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anisotropic electrical properties of aligned PtSe_(2) nanoribbon arrays grown by a pre-patterned selective selenization process

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Nano Research 2022年第5期15卷 4668-4676页

作者： Huaipeng Wang Zhifang Liu Yilin Sun Xiaofan Ping Jianlong Xu Yingtao Ding Haowen Hu Dan Xie Tianling Ren School of Integrated Circuits Beijing National Research Center for Information Science and Technology(BNRist)Tsinghua UniversityBeijing 100084China Department of Chemistry Tsinghua UniversityBeijing 100084China School of Integrated Circuits and Electronics Beijing Institute of TechnologyBeijing 100081China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China State Key Lab of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

This study proposes a feasible and scalable production strategy to naturally obtain aligned platinum diselenide(PtSe_(2))nanoribbon arrays with anisotropic *** anisotropic properties of two-dimensional(2D)materials,especially transition-metal dichalcogenides(TMDs),have attracted great interest in *** dependence of physical properties on their lattice orientations is of particular interest because of its potential in diverse applications,such as nanoelectronics and ***-dimensional(1D)nanostructures facilitate many feasible production strategies for shaping 2D materials into unidirectional 1D nanostructures,providing methods to investigate the anisotropic properties of 2D materials based on their lattice orientations and *** natural alignment of zigzag(ZZ)PtSe_(2) nanoribbons is experimentally demonstrated using angle-resolved polarized Raman spectroscopy(ARPRS),and the selective growth mechanism is further theoretically revealed by comparing edges and edge energies of different orientations using the density functional theory(DFT).Back-gate field-effect transistors(FETs)are also constructed of unidirectional PtSe_(2) nanoribbons to investigate their anisotropic electrical properties,which align with the results of the projected density of states(DOS)*** work provides new insight into the anisotropic properties of 2D materials and a feasible investigation strategy from experimental and theoretical perspectives.

关键词： PtSe_(2) scalable production anisotropic properties nanoribbons density functional theory

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Serrated chip characteristics and formation mechanism in high-speed machining of selective laser melted Ti6Al4V alloys

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Science China(Technological Sciences) 2023年第5期66卷 1435-1450页

作者： LIU DeJian WANG YouQiang NI ChenBing ZHU LiDa ZHENG ZhongPeng School of Mechanical and Automotive Engineering Qingdao University of TechnologyQingdao266520China Key Lab of Industrial Fluid Energy Conservation and Pollution Control Ministry of EducationQingdao266520China School of Mechanical Engineering and Automation Northeastern UniversityShenyang110819China School of Mechanical Engineering Tsinghua UniversityBeijing100084China

Serrated chips,consisting of extremely uneven plastic deformation,are a prominent feature of high-speed machining of difficultto-machine *** paper focuses on the evolution of chip form,chip morphology features(chip free surface,tool-chip contact surface,and chip edge),and chip segment parameters in subsequent high-speed(vc=50 and 150 m min-1)machining of selective laser melted(SLMed)Ti6Al4V alloys,which are significantly different from conventional Ti6Al4V alloy in microstructure,mechanical properties and *** effect of laser beam scanning schemes(0°,67.5°,and 90°),machined surfaces(top and front),and cutting speeds on serrated chip characteristics of SLMed Ti6Al4Valloys was *** on the Johnson-Cook constitutive model of SLMed Ti6Al4Valloys,an orthogonal cutting model was developed to better understand the effect of physical-mechanical properties on the shear localization,which dominates the formation mechanism of serrated chips in post-machining of SLMed Ti6Al4V *** results showed that the critical cutting speed(CCS)for chip serration of SLMed Ti6Al4V alloy is lower than that for serrated chips of conventional Ti6Al4V alloy,and the serrated profile of SLMed Ti6Al4V chips was more regular and ***,due to anisotropic microstructure and mechanical properties of SLMed Ti6Al4Valloys,the serration degree of chips produced on the top surfaces of SLMed Ti6Al4Valloys is more prominent than that of chips generated on the front *** addition,because of the poor deformation coordination and high plastic flow stresses of needle-like martensiteα′,the plastic flow and grain distortion in the adiabatic shear band(ASB)of SLMed Ti6Al4V chips are significantly smaller than those in the ASB of conventional Ti6Al4V with equiaxed grains.

关键词： serrated chips selective laser melted Ti6Al4V alloys high-speed machining chip characteristics anisotropic properties

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First-principles investigations on structural stability,mechanical,and thermodynamic properties of LaT2Al20(T=Ti,V,Cr,Nb,and Ta) intermetallic cage compounds

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Chinese Physics B 2018年第12期27卷 397-404页

作者： Shanyu Quan Xudong Zhang Cong Liu Wei Jiang School of Science Shenyang University of TechnologyShenyang 110870China School of Materials Science and Engineering Shenyang University of TechnologyShenyang 110870China

First principles calculations were used to explore the structural stability, mechanical properties, and thermodynamic properties of LaT2Al20(T = Ti, V, Cr, Nb, and Ta) intermetallics. The calculated formation enthalpy and phonon frequencies indicate that LaT2Al20intermetallics exhibit the structural stability. The elastic moduli(B, G, E, and Hv) indicate that these intermetallics possess the better elastic properties than pure Al. The values of Poisson’s ratio v and B/G demonstrate that LaT2Al20intermetallics are all brittle materials. The anisotropy of elasticity and Young’s modulus(three-and two-dimensional figures) indicate that LaT2Al20compounds are anisotropic. Importantly, the calculated thermal quantities demonstrate that LaT2Al20intermetallics possess the better thermal physical properties than pure Al at high temperatures.

关键词： LaT_2Al_(20) intermetallics mechanical properties anisotropic properties dynamical and thermodynamic properties first-principles calculations

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Highly Aligned Graphene Aerogels for Multifunctional Composites

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Nano-Micro Letters 2024年第6期16卷 276-342页

作者： Ying Wu Chao An Yaru Guo Yangyang Zong Naisheng Jiang Qingbin Zheng Zhong‑Zhen Yu Beijing Advanced Innovation Center for Materials Genome Engineering School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083People’s Republic of China Institute of Materials Intelligent Technology Liaoning Academy of MaterialsShenyang 110004People’s Republic of China School of Science and Engineering The Chinese University of Hong KongShenzhenShenzhenGuangdong 518172People’s Republic of China State Key Laboratory of Organic‑Inorganic Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029People’s Republic of China

Stemming from the unique in-plane honeycomb lattice structure and the sp^(2)hybridized carbon atoms bonded by exceptionally strong carbon–carbon bonds,graphene exhibits remarkable anisotropic electrical,mechanical,and thermal *** maximize the utilization of graphene’s in-plane properties,pre-constructed and aligned structures,such as oriented aerogels,films,and fibers,have been *** unique combination of aligned structure,high surface area,excellent electrical conductivity,mechanical stability,thermal conductivity,and porous nature of highly aligned graphene aerogels allows for tailored and enhanced performance in specific directions,enabling advancements in diverse *** review provides a comprehensive overview of recent advances in highly aligned graphene aerogels and their *** highlights the fabrication methods of aligned graphene aerogels and the optimization of alignment which can be estimated both qualitatively and *** oriented scaffolds endow graphene aerogels and their composites with anisotropic properties,showing enhanced electrical,mechanical,and thermal properties along the alignment at the sacrifice of the perpendicular *** review showcases remarkable properties and applications of aligned graphene aerogels and their composites,such as their suitability for electronics,environmental applications,thermal management,and energy *** and potential opportunities are proposed to offer new insights into prospects of this material.

关键词： Highly aligned graphene aerogels Quantitative characterization of alignment Multifunctional composites anisotropic properties Multifunctional applications

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Recent advances in anisotropic two-dimensional materials and device applications

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Nano Research 2021年第4期14卷 897-919页

作者： Jinlai Zhao Dingtao Ma Cong Wang Zhinan Guo Bin Zhang Jianqing Li Guohui Nie Ni Xie Han Zhang Institute of Microscale Optoelectronics and Second Peoples Hospital Health Science CenterShenzhen UniversityShenzhen 518060China Faculty of Information Technology Macao University of Science and TechnologyAvenida Wai LongTaipaMacao 999078China College of Materials Science and Engineering Shenzhen Key Laboratory of Polymer Science and TechnologyGuangdong Research Center for Interfacial Engineering of Functional MaterialsShenzhen 518060China

Two-dimensional(2D)materials,such as transition metal dichalcogenides(TMDs),black phosphorus(BP),MXene and borophene,have aroused extensive attention since the discovery of graphene in *** have wide range of applications in many research fields,such as optoelectronic devices,energy storage,catalysis,owing to their striking physical and chemical *** them,anisotropic 2D material is one kind of 2D materials that possess different properties along different directions caused by the intrinsic anisotropic atoms5 arrangement of the 2D materials,mainly including BP,borophene,low-symmetry TMDs(ReSe2 and ReSa)and group IV monochalcogenides(SnS,SnSe,GeS,and GeSe).Recently,a series of new devices has been fabricated based on these anisotropic 2D *** this review,we start from a brief introduction of the classifications,crystal structures,preparation techniques,stability,as well as the strategy to discriminate the anisotropic characteristics of 2D ***,the recent advanced applications including electronic devices,optoelectronic devices,thermoelectric devices and nanomechanical devices based on the anisotropic 2D materials both in experiment and theory have been ***,the current challenges and prospects in device designs,integration,mechanical analysis,and micro-/nano-fabrication techniques related to anisotropic 2D materials have been *** review is aimed to give a generalized knowledge of anisotropic 2D materials and their current devices applications,and thus inspiring the exploration and development of other kinds of new anisotropic 2D materials and various novel device applications.

关键词： two-dimensional(2D)materials low-symmetry anisotropic properties black phosphorus device applications

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Physical properties of C-Si Alloys in C2/m Structure

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Communications in Theoretical Physics 2017年第8期67卷 259-268页

作者：王乾坤柴常春樊庆扬杨银堂 Key Laboratory of Ministry of Education for Wide Band-Gap Semiconductor Materials and Devices School of Microelectronics Xidian University

Using the first principles calculations based on density functional theory, the crystal structure, elastic anisotropy, and electronic properties of carbon, silicon and their alloys （C12Si4, C8Si8, and C4Si12） in a monoclinic structure （C2/m） are investigated. The calculated results such as lattice parameters, elastic constants, bulk modulus, and shear modulus of C16 and Si16 in C2/m structure are in good accord with previous work. The elastic constants show that C16, Si16, and their alloys in C2/m structure are mechanically stable. The calculated results of universal anisotropy index, compression and shear anisotropy percent factors indicate that C-Si alloys present elastic anisotropy, and CsSis shows a greater anisotropy. The Poisson＇s ratio and the BIG value show that C8Si8 is ductile material and other four C-Si alloys are brittle materials. In addition, Debye temperature and average sound velocity are predicted utilizing elastic modulus and density of C-Si alloys. The band structure and the partial density of states imply that C16 and Si16 are indirect band gap semiconductors, while 612Si4, C8Si8, and C4Si12 are semi-metallic alloys.

关键词： C-Si alloys elastic properties anisotropic properties electronic properties

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