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Stability of mixed-halide wide bandgap perovskite solar cells: Strategies and progress

Journal of Energy Chemistry 2021年第10期30卷 395-415,I0011页

作者： Lei Tao Jian Qiu Bo Sun Xiaojuan Wang Xueqin Ran Lin Song Wei Shi Qi Zhong Ping Li Hui Zhang Yingdong Xia Peter Müller-Buschbaum Yonghua Chen Key Laboratory of Flexible Electronics(KLOFE)&Institution of Advanced Materials(IAM) Nanjing Tech University(Nanjing Tech)Nanjing 211816JiangsuChina Frontiers Science Center for Flexible Electronics Xi’an Institute of Flexible Electronics(IFE)and Xi’an Institute of Biomedical Materials&EngineeringNorthwestern Polytechnical UniversityXi’an 710072ShaanxiChina Key Laboratory of Advanced Textile Materials&Manufacturing Technology Ministry of EducationZhejiang Sci-Tech UniversityHangzhou 310018ZhejiangChina Lehrstuhl für Funktionelle Materialien Physik DepartmentTechnische Universität MünchenJames-Franck-Str.185748 GarchingGermany Heinz Maier-Leibnitz Zentrum(MLZ) Technische Universität MünchenLichtenbergstr.185748 GarchingGermany

Benefiting from the superior optoelectronic properties and low-cost manufacturing techniques,mixedhalide wide bandgap(WBG)perovskite solar cells(PSCs)are currently considered as ideal top cells for fabricating multi-junction or tandem solar cells,which are designed to beyond the Shockley-Queisser(S-Q)limit of single-junction solar ***,the poor long-term operational stability of WBG PSCs limits their further employment and hinders the marketization of multi-junction or tandem solar *** this review,recent progresses on improving environmental stability of mixed-halide WBG PSCs through different strategies,including compositional engineering,additive engineering,interface engineering,and other strategies,are ***,the outlook and potential direction are discussed and explored to promote the further development of WBG PSCs and their applications in multijunction or tandem solar cells.

关键词： Mixed halide perovskite Stability Tandem solar cells wide bandgap perovskite

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Strategies toward Highly Efficient Monolithic perovskite/Organic Tandem Solar Cells

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中国化学:英文版 2023年第14期41卷 1753-1768页

作者： Shan Jiang Zhiyang Xu Fuzhi Wang Shilei Tian Yang Wang Chenghao Li Zhan'ao Tan State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources North China Electric Power UniversityBeijing102206 China Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical TechnologyBeijing100029 China Department of Coal and Syngas Conversion Sinopec Research Institute of Petroleum ProcessingBeijing100083 China

Constructing monolithic tandem solar cells (TSCs) is an effective method to break the Shockley–Queisser (S–Q) radiative efficiency limit for single-junction solar cells. Employing the wide bandgap perovskite materials and low bandgap organic materials as absorber layers for front and rear subcells, respectively, to construct perovskite/organic TSCs can complementarily absorb sunlight in ultraviolet-visible (UV-Vis) range by front perovskite and near-infrared (NIR) range by rear organic molecules, thus reducing the thermalization energy losses. Besides the subcells, the interconnection layer (ICL), which physically and electrically connects the front and rear subcells, is also an important tunnel junction to recombine charges. In this review, we summarize the optimization strategies of wide bandgap perovskites for front subcell, narrow bandgap organic material for rear subcell, and the ICLs employed in monolithic perovskite/organic TSCs.

关键词： perovskite solar cells wide bandgap perovskite Low bandgap organic molecule Tandem solar cells Subcells Interconnection layer Efficiency Open-circuit voltage

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