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Recent progress on nanostructured bimetallic electrocatalysts for water splitting and electroreduction of carbon dioxide

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Journal of Semiconductors 2020年第9期41卷 59-77页

作者： Can Cui Xiaosong Hu Liaoyong Wen Department of Materials Science and Engineering&Institute of Materials Science University of ConnecticutStorrsConnecticut06269-3136United States of America Key Laboratory of 3D Micro/Nano Fabrication and Characterization of Zhejiang Province School of EngineeringWestlake UniversityHangzhou 310024China

The exploitation of renewable energy as well as the elimination of the harmful impact of excessive carbon emission are worldwide concerns for sustainable development of the ecological environment on *** address that,the technologies regarding energy conversion systems,such as water splitting and electroreduction of carbon dioxide,have attracted significant attention for a few ***,to date,the production of green fuels and/or high energy density chemicals like hydrogen,methane,and ethanol,are still suffering from many drawbacks including high energy consumption,low selectivity,and sluggish reaction *** this regard,nanostructured bimetallic materials that is capable of taking the full benefits of the coupling effects between different elements/components with structure modification in nanoscale are considered as a promising strategy for high-performance ***,this review aims to outline the important progress of these nanostructured bimetallic *** starts with the introduction of some important fundamental background knowledge about the reaction mechanism to understand how these reactions ***,we summarize the most recent progress regarding how the nanostructured bimetallic electrocatalysts manipulate the activity and selectivity of catalytic reactions in the order of bimetallic alloying effect,interface/substrate effect of bi-component electrocatalyst,and nanostructuring effect.

关键词： bimetallic electrocatalysts nanostructures water splitting electroreduction of carbon dioxide

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