indonesia Jl.PUSPIPTEK Tangerang SelatanBanten 15314Indonesia Institute of Biomass Engineering Key Laboratory of Energy Plants Resource and UtilizationMinistry of Agriculture and Rural AffairsSouth China Agricultural UniversityGuangzhou 510642China

Emerging two-dimensional(2D)layered metal carbide and nitride materials,commonly termed MXenes,are increasingly recognized for their applications across diverse fields such as energy,environment,and catalysis.In the past few years,MXenes/carbon nanotubes(CNTs)-based hybrids have attracted extensive attention as an important catalyst in energy and environmental fields,due to their superior multifunctions and mechanical stability.This review aims to address the fabrication strategies,the identification of the enhancement mechanisms,and recent progress regarding the design and modification of MXenes/CNTs-based hybrids.A myriad of fabrication techniques have been systematically summarized,including mechanical mixing,spray drying,three-dimensional(3D)printing,self-assembly/in-situ growth,freeze drying,templating,hydrothermal methods,chemical vapor deposition(CVD),and rolling.Importantly,the identification of the enhancement mechanisms was thoroughly discussed from the two dimensions of theoretical simulations and in-situ analysis.Moreover,the recent advancements in profound applications of MXenes/CNTs-based hybrids have also been carefully revealed,including energy storage devices,sensors,water purification systems,and microwave absorption.We also underscore anticipated challenges related to their fabrication,structure,underlying mechanisms,modification approaches,and emergent applications.Consequently,this review offers insights into prospective directions and the future trajectory for these promising hybrids.It is expected that this review can inspire new ideas or provide new research methods for future studies.

关键词： MXenes/carbon nanotubes(CNTs)-based hybrids fabrication applications modification strategies

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fabrication and mechanical behavior of 2D-C_(f)/Ta_(x)Hf_(1−x)C–SiC composites by a low-temperature and highly-efficient route

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Journal of Advanced Ceramics 2023年第10期12卷 1961-1972页

作者： Xuegang Zou Dewei Ni Bowen Chen Feiyan Cai Le Gao Ping He Yusheng Ding Xiangyu Zhang Shaoming Dong State Key Laboratory of High-Performance Ceramics&Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China Structural Ceramics and Composites Engineering Research Center Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China University of Chinese Academy of Sciences Beijing 100049China Hangzhou Institute for Advanced Study University of Chinese Academy of SciencesHangzhouChina

C_(f)/Ta_(x)Hf_(1−x)C–SiC composites are ideal thermal structural materials for service under extreme conditions of hypersonic vehicles.However,how to synthesize TaxHf1-xC powders and efficiently fabricate C_(f)/Ta_(x)Hf_(1−x)C–SiC composites still faces some challenges.Furthermore,mechanical properties and thermophysical properties of Ta_(x)Hf_(1−x)C vary with the composition,but not monotonically.In-depth analysis of mechanical behaviors of the C_(f)/Ta_(x)Hf_(1−x)C–SiC composites is extremely important for their development and applications.In this study,the Ta_(x)Hf_(1−x)C powders(x=0.2,0.5,0.8)were successfully synthesized via solid solution of TaC and HfC at a relatively low temperature of 1800℃,with a small amount of Si as an additive.Subsequently,the efficient fabrication of 2D-C_(f)/Ta_(x)Hf_(1−x)C–SiC composites was achieved by slurry impregnation and lamination(SIL)combined with precursor infiltration and pyrolysis(PIP).In addition,the mechanical behavior of the composites was investigated systematically.It is demonstrated that the composites present remarkable non-brittle fractures,including a large number of fiber pull out and interphase debonding.Also,the fracture failure involves a complex process of microcrack generation and propagation,matrix cracking,and layer fracture.Moreover,the interfacial bonding between the fibers and the matrix is enhanced as the Ta∶Hf ratio decreases from 4∶1 to 1∶4.As a result,C_(f)/Ta_(0.2)Hf_(0.8)C–SiC composites exhibit exceptional flexural strength of 437±19 MPa,improved by 46%compared with C_(f)/Ta_(0.8)Hf_(0.2)C–SiC(299±19 MPa).This study provides a new perception of design and fabrication of ultra-high-temperature ceramic(UHTC)matrix composites with high performance.

