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Recent Advances of electroplating additives Enabling Lithium Metal Anodes to Applicable Battery Techniques

Energy & Environmental Materials 2021年第3期4卷 284-292页

作者： Xianshu Wang Weicong Mai Xiongcong Guan Qi Liu Wenqiang Tu Weishan Li Feiyu Kang Baohua Li Shenzhen Key Laboratory on Power Battery Safety and Shenzhen Geim Graphene Center Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China School of Materials Science and Engineering Tsinghua UniversityBeijing 100084China School of Chemistry South China Normal UniversityGuangzhou 510006China National and Local Joint Engineering Research Center of MPTES in High Energy and Safety LIBs Engineering Research Center of MTEES(Ministry of Education)and Key Lab.of ETESPG(GHEI)South China Normal UniversityGuangzhou 510006China

Lithium(Li)metal batteries have long been deemed as the representative high-energy-density energy storage systems due to the ultrahigh theoretical capacity and lowest electrochemical potential of Li metal ***,the intractable dendritic Li deposition during cycling greatly restrains the large-scale applications of Li metal *** advances have been explored to address this issue,among which a specific class of electrolyte additives for electroplating is deeply impressive,as they are economic and *** from the conventional additives that construct solid electrolyte interphase(SEI)layer on anodes,they make dendrite-free Li metal anodes feasible through altering Li plating *** this research news article,the interlinked principles between industrial electroplating and Li deposition are firstly *** featured effects of electroplating additives on regulating Li plating morphology are also summarized and mainly divided into three categories:co-deposition with Li cation,coordination with Li cation,and leveling effect of Li ***,the mechanism exploration or derivative use of electroplating additive for dendrite suppression and potential research directions are proposed,with emphasizing that industrial electroplating might enable Li metal anode to scalable battery techniques and spread to metal battery systems beyond Li.

关键词： electroplating additives lithium metal anodes co-deposition coordination leveling effect

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