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Photoinduced difunctionalization with bifunctional reagents containing N-heteroaryl moieties

Science China Chemistry 2023年第6期66卷 1688-1700页

作者： Wooseok Lee Inyoung Park Sungwoo Hong Department of Chemistry Korea Advanced Institute of Science and Technology(KAIST)Daejeon 34141Republic of Korea Center for Catalytic Hydrocarbon Functionalizations Institute for Basic Science(IBS)Daejeon 34141Republic of Korea

bifunctional reagents that serve as dual coupling partners with an activating species have emerged as valuable synthetic tools in organic *** allow for the development of diverse reaction modes with enhanced efficiency and structural variability,which is in high demand for atom-economic and sustainable *** them,bifunctional reagents containing Nheteroaryl groups have received much attention due to their ability to introduce privileged N-heteroaryl moieties into complex molecules that are otherwise challenging to ***,these reagents have been employed under visible-light conditions to achieve various synthetic applications,enabling difunctionalization of alkenes,alkynes,and[1.1.1]propellanes under mild reaction conditions,providing access to highly functionalized *** this review,we provide an overview of the recent achievements and applications of photoinduced difunctionalization using bifunctional reagents containing N-heteroaryl *** systematically categorize the representative contributions in the field based on bifunctional reagents and their reactivity *** review aims to highlight the potential of these reagents as powerful synthetic tools for sustainable and diverse synthesis.

关键词： bifunctional reagents N-heteroarylation photoreaction difunctionalization radical reaction

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