关键词： mechanical properties microstructure fabrication 2D-C_(f)/Ta_(x)Hf_(1−x)C-SiC composites

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Circularly Polarized Light-Enabled Chiral Nanomaterials:From fabrication to Application

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Nano-Micro Letters 2023年第3期15卷 171-189页

作者： Changlong Hao Gaoyang Wang Chen Chen Jun Xu Chuanlai Xu Hua Kuang Liguang Xu International Joint Research Laboratory for Biointerface and Biodetection State Key Lab of Food Science and TechnologySchool of Food Science and TechnologyJiangnan UniversityWuxiJiangsu 214122People’s Republic of China Department of Neurology China National Clinical Research Center for Neurological DiseasesBeijing Tiantan HospitalCapital Medical UniversityNo.119 South 4Th Ring West RoadBeijing 100070People’s Republic of China

For decades,chiral nanomaterials have been extensively studied because of their extraordinary properties.Chiral nanostructures have attracted a lot of interest because of their potential applications including biosensing,asymmetric catalysis,optical devices,and negative index materials.Circularly polarized light(CPL)is the most attractive source for chirality owing to its high availability,and now it has been used as a chiral source for the preparation of chiral matter.In this review,the recent progress in the field of CPL-enabled chiral nanomaterials is summarized.Firstly,the recent advancements in the fabrication of chiral materials using circularly polarized light are described,focusing on the unique strategies.Secondly,an overview of the potential applications of chiral nanomaterials driven by CPL is provided,with a particular emphasis on biosensing,catalysis,and phototherapy.Finally,a perspective on the challenges in the field of CPL-enabled chiral nanomaterials is given.

关键词： Circularly polarized light Chiral Nanomaterials fabrication Application

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Recent progress in high-resolution tactile sensor array: From sensor fabrication to advanced applications

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Progress in Natural Science:Materials International 2023年第1期33卷 55-66页

作者： Rui Wang Shaoxiong Hu Wei Zhu Yue Huang Wenhao Wang Ying Li Yuchen Yang Jiajie Yu Yuan Deng Research Institute for Frontier Science Beihang University School of Materials Science and Engineering Beihang University Key Laboratory of Intelligent Sensing Materials Chip Integration Technology of Zhejiang Province(2021E10022) Hangzhou Innovation Institute of Beihang University

Tactile sensors can transform the environmental stimuli into electrical signals to perceive and quantify the environmental information, which show huge application prospects. The development of bionic robots and wearable devices towards intelligence has put high demands on the performance of tactile sensor arrays. Herein,the current state-of-the-art tactile sensor arrays over recent years have been summarized, from sensor array fabrication to advanced applications. The main preparation methods of patterned array including screen printing,3D printing, laser microprocessing, and textile technology are discussed in detail. Strategies to optimize the signal crosstalk caused by flexible high-density sensor arrays are systematically introduced from the perspective of structure design and circuit design. Furthermore, advanced tactile sensors are not limited to a single pressure sensing function, and hence the development of multimodal detection for sensors has been discussed. In order to promote the adaptability in applications, stretchable and self-powered versatile integration scheme for advanced sensing are briefly described. Then, by means of machine learning and neural networks, it is possible to deeply explore the information embedded in the tactile acquisition signal with enriched application scenarios. Finally,the current challenges and the future perspectives for flexible tactile sensor arrays towards practical use are provided.

关键词： Tactile sensor arrays fabrication Anti-crosstalk design Integration strategy Advanced application

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Recent progress and challenges in interdigital microbatteries:fabrication, functionalization and integration

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Journal of Energy Chemistry 2023年第3期78卷 294-314,I0009页

作者： Li Song Xuting Jin Chunlong Dai Yuyang Han Jiatao Zhang Yang Zhao Zhipan Zhang Liangti Qu Key Laboratory of Cluster Science Ministry of Education of ChinaKey Laboratory of Photoelectronic/Electrophotonic Conversion MaterialsSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 100081China Engineering Research Center of Advanced Functional Material Manufacturing of Ministry of Education School of Chemical EngineeringZhengzhou UniversityZhengzhou 450001Henan China School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Key Lab of Organic Optoelectronics and Molecular Engineering of Ministry of Education Department of ChemistryTsinghua UniversityBeijing 100084China

Currently,the increasing demands for portable,implantable,and wearable electronics have triggered the interest in miniaturized energy storage devices.Different from conventional energy storage devices,interdigital microbatteries(IMBs) are free of separators and prepared on a single substrate,potentially achieving a short ionic diffusion path and better performance.Meanwhile,they can be easily fabricated and integrated into on-chip miniaturized electronics,holding the promise to provide long-lasting power for advanced microelectronic devices.To date,while many seminal works have been reviewed the topic of microbatteries,there is no work that systematically summarizes the development of IMBs of high energy density and stable voltage platforms from fabrication,functionalization to integration.The current review focuses on the most recent progress in IMBs,discussing advanced micromachining techniques with compatible features to construct high-performance IMBs with smart functions and intelligent integrated systems.The future opportunities and challenges of IMBs are also highlighted,calling for more efforts in this dynamic and fast-growing research field.

