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Efficient removal of heavy metals from electroplating wastewater using polymer ligands

Frontiers of Environmental Science & Engineering 2016年第2期10卷 352-361页

作者： Md. Lutfor RAHMAN Shaheen M. SARKAR Mashitah Mohd YUSOFF Faculty of Industrial Sciences & Technology Universiti Malaysia Pahang 26300 Gambang Kuantan Malaysia

Poly（hydroxamic acid）-poly（amidoxime） che- lating ligands were synthesized from poly（methyl acrylate-co-acrylonitrile） grafted acacia cellulose for removing toxic metal ions from industrial wastewaters. These ligands showed higher adsorption capacity to copper （2.80 mmol. g-l） at pH 6. In addition, sorption capacities to other metal ions such as iron, zinc, chromium, and nickel were also found high at pH 6. The metal ions sorption rate （tl/2） was very fast. The rate of adsorption of copper, iron, zinc, chromium, nickel, cobalt, cadmium and lead were 4, 5, 7, 5, 5, 8, 9 and 11 min, respectively. Therefore, these ligands have an advantage to the metal ions removal using the column technique. We have successfully investigated the known concentration of metal ions using various parameters, which is essential for designing a fixed bed column with ligands. The wastewater from electroplating plants used in this study, having chromium, zinc, nickel, copper and iron, etc. For chromium wastewater, ICP analysis showed that the Cr removal was 99.8% and other metal ions such as Cu, Ni, Fe, Zn, Cd, Pb, Co and Mn removal were 94.7%, 99.2%, 99.9%, 99.9%, 99.5%, 99.9%, 95.6% and 97.6%, respectively. In case of cyanide wastewater, the metal removal, especially Ni and Zn removal were 96.5 and 95.2% at higher initial concentra- tion. For acid/alkali wastewater, metal ions removing for Cd, Cr and Fe were 99.2%, 99.5% and 99.9%, respectively. Overall, these ligands are useful for metal removal by column method from industrial wastewater especially plating wastewater.

关键词： heavy metals adsorption wastewater chelat-ing ligands plating industry

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