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wettability gradient-Induced Diode:MXene-Engineered Membrane for Passive-Evaporative Cooling

Nano-Micro Letters 2024年第8期16卷 382-397页

作者： Leqi Lei Shuo Meng Yifan Si Shuo Shi Hanbai Wu Jieqiong Yang Jinlian Hu Department of Biomedical Engineering City University of Hong KongHong Kong S.A.R 999077China

Thermoregulatory textiles,leveraging high-emissivity structural materials,have arisen as a promising candidate for personal cooling management;however,their advancement has been hindered by the underperformed water moisture transportation capacity,which impacts on their thermophysiological comfort.Herein,we designed a wettability-gradient-induced-diode(WGID)membrane achieving by MXene-engineered electrospun technology,which could facilitate heat dissipation and moisture-wicking transportation.As a result,the obtained WGID membrane could obtain a cooling temperature of 1.5℃ in the“dry”state,and 7.1℃ in the“wet”state,which was ascribed to its high emissivity of 96.40%in the MIR range,superior thermal conductivity of 0.3349 W m^(-1) K^(-1)(based on radiation-and conduction-controlled mechanisms),and unidirectional moisture transportation property.The proposed design offers an approach for meticulously engineering electrospun membranes with enhanced heat dissipation and moisture transportation,thereby paving the way for developing more efficient and comfortable thermoregulatory textiles in a high-humidity microenvironment.

关键词： Passive-evaporative cooling MXene Electrospun membrane wettability gradient Diode

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Trilayered Fibrous Dressing with wettability gradient for Spontaneous and Directional Transport of Massive Exudate and Wound Healing Promotion

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Advanced Fiber Materials 2023年第2期5卷 574-587页

作者： Lei Liu Hengqiu Sun Jiaming Zhang Bingjie Xu Yujie Gao Dongming Qi Zhengwei Mao Jindan Wu MOE Key Laboratory of Advanced Textile Materials&Manufacturing Technology Zhejiang Sci-Tech UniversityHangzhou 310018China Department of Pediatric Surgery Taizhou Women and Children’s Hospital of Wenzhou Medical UniversityTaizhou 318000China MOE Key Laboratory of Macromolecular Synthesis and Functionalization Department of Polymer Science and EngineeringZhejiang UniversityHangzhou 310027China

Excessive exudate at wound sites increases treatment difficulty and severely decelerates the healing process.In wound exu-date management,dressings with unidirectional liquid transport capability have exhibited enormous potential.However,it remains challenging to improve the one-way liquid transport efficiency.Herein,a trilayered fibrous dressing is constructed by sequentially electrospinning polyurethane(PU)and polyvinylidene fluoride(PVDF)onto cotton fabric.Through hot pressing,a stable wettability gradient is formed across the PVDF/PU/cotton dressing due to the melting and bridging of PU nanofib-ers.The trilayered dressing exhibited rapid unidirectional transport with water penetrating from the hydrophobic side to the hydrophilic side in 6 s.The hydrostatic pressure from the hydrophilic side to the hydrophobic side is 569%higher than that from the hydrophobic side to the hydrophilic side,indicating that the dressing has a profound unidirectional conductivity.In vivo experiments demonstrates that the trilayered dressing can accelerate the wound healing process,especially in the early stages of wound occurrence,by quickly draining the excessive exudate.This study provides a new method to construct wound dressings with wettability gradients,which are advantageous for efficient exudate removal.

关键词： Trilayered fibrous dressing Exudate pumping PU nanofibers wettability gradient Wound healing

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On the spreading behavior of a droplet on a circular cylinder using the lattice Boltzmann method

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Chinese Physics B 2024年第6期33卷 434-443页

作者：杨帆金虎戴梦瑶 School of Energy and Power Engineering University of Shanghai for Science and TechnologyShanghai 200093China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering Shanghai 200093China

The study of a droplet spreading on a circular cylinder under gravity was carried out using the pseudo-potential lattice Boltzmann high-density ratios multiphase model with a non-ideal Peng–Robinson equation of state. The calculation results indicate that the motion of the droplet on the cylinder can be divided into three stages: spreading, sliding, and aggregating.The contact length and contact time of a droplet on a cylindrical surface can be affected by factors such as the wettability gradient of the cylindrical wall, the Bond number, and droplet size. Furthermore, phase diagrams showing the relationship between Bond number, cylinder wall wettability gradient, and contact time as well as maximum contact length for three different droplet sizes are given. A theoretical foundation for additional research into the heat and mass transfer process between the droplet and the cylinder can be established by comprehending the variable rules of maximum contact length and contact time.

关键词： lattice Boltzmann methods droplet circular cylinder wettability gradient

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Electrospinning Janus Nanofibrous Membrane for Unidirectional Liquid Penetration and Its Applications

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Chemical Research in Chinese Universities 2021年第3期37卷 337-354页

作者： HOU Lanlan LIU Jingchong LI Dianming GAO Yuan WANG Yaqiong HU Rongjun REN Wen XIE Shuixiang CUI Zhimin WANG Nü State Key Laboratory of Petroleum Pollution Control CNPC Research Institute of Safety and Environmental TechnologyBeijing102206P.R.China Key Laboratory of Bioinspired Smart Interfacial Science and Technology of Ministry of Education Beijing Key Laboratory of Bioinspired Energy Materials and DevicesSchool of ChemistryBeijing Advanced Innovation Center for Biomedical EngineeringBeihang UniversityBeijing100191P.R.China

Janus membrane with opposite wettability on its two sides has witnessed an explosion of interest in the field of liquid spontaneous and directional transport for their promising prospect.The advances in fabrication technology and natural bionics have brought remarkable progress for the development of Janus materials.Among the exciting progress,the micro/nanofabrication technique of electrospinning shows advantages in constructing thin porous fibrous membrane materials with controllable surface wettability and hierarchical structures.Here,a brief review of bioinspired Janus membrane for unidirectional liquid penetration fabricated by electrospinning is presented,and the underlying scientific mechanism is discussed with an emphasis on the materials design involving asymmetric surface wettability and micro-topology structure.An overview of recent emerging applications is also reviewed,with special attentions to liquid separation,water collection,distillation,and smart textile,etc.As researchers keep to develop more efficient strategies on designing new Janus membrane with higher performances,it has become increasingly important to understand the mechanism of liquid moving dynamics at the asymmetric interface in order to better recognize the scientific limitations currently hindering the field development.At last,the challenges currently faced and possible strategies on developing new Janus membranes for optimization and engineering in the future are proposed.

关键词： Electrospinning Nanofiber Janus membrane Unidirectional penetration wettability gradient

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