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electrolytic cell engineering and device optimization for electrosynthesis of e-biofuels via co-valorisation of bio-feedstocks and captured CO_(2)

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Frontiers of Chemical Science and engineering 2021年第1期15卷 208-219页

作者： Faraz Montazersadgh Hao Zhang Anas Alkayal Benjamin Buckley Ben W.Kolosz Bing Xu Jin Xuan Department of Chemical engineering Loughborough UniversityLoughboroughLE113TUUK Department of Chemistry Loughborough UniversityLoughboroughLE113TUUK Department of Chemical engineering Worcester Polytechnic InstituteWorcesterMA 01609-2280USA Department of Accountancy Economics and FinanceHeriot-Watt UniversityEdinburghEH144ASUK

Utilizing CO_(2) in an electro-chemical process and synthesizing value-added chemicals are amongst the few viable and scalable pathways in carbon capture and utilization ***_(2) electro-reduction is also counted as one of the main options entailing less fossil fuel consumption and as a future electrical energy storage *** current study aims at developing a new electrochemical platform to produce low-carbon e-biofuel through multifunctional electrosynthesis and integrated co-valorisation of biomass feedstocks with captured CO_(2).In this approach,CO_(2) is reduced at the cathode to produce drop-in fuels(e.g.,methanol)while value-added chemicals(e.g.,selective oxidation of alcohols,aldehydes,carboxylic acids and amines/amides)are produced at the *** this work,a numerical model of a continuous-flow design considering various anodic and cathodic reactions was built to determine the most techno-economically feasible configurations from the aspects of energy efficiency,environment impact and economical *** reactor design was then optimized via parametric analysis.

关键词： electrosynthesis e-biofuels CO_(2)utilization computational model

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