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Reversible solid-oxide cells for clean and sustainable energy

Clean Energy 2019年第3期3卷 175-201页

作者： M.B.Mogensen M.Chen H.L.Frandsen C.Graves J.B.Hansen K.V.Hansen A.Hauch T.Jacobsen S.H.Jensen T.L.Skafte X.Sun Department of Energy Conversion and Storage Technical University of Denmark(DTU)Frederiksborgvej 399DK-4000 RoskildeDenmark Haldor Topsøe Haldor Topsøes Allé1DK-2800 Lyngby Department of Chemistry Technical University of DenmarkDK-2800 Kgs.LyngbyDenmark DynElectro ApS DK-4621 GadstrupDenmark

This review gives first a brief view of the potential availability of sustainable *** is clear that over 100 times more solar photovoltaic energy than necessary is readily accessible and that practically available wind alone may deliver sufficient energy supply to the *** to the intermittency of these sources,effective and inexpensive energy-conversion and storage technology is *** for the possible electrolysis application of reversible solid-oxide cells(RSOCs),including a comparison of power-to-fuel/fuel-to-power to other energy-conversion and storage technologies is *** electrochemistry and chemistry of H_(2)O,CO_(2),H_(2),CO,CnHm(hydrocarbons)and NH3,including thermodynamics and cell performance,are *** mechanical strength of popular cell supports is outlined,and newly found stronger materials are *** cell-degradation mechanisms,including the effect of common impurities in gases and materials(such as S and Si),plus the deleterious effects of carbon deposition in the fuel electrode are described followed by explanations of how to avoid or ease the *** of how RSOCs powered by sustainable energy may be applied on a large scale for the transportation sector via power-to-fuel technology and for integration with the electrical grid together with seasonal storage are ***,a brief comparison of RSOCs to other electrolysis cells and an outlook with examples of actions necessary to commercialize RSOC applications are sketched.

关键词： electrolysis fuel cells solid-oxide cells power-to-fuel electrochemical syngas

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