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Polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) emissions from electric arc furnaces for steelmaking

Emerging Contaminants 2020年第1期6卷 330-336页

作者： Qiuting Yang Lili Yang Jia Shen Yuanping Yang Minxiang Wang Xiaoyun Liu Xuejing Shen Changliang Li Jia Xu Fengfeng Li Da Li Guorui Liu Minghui Zheng Central Iron&Steel Research Institute Beijing100081China State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesP.O.Box 2871Beijing100085China School of Environment Hangzhou Institute for Advanced StudyUCASHangzhouChina

The proportion of steel produced using electric arc furnaces(EAFs)is *** this study,polychlorinated dibenzo-p-dioxins and dibenzofurans(PCDD/Fs)concentrations and patterns in stack gas samples from three typical EAFs in steelmaking plants were determined to allow the contributions of EAFs in steelmaking plants to PCDD/Fs emissions in China to be *** collection was accomplished by adopting the automatic isokinetic sampling technique,then the PCDD/Fs congeners concentrations were analyzed qualitatively and quantitatively by isotope dilution high-resolution gas chromatography high-resolution mass spectrometry(HRGC-HRMS).The mean PCDD/Fs mass concentrations in stack gases emitted during the scrap preheating phase of plants E1,E2,and E3 were 0.48,385.55,and 0.34 ng Nm^-3,respectively,and the total toxic equivalent(WHO2005-TEQ)concentrations were 0.05,33.16,and 0.03 ng Nm^-3,*** PCDD/Fs mass concentration in stack gases emitted during the melting phase at plant E3 was 0.12 ng Nm^-3(0.02 ng WHO2005-TEQ Nm^-3).The operational temperature of the bag filter of the preheating in the E2 EAF was as high as 230℃,which is conducive to the generation of PCDD/Fs,whether the temperature in the bag filter of E1(150℃)and E3(120℃)are ***,the bag filter temperature is suggested to be best controlled to below 150℃.The emission factors(EF)for PCDD/Fs released into the air during the scrap preheating phase for plants E1,E2,and E3 were 0.13,52,and 0.10 mg WHO2005-TEQ t1,respectively,and the EF for the smelting phase from plant E3 was 0.14 mg WHO2005-TEQ t*** emission factor in E2 is 5 times higher than the highest current UNEP toolkit factor for EAFs(10 mg TEQ/tonne steel).Therefore,an update for the UNEP toolkit emission factor for a few case plants is *** congeners,including 2,3,7,8-TeCDF,1,2,3,4,6,7,8-HpCDF,and 1,2,3,4,6,7,8-HpCDD,were dominant during the preheating phase,while 2,3,7,8-TeCDF,1,2,3,7,8-PeCDF,and 2,3,4,7,8-PeCDF

关键词： electric arc furnaces PCDD/Fs Stack gas Congener profile Emission factors

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Ultrasound effects on zinc recovery from EAF dust by sulfuric acid leaching

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International Journal of Minerals,Metallurgy and Materials 2015年第4期22卷 353-362页

作者： K.Brunelli M.Dabalà Department of Industrial Engineering University of Padua

In this work, an ultrasound-assisted leaching process was studied for the recovery of zinc from electric arc furnace （EAF） dust, in which zinc was mainly present in the form of franklinite （60%）. HydrometaUurgy is emerging as a preferred process for the recovery of a va- riety of metals, and the use of ultrasound could offer advantages over the conventional leaching process, especially for the dissolution of franklinite. Franklinite is a refractory phase that is difficult to leach and represents the main obstacle in conventional hydrometallurgy proc- essing. Atmospheric leaching with different sulfuric acid concentrations （0.2-2.0 M） at two temperatures （323 and 353 K） was performed. The tests were conducted using both conventional and ultrasound-assisted leaching. After the leaching tests, the solid residues were charac- terized by scanning electron microscopy （SEM） and X-ray diffraction （XRD） techniques, whereas the leach liquor was analyzed by induc- tively coupled plasma spectroscopy OCP）. The use of ultrasound facilitated the dissolution of franklinite at low acid concentrations and re- suited in a greater zinc recovery under all of the investigated operating conditions.

关键词： zinc recovery ultrasound electric arc furnaces dust leaching

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A novel robust adaptive controller for EAF electrode regulator system based on approximate model method

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Journal of Central South University 2012年第8期19卷 2158-2166页

作者：李磊毛志忠 School of Information Science and Engineering Northeastern University

The electrode regulator system is a complex system with many variables, strong coupling and strong nonlinearity, while conventional control methods such as proportional integral derivative （PID） can not meet the requirements. A robust adaptive neural network controller （RANNC） for electrode regulator system was proposed. Artificial neural networks were established to learn the system dynamics. The nonlinear control law was derived directly based on an input-output approximating method via the Taylor expansion, which avoids complex control development and intensive computation. The stability of the closed-loop system was established by the Lyapunov method. The current fluctuation relative percentage is less than ±8% and heating rate is up to 6.32 ℃/min when the proposed controller is used. The experiment results show that the proposed control scheme is better than inverse neural network controller （INNC） and PID controller （PIDC）.

关键词： approximate model electric arc furnaces nonlinear control normalized radial basis function neural network (NRBFNN)

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