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Porous hybrid scaffold strategy for the realization of lightweight,highly efficient microwave absorbing materials

Journal of Materials Science & Technology 2022年第34期129卷 215-222页

作者： Meng Zhu Yuting Lei Heng Wu Luo Kong Hailong Xu Xuanxuan Yan Yongjian Xu Lei Dai Shaanxi Provincial Key Laboratory of Papermaking Technology and Specialty Paper Development Key Laboratory of Paper Based Functional MaterialsChina National Light IndustryNational Demonstration Center for Experimental Light Chemistry Engineering EducationShaanxi University of Science and TechnologyXi’an 710021China School of Engineering Computer and Mathematics SciencesAuckland University of Technology55 Wellesley Street EastAucklandNew Zealand School of Materials Science and Engineering Shaanxi University of Science and TechnologyXi’an 710021China Laboratory for Advanced Interfacial Materials and Devices Research Center for Smart Wearable TechnologyInstitute of Textiles and Clothingthe Hong Kong Polytechnic UniversityHong Kong SAR 999077China

Exploring an advanced and efficient electromagnetic(EM) wave absorbing material by improving dielectric loss capacity and adjusting impendence matching is crucial yet challenging. Herein, the bacterial cellulose(BC) derived carbon aerogel(CA) with a robust nanofibrous network was used as a conductive loss scaffold to dissipate EM waves effectively, and the Zn O microparticles with excellent dielectric properties and low electrical conductivity were decorated on the scaffold to adjust dielectric parameters and impedance matching adequately. By using different zinc precursors, the tunable size and morphologies of Zn O crystals were obtained due to the growth rate of different crystallographic, including flowerlike, nanorod like, and cauliflower-like morphologies, which is beneficial to strong multiple reflections,intensive interfacial polarization, better impendence matching, as well as excellent maintenance of the hierarchical structure. Owing to the appropriate impendence matching and the considerable EM wave dissipation, the CA@zno composites achieve a superior EM absorbing performance with a broad effective absorbing bandwidth(whole X band) and a minimum reflection coefficient(-53.3 d B). This work paves a new way for developing lightweight and highly efficient EM absorbing materials comprising the carbon scaffold and semiconductor microparticles.

关键词： Carbon scaffold zno microparticles Morphologies Impedance matching Microwave absorption

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