关键词： Interdigital microbatteries fabrication Functionalization

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Design,fabrication,and realisation of a robotic fish actuated by dielectric elastomer with a passive fin

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IET Cyber-Systems and Robotics 2023年第2期5卷 48-55页

作者： Zekai Wang Junqiang Lou Xingdong Xiao Guoping Li Yimin Deng College of Mechanical and Electrical Engineering Zhejiang Industrial Polytechnic CollegeShaoxingChina College of Mechanical Engineering and Mechanics Ningbo UniversityNingboChina State Key Laboratory of Industrial Control Technology Zhejiang UniversityHangzhouChina

Robotic fish actuated by smart materials has attracted extensive attention and has been widely used in many applications.In this study,a robotic fish actuated by dielectric elastomer(DE)films is proposed.The tensile behaviours of DE film VHB4905 are studied,and the Ogden constitutive equation is employed to describe the stress‐strain behaviour of the DE film.The fabrication processes of the robotic fish,including prestretching treatment of the DE films,electrode coating with carbon paste,and waterproof treatment,are illustrated in detail.The dynamic response of the fabricated DE actuators under different excitation voltages is tested based on the experimental setup.Experimental results show that the first‐order natural frequencies of the obtained DE actuator in air is 4.05 Hz.Finally,the swimming performances of the proposed robotic fish at different driving levels are demonstrated,and it achieves an average swimming speed of 20.38 mm/s,with a driving voltage of 5kV at 0.8 Hz.

关键词： dielectric elastomer fabrication robotic fish swimming performances

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Stretchable Electrochemical Sensors: From Electrode fabrication to Cell Mechanotransduction Monitoring

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Chinese Journal of Chemistry 2023年第4期41卷 443-457页

作者： Wen-Ting Fan Wei-Hua Huang Yan-Ling Liu College of Chemistry and Molecular Sciences Wuhan UniversityWuhanHubei430072 China

Electrochemical sensing faces huge challenges in characterizing the transient release of biochemical molecules from deformed cells,due to the severely mechanical mismatch between rigid electrodes and soft cells.In recent years,the emergence of stretchable electrochemical sensors has made a breakthrough by complying with the deformation of living cells and simultaneous monitoring of mechanically evoked biochemical signals.This review first summarizes two fundamental strategies for the fabrication of stretchable electrodes from the points of structure and material.Next,recent progresses in construction of functionalized interface to improve the performance of stretchable electrochemical sensors are presented.Then,the application of stretchable electrochemical sensors in real-time monitoring of biomolecules released by mechanically sensitive cells is introduced.Finally,some perspectives and challenges of stretchable electrochemical sensors regarding cell detection are discussed.

关键词： Stretchable electrode Electrochemical sensing fabrication Functionalization Cell mechanotransduction

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Artificial nanomotors: fabrication, locomotion characterization, motion manipulation, and biomedical applications

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Interdisciplinary Materials 2022年第2期1卷 256-280页

作者： Liangmeng Wang Xiaomeng Hao Zhixue Gao Zili Yang Yi Long Ming Luo Jianguo Guan State Key Laboratory of Advanced Technology for Materials Synthesis and Processing International School of Materials Science and EngineeringWuhan University of TechnologyWuhanPeople's Republic of China School of Materials Science&Engineering Nanyang Technological UniversitySingaporeSingapore

Artificial nanomotors are nanoscale machines capable of converting surrounding other energy into mechanical motion and thus entering the tissues and cells of organisms.They hold great potential to revolutionize the diagnosis and treatment of diseases by actively targeting the lesion location,though there are many new challenges that arise with decreasing the size to nanoscale.This review sum-marizes and comments on the state-of-the-art artificial nanomotors with ad-vantages and limitations.It starts with the fabrication methods,including common physical vapor deposition and colloidal chemistry methods,followed by the locomotion characterization and motion manipulation.Then,the in vitro and in vivo biomedical applications are introduced in detail.The challenges and future prospects are discussed at the end.

关键词： biomedical application fabrication locomotion characterization motion manipulation nanomotor

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fabrication of lithium niobate metasurfaces via a combination of FIB and ICP-RIE

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Chinese Optics Letters 2022年第11期20卷 95-99页

作者：靳春艳兀伟曹雷高博锋陈嘉鑫蔡卫任梦昕许京军 Key Laboratory of Weak-Light Nonlinear Photonics Ministry of EducationSchool of Physics and TEDA Applied Physics InstituteNankai UniversityTianjin 300071China Science and Technology on Electro-Optical Information Security Control Laboratory Tianjin 300308China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China

Lithium niobate(LN)metasurfaces have emerged as a new platform for manipulating electromagnetic waves.Here,we report a fabrication technique for LN nano-grating metasurfaces by combining focused ion beam(FIB)milling with inductively coupled plasma reactive ion etching(ICP-RIE).Steep sidewalls with angles larger than 80°are achieved.Sharp quasi-bound states in the continuum are observed from our metasurfaces.The measured transmission spectra show good agreement with the numerical simulations,confirming the high quality of the fabricated metasurfaces.Our technique can be applied to fabricate the LN metasurfaces with sharp resonances for various applications in optical communications,on-chip photonics,laser physics,sensing,and so on.

关键词： lithium niobate metasurfaces fabrication FIB ICP-RIE

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