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Recent advances in metal-organic frameworks for catalytic CO_(2) hydrogenation to diverse products

Nano Research 2022年第12期15卷 10110-10133页

作者： Shengxian Shao Chengqian Cui Zhiyong Tang Guodong Li CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing100190China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing100049China

Selective hydrogenation of CO_(2) to high value-added chemicals,not only gives an effective way to reduce the concentration of CO_(2),but also provides the precursors to advance the industrial manufacturing of chemicals and *** the well-defined reticular frameworks and flexible modifiability,metal-organic frameworks(MOFs)can be the ideal platform to construct the enabled catalysts for CO_(2) hydrogenation,because they have shown the great potential for the enhancement of catalytic activity,the precise control of selectivity,and the excellent *** this review,we systematically summarize the recent advances in MOFs based catalysts for CO_(2) hydrogenation towards diverse ***,synthesis strategies for different kinds of MOFs based catalysts are ***,selective hydrogenation of CO_(2) towards CO and methane is discussed over various metal nanoparticles/MOFs ***,heterogenization and isolation of molecular catalysts by MOFs are elaborated for producing formic ***,selective hydrogenation of CO_(2) toward methanol is discussed in terms of interface structures of Cu,Zn,and metal nodes of MOFs,the synergy between auxiliary sites and noble metal,and tandem catalytic systems of molecular catalysts and Lewis acid ***,the integration of multiple metal sites,promoters,and cocatalysts into MOFs is described for the selective hydrogenation of CO_(2) to C2+*** those,the key issue about the stability of MOFs based catalysts for CO_(2) hydrogenation reaction is ***,the summary and perspective about MOFs based catalysts for selective CO_(2) hydrogenation and mechanism research are proposed.

关键词： selective CO_(2)hydrogenation metal-organic frameworks(MOFs) noble metal nonnoble metal diverse products mechanism

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