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Latest Advances in High-Voltage and High-Energy-Density aqueous rechargeable batteries

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Electrochemical Energy Reviews 2021年第1期4卷 1-34页

作者： Xinhai Yuan Fuxiang Ma Linqing Zuo Jing Wang Nengfei Yu Yuhui Chen Yusong Zhu Qinghong Huang Rudolf Holze Yuping Wu Teunis van Ree Institute of Advanced Materials(IAM) School of Energy Science and EngineeringChina State Key Laboratory of Materials-Oriented Chemical EngineeringNanjing Tech UniversityNanjing 210009JiangsuChina Institute of Chemistry Saint Petersburg State UniversitySt.Petersburg 199034Russia Institute of Chemistry Chemnitz University of TechnologyAG ElektrochemieChemnitzGermany Department of Chemistry University of VendaThohoyandou 0950South Africa

aqueous rechargeable batteries(ARBs)have become a lively research theme due to their advantages of low cost,safety,environmental friendliness,and easy ***,since its inception,the aqueous solution energy storage sys-tem has always faced some problems,which hinders its development,such as the narrow electrochemical stability window of water,poor percolation of electrode materials,and low energy *** recent years,to overcome the shortcomings of the aqueous solution-based energy storage system,some very pioneering work has been done,which also provides a great inspiration for further research and development of future high-performance aqueous energy storage *** this paper,the latest advances in various ARBs with high voltage and high energy density are *** include aqueous rechargeable lithium,sodium,potassium,ammonium,zinc,magnesium,calcium,and aluminum *** chal-lenges are pointed out.

关键词： aqueous rechargeable batteries aqueous electrolyte High voltage High energy density

Progress in aqueous rechargeable batteries

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Green Energy & Environment 2018年第1期3卷 20-41页

作者： Jilei Liu Chaohe Xu Zhen Chen Shibing Ni ZeXiang Shen Division of Physics and Applied Physics School of Physical and Mathematical SciencesNanyang Technological University College of Aerospace Engineering Chongqing University College of Materials and Chemical Engineering China Three Gorges University

Over the past decades, a series of aqueous rechargeable batteries(ARBs) were explored, investigated and demonstrated. Among them,aqueous rechargeable alkali-metal ion(Li^+Na^+, K^+) batteries, aqueous rechargeable-metal ion(Zn^(2+),Mg^(2+), Ca^(2+), Al^(3+)) batteries and aqueous rechargeable hybrid batteries are standing out due to peculiar properties. In this review, we focus on the fundamental basics of these batteries, and discuss the scientific and/or technological achievements and challenges. By critically reviewing state-of-the-art technologies and the most promising results so far, we aim to analyze the benefits of ARBs and the critical issues to be addressed, and to promote better development of ARBs.

关键词： aqueous rechargeable batteries Hybrid Fundamental basics Challenges

Reinventing the mechanism of high-performance Bi anode in aqueous K^+ rechargeable batteries

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Journal of Energy Chemistry 2020年第9期29卷 21-28,I0002页

作者： Tingting Qin Xuefeng Chu Ting Deng Boran Wang Xiaoyu Zhang Taowen Dong Zhengming Li Xiaofeng Fan Xin Ge Zizhun Wang Peng Wang Wei Zhang Weitao Zheng State Key Laboratory of Automotive Simulation and Control and School of Materials Science&Engineeringand Electron Microscopy Centerand International Center of Future ScienceJilin UniversityChangchun 130012JilinChina Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074HubeiChina Key Laboratory of Architectural Cold Climate Energy Management Ministry of EducationJilin Jianzhu UniversityChangchun 130118JilinChina State Key Laboratory of Inorganic Synthesis&Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012JilinChina Basque Foundation for Science IKERBASQUEBilbao 48013Spain

Increasing attention has been paid to rechargeable aqueous batteries due to their high safety and low ***,they remain in their infancy because of the limited choice of available anode materials with high specific capacity and satisfying cycling *** metal with layered structure can act as an ideal anode material with high capacity;however,the energy storage mechanism has not well ***,we demonstrate that Bi metal enables affording ultra-high specific capacity(254.3 mAh g^-1),superior rate capability and a capacity retention of 88.8%after 1600 *** from the previously-reported redox reaction mechanisms of Bi electrode,efficient(de)alloying of K+is responsible for its excellent *** excellent aqueous Bi battery is fabricated by matching Bi anode with Co(OH)2 cathode in KOH(1 M)*** outstanding performance is quite adequate and competitive for electrochemical energy storage devices.

关键词： aqueous rechargeable batteries Bi anode K^+ Alloying Mechanism

Ultrahigh-energy and-power aqueous rechargeable zinc-ion microbatteries based on highly cation-compatible vanadium oxides

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Journal of Materials Science & Technology 2022年第25期120卷 159-166页

作者： Sheng-Bo Wang Qing Ran Wu-Bin Wan Hang Shi Shu-Pei Zeng Zi Wen Xing-You Lang Qing Jiang Key Laboratory of Automobile Materials(Jilin University) Ministry of Education and School of Materials Science and EngineeringJilin UniversityChangchun 130022China State Key Laboratory of Automotive Simulation and Control Jilin UniversityChangchun 130022China

aqueous multivalent-metal-ion intercalation chemistries hold genuine promise to develop safe and powerful microbatteries for potential use in many miniaturized ***,their development is beset by state-of-the-art electrode materials having practical capacities far below their theoretical *** we demonstrate that high compatibility between layered transition-metal oxide hosts and hydrated cation guests substantially boost their multi-electron-redox reactions to offer higher capacities and rate capability,based on typical bipolar vanadium oxides preintercalated with hydrated cations(M_(x)V_(2)O_(5)).When seamlessly integrated on Au current microcollectors with a three-dimensional bicontinuous nanoporous architecture that offers high pathways of electron transfer and ion transport,the constituent Zn_(x)V_(2)O_(5) exhibits specific capacity of as high as∼527 mAh g^(−1) at 5 mV s^(−1) and retains∼300 mAh g^(−1) at 200 mV s^(−1) in 1 M ZnSO_(4) aqueous electrolyte,outperforming the M_(x)V_(2)O_(5)(M=Li,Na,K,Mg).This allows aqueous rechargeable zinc-ion microbatteries constructed with symmetric nanoporous Zn_(x)V_(2)O_(5)/Au interdigital microelectrodes as anode and cathode to show high-density energy of∼358 mWh cm^(−3)(a value that is forty-fold higher than that of 4 V/500μAh Li thin film battery)at high levels of power delivery.

关键词： Multivalent metal ions aqueous rechargeable batteries Microbatteries Nanoporous metals Metal/oxide composites

吩嗪类衍生物用于快速充放电和长寿命的水系钾离子全电池负极

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Science China Materials 2024年第5期67卷 1464-1470页

作者：郑易帆于丹丹王健晨杨杰罗稳戈天奇秦来顺黄岳翔陈达 College of Materials and Chemistry China Jiliang UniversityHangzhou310018China Hydrogen Energy Research Center PetroChina Petrochemical Research Institute Beijing102200China

有机电极材料因具有结构多样性和可持续性,在水系钾离子电池研究领域展示出广阔的前景,但它们大多数存在导电性差、易溶于电解液的问题,导致电极活性物质利用率低、循环稳定性差.本文通过含氮苯环的共轭延申、引入氰基活性中心,获得了3C... 详细信息

有机电极材料因具有结构多样性和可持续性,在水系钾离子电池研究领域展示出广阔的前景,但它们大多数存在导电性差、易溶于电解液的问题,导致电极活性物质利用率低、循环稳定性差.本文通过含氮苯环的共轭延申、引入氰基活性中心,获得了3CN-HATN.与经#吩嗪负极相比,3CN-HATN的最低未占据分子轨道能级更低,更容易被还原,且其能带隙较窄,改善了导电性,其共轭结构可有效抑制循环过程中3CN-HATN的溶解.3CN-HATN负极在80 C(1 C=350 mA g^(-1))下比容量高达233.8 mA h g^(-1),将其与Ni(OH)_(2)正极匹配,构建的水系钾离子全电池具备优异的循环稳定性和快充性能,30 C下循环10,000圈后容量保持率达81.5%.

关键词： aqueous rechargeable batteries π-conjugated structure organic electrodes K+storage phenazine derivatives

Advanced Organic Materials for Nonmetallic Charge Carrier-Based batteries

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Renewables 2023年第5期1卷 541-561页

作者： Tao Sun Guanglei Ren Qi Jie Wu Mao song Liu Qian Yang Xingwen Cheng Yuqiao Zhang Long Zhang Shun Li Weidong Shi Jianming Zhang Institute of Quantum and Sustainable Technology(IQST) School of Chemistry and Chemical EngineeringJiangsu UniversityZhenjiang 212013(China)

Organic electrode materials(OEMs),withmerits of structural diversity,molecular-level controllability,resource abundance,and environmental friendliness,have become a promising electrode candidate for low-carbon renewable ***,environmentally benign,and sustainable aqueous rechargeable batteries are particularly appealing for large-scale energy storage *** review aims to provide an insightful discussion of OEMs in nonmetallic charge carrier-based batteries,especially for the application in aqueous rechargeable *** emerging application of OEMs in versatile aqueous batteries will be analyzed emphatically,including aqueous proton batteries,aqueous ammonium-ion batteries,and air self-charging *** expect that this review can serve as a guide for the future development of OEMs in nonmetallic charge carrier-based batteries and provide inspiration for unmet challenges.

关键词： aqueous rechargeable batteries organic electrode materials nonmetallic charge carrier electrochemistry