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structure-regulated fluorine-containing additives to improve the performance of perovskite solar cells

Nano Research 2024年第7期17卷 6080-6086页

作者： Peiya Chen Xiaoman Bi Hao Yan Yingjie Zhao Yihao Liu Zhuo Huang Qian Xiao Yongpeng Yang Shasha Zhang Yiqiang Zhang Yanlin Song Henan Institute of Advanced Technology College of ChemistrySchool of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China Key Laboratory of Green Printing CAS Research/Education Center for Excellence in Molecular SciencesInstitute of ChemistryChinese Academy of Sciences(ICCAS)Beijing Engineering Research Center of Nanomaterials for Green Printing TechnologyNational Laboratory for Molecular Sciences(BNLMS)Beijing 100190China

Perovskite solar cells(PSCs)have seen remarkable progress in recent years,largely attributed to various additives that enhance both efficiency and *** these,fluorine-containing additives have garnered significant interest because of their unique hydrophobic properties,effective defect passivation,and regulation capability on the crystallization ***,a targeted structural approach to design such additives is necessary to further enhance the performance of ***,fluoroalkyl ethylene with different fluoroalkyl chain lengths(CH_(2)CH(CF_(2))nCF_(3),n=3,5,and 7)as liquid additives is used to investigate influences of fluoroalkyl chain lengths on crystallization regulation and defect *** findings indicate that optimizing the quantity of F groups plays a crucial role in regulating the electron cloud distribution within the additive *** optimization fosters strong hydrogen bonds and coordination effects with FA+and uncoordinated Pb^(2+),ultimately enhancing crystal quality and device ***,1H,1H,2H-perfluoro-1-hexene(PF_(3))with the optimal number of F presents the most effective modulation effect.A PSC utilizing PF_(3)achieves an efficiency of 24.05%,and exhibits exceptional stability against humidity and thermal *** work sheds light on the importance of tailored structure designs in additives for achieving high-performance PSCs.

关键词： perovskite solar cells fluorine number additive structure crystallization regulation defect passivation

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EFFICIENT ESTIMATION OF SEEMINGLY UNRELATED additive NONPARAMETRIC REGRESSION MODELS

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Journal of Systems Science & Complexity 2013年第4期26卷 595-608页

作者： YUAN Yuan YOU Jinhong ZHOU Yong School of Statistics and Management Shanghai University of Finance and Economics Academy of Mathematics and Systems Science Chinese Academy of Sciences

This paper is concerned with the estimating problem of seemingly unrelated(SU)nonparametric additive regression models.A polynomial spline based two-stage efficient approach is proposed to estimate the nonparametric components,which takes both of the additive structure and correlation between equations into *** asymptotic normality of the derived estimators are *** authors also show they own some advantages,including they are asymptotically more efficient than those based on only the individual regression equation and have an oracle property,which is the asymptotic distribution of each additive component is the same as it would be if the other components were known with *** simulation studies are conducted to illustrate the finite sample performance of the proposed *** the proposed procedure to a real data set is also made.

关键词： additive structure asymptotic normality nonparametric modelling polynomial spline seemingly unrelated regression two-stage estimation.

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