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Silver nanoparticles on UiO-66(Zr)metal-organic frameworks for water disinfection application

Food Science and Human Wellness 2022年第2期11卷 269-276页

作者： Hui Chen Chen Qiu Yiran Jiang Xinyu Liao Dan Wu Mofei Shen Tian Ding College of Biosystems Engineering and Food Science Zhejiang UniversityHangzhou 310058China

Drinking water disinfection is an essential process to assure public health all over the world.In this study,silver nanoparticles(AgNPs)on UiO-66(Zr)Metal-Organic Frameworks(Ag@UiO-66)is proposed as a potential water disinfection strategy.AgNPs are synthesized using polyvinyl pyrrolidone(PVP)as stabilizing agent,and sodium borohydride as reducing agent are subsequently embedded on UiO-66,a high-stability organometallic framework.The effect of premixing time,reaction time and reactant concentration on the loading rate of AgNPs on UiO-66 was investigated.The maximum load rate of AgNPs on UiO-66 could reach 13%when the premixing time is 3 h,the reaction time is 45 min and the concentration of AgNO_(3) is10μg/mL.The formation of AgNPs loaded on UiO-66 was observed and confirmed with ultraviolet and visible spectrophotometry(UV-Vis),scanning electron microscopy(SEM),infrared emission spectroscopy(IES)and X-ray diffraction(XRD)analysis.Ag@UiO-66 exhibited strong antibacterial activity against both Gramnegative Escherichia coli and Gram-positive Staphylococcus aureus,with minimum inhibitory concentrations(MIC)of 64 and 128μg/mL,respectively.The germicidal efficacy of Ag@UiO-66 enhanced significantly as the temperature rose from 4℃to 37℃.The results indicate that Ag@UiO-66 is potential candidate as a feasible water disinfection material.

关键词： Metal-organic framework Silver nanoparticles Antibacterial effects water disinfection

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Bacteria inactivation by sulfate radical:progress and non-negligible disinfection by-products

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Frontiers of Environmental Science & Engineering 2023年第3期17卷 23-36页

作者： Xin Zhou Xiaoya Ren Yu Chen Haopeng Feng Jiangfang Yu Kang Peng Yuying Zhang Wenhao Chen Jing Tang Jiajia Wang Lin Tang College of Environmental Science and Engineering Hunan UniversityChangsha 410082China Key Laboratory of Environmental Biology and Pollution Control(Hunan University) Ministry of EducationChangsha 410082China

Sulfate radicals have been increasingly used for the pathogen inactivation due to their strong redox ability and high selectivity for electron-rich species in the last decade.The application of sulfate radicals in water disinfection has become a very promising technology.However,there is currently a lack of reviews of sulfate radicals inactivated pathogenic microorganisms.At the same time,less attention has been paid to disinfection by-products produced by the use of sulfate radicals to inactivate microorganisms.This paper begins with a brief overview of sulfate radicals’properties.Then,the progress in water disinfection by sulfate radicals is summarized.The mechanism and inactivation kinetics of inactivating microorganisms are briefly described.After that,the disinfection by-products produced by reactions of sulfate radicals with chlorine,bromine,iodide ions and organic halogens in water are also discussed.In response to these possible challenges,this article concludes with some specific solutions and future research directions.

关键词： Sulfate radicals disinfection by-products Inactivation mechanisms Bacterial inactivation water disinfection

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Regulating crystallinity in linear conjugated polymer to boost the internal electric field for remarkable visible-light-driven disinfection

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Journal of Materials Science & Technology 2023年第6期137卷 26-35页

作者： Dawei Zhang Chengling Yang Hanwen Wang Yukun Yan Zhanyong Wang Xiangrong Li Yan Liang Jinsong Zhang Jun Xiao Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China College of Bioscience and Biotechnology Shenyang Agricultural UniversityShenyang 110866China College of Light Industry Liaoning UniversityShenyang 110036China

Conjugated linear polymers are promising metal-free photocatalysts for visible-light-driven photocatalytic water disinfection,but it was still bottlenecked by the insufficient photogenerated charge separation and transport(CST)process.Herein,we obtained the highly crystalline imine-linked conjugated linear poly-mer(ODA-BPAH)with a greatly enhanced CST process.The highly crystalline ODA-BPAH exhibited excel-lent broad-spectrum water disinfection efficiency up to 99.99999%in 1 h,which is among the reported highest of state-of-the-art photocatalysts.The crystallinity of ODA-BPAH was regulated by simply turn-ing the solvent and the experiment results revealed that the ODA-BPAH with high crystallinity exhibited higher internal electric field strength and photocatalytic performance than that with low crystallinity,which indicates that higher crystallinity in linear conjugated polymers contributes to superior CST ef-ficiency as well as the generation of reactive oxygen species.This work highlights the impact of poly-mer crystallinity on the internal electric field and proves that linear poly-imine could be a new type of promising metal-free photocatalyst for water treatment.

关键词： Polymeric photocatalysts water disinfection Imine-linked conjugated polymer High crystallinity Internal electric field

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E. coli and bacteriophage MS2 disinfection by UV, ozone and the combined UV and ozone processes

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Frontiers of Environmental Science & Engineering 2014年第4期8卷 547-552页

作者： Jingyun FANG Huiling LIU Chii SHANG Minzhen ZENG Mengling NI Wei LIU State Key Laboratory of Urban water Resources and Environment Harbin Institute of Technology Harbin 150090 China School of Environmental Science and Technology Sun Yat-Sen University Guangzhou 510275 China Department of Civil and Environmental Engineering the Hong Kong University of Science and Technology Hong Kong China water & Urban Development AECOM Asia Co. Ltd. Hung Kong China

The combination of low-dose ozone with ultraviolet （UV） irradiation should be an option to give benefit to disinfection and reduce drawbacks of UV and ozone disinfection. However, less is known about the disinfection performance of UV and ozone （UV/ozone） coexposure and sequential UV-followed-by-ozone （UV- ozone） and ozone-followed-by-UV （ozone-UV） expo- sures. In this study, inactivation of E. coli and bacterioph- age MS2 by UV, ozone, UV/ozone coexposure, and sequential UV-ozone and ozone-UV exposures was investigated and compared. Synergistic effects of 0.5-0.9 log kill on E. coli inactivation, including increases in the rate and efficiency, were observed after the UV/ozone coexposure at ozone concentrations as low as 0.05 mg-L-1 in ultrapure water. The coexposure with 0.02-mg.L-1 ozone did not enhance the inactivation but repressed E. coli photoreactivation. Little enhancement on E. coli inactivation was found after the sequential UV-ozone or ozone-UV exposures. The synergistic effect on MS2 inactivation was less significant after the UV/ozone coexposure, and more significant after the sequential ozone-UV and UV-ozone exposures, which was 0.2 log kill for the former and 0.8 log kill for the latter two processes, at ozone dose of 0.1 mg. t-1 and UV dose of 8.55 mJ. cm 2 in ultrapure water. The synergistic effects on disinfection were also observed in tap water. These results show that the combination of UV and low-dose ozone is a promising technology for securing microbiological quality of water.

关键词： bacteria inactivation photoreactivation water disinfection UV ozone

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Impact of density of coating agent on antibacterial activity of silver nanoparticle impregnated plasma treated activated carbon

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Journal of Environmental Sciences 2018年第5期30卷 136-144页

作者： Pritam Biswas Rajdip BANDyopadhyaya Department of Chemical Engineering Indian Institute of Technology Bