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Degradation of dissolved organic matter in effluent of municipal wastewater plant by a combined tidal and subsurface flow constructed wetland

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Journal of Environmental Sciences 2021年第8期33卷 171-181页

作者： Chunjian Lyu Ruixia Liu Xiaojie Li Yonghui Song Hongjie Gao Basin Research Center for Water Pollution Control Chinese Research Academy of Environmental SciencesBeijing 100012China College of Water Sciences Beijing Normal UniversityBeijing 100875China

Dissolved organic matter(DOM)is an important constituent of wastewater treatment plant(WWTP)effluent.A novel combined tidal and subsurface flow constructed wetland(TF-SSFCW)of 90 L was constructed for a ten-month trial of advanced treatment of the WWTP *** emission matrix(EEM)fluorescence spectroscopy,parallel factor(PARAFAC)analysis and a two end-member mixing model were employed to characterize the composition and removal process of the effluent DOM(EfOM)from the *** results showed that the TF-SSF-CW performed an efficient EfOM removal with dissolved organic carbon(DOC)removal rate of 88%and dissolved organic nitrogen(DON)removal rate of 91%.Further analysis demonstrated that the EfOM consisted mainly of two protein moieties and two humic-like groups;protein moieties(76%)constituted the main content of EfOM in raw water and humic-like groups(57%)became the dominating contributor after *** EfOM from the WWTP was mainly of aquatic bacterial origin and evolved to a higher proportion of terrigenous origin with higher humification in the TF-SSF-CW effluent.A common controlling treatment-related factor for determining the concentrations of the same kind of substances(protein groups or humic-like groups)was revealed to exist,and the ratio of removal rates between the same substances in treatment was *** study demonstrates that the TF-SSF-CW can be a novel and effective treatment method for the EfOM from WWTPs,and is helpful for understanding of the character of EfOM in wetland treatment.

关键词： Constructed wetland effluent organic matter Excitation emission matrices PARAFAC analysis

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Formation of regulated and unregulated disinfection byproducts during chlorination and chloramination: Roles of dissolved organic matter type, bromide, and iodide

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Journal of Environmental Sciences 2022年第7期34卷 151-160页

作者： Yunsi Liu Keqiang Liu Michael J.Plewa Tanju Karanfil Chao Liu Key Laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China Water Conservancy Development Research Center Taihu Basin AuthorityMinistry of Water ResourcesShanghai 200433China Department of Crop Sciences and the Safe Global Water InstituteUniversity of Illinois at Urbana-ChampaignUrbanaIL 61801USA Department of Environmental Engineering and Earth Sciences Clemson UniversityAndersonSC 29625USA

Algal blooms and wastewater effluents can introduce algal organic matter(AOM) and effluent organic matter(Ef OM) into surface waters, respectively. In this study, the impact of bromide and iodide on the formation of halogenated disinfection byproducts(DBPs) during chlorination and chloramination from various types of dissolved organic matter(DOM, e.g., natural organic matter(NOM), AOM, and Ef OM) were investigated based on the data collected from literature. In general, higher formation of trihalomethanes(THMs) and haloacetic acids(HAAs) was observed in NOM than AOM and Ef OM, indicating high reactivities of phenolic moieties with both chlorine and monochloramine. The formation of haloacetaldehydes(HALs), haloacetonitriles(HANs) and haloacetamides(HAMs) was much lower than THMs and HAAs. Increasing initial bromide concentrations increased the formation of THMs, HAAs, HANs, and HAMs, but not HALs. Bromine substitution factor(BSF) values of DBPs formed in chlorination decreased as specific ultraviolet absorbance(SUVA) increased. AOM favored the formation of iodinated THMs(I-THMs) during chloramination using preformed chloramines and chlorination-chloramination processes. Increasing prechlorination time can reduce the I-THM concentrations because of the conversion of iodide to iodate, but this increased the formation of chlorinated and brominated DBPs. In an analogous way, iodine substitution factor(ISF) values of I-THMs formed in chloramination decreased as SUVA values of DOM increased. Compared to chlorination, the formation of noniodinated DBPs is low in chloramination.

关键词： Disinfection byproducts Natural organic matter Algal organic matter effluent organic matter Bromide Iodide Chlorination Chloramination

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Influence of EfOM on the Oxidation of Micropollutants by Ozone and UVIH2O2 in Secondary effluents

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Journal of Environmental Science and Engineering 2011年第6期5卷 789-798页

作者： S.P. Vieira R.F. Dantas S. Esplugas C. Sansx C. Sans M. Dezotti Federal University of Rio de Janeiro Rio de Janeiro 21941-972 Brazil Chemical Engineering Department University of Barcelona Barcelona Marti i Franquks 1 08028 Spain

The aim of this work was to study the influence of effluent organic matter （EfOM） on micropollutants removal by ozone and UV/H2O2. To perform the experiments, deionized water and municipal secondary effluents （SE） were artificially contaminated with atrazine （ATZ） and treated by the two proposed methods. ATZ concentration, COD and TOC were recorded along the reaction time and used to evaluate EfOM effect on the system efficiency. Results demonstrate that the presence of EfOM can significantly reduce the micropollutant removal rate due to competition of EfOM components to react with radicals and/or molecular ozone. The hydroxyl radical scavenging caused by EfOM was quantified as well as the contribution of molecular ozone and .OH radicals during the ozonation of SE. EfOM components promoted higher inhibition of ATZ oxidation by hydroxyl radicals than by molecular ozone.

关键词： Secondary effluents effluent organic matter UV/I-I202 ozonation atrazine pesticides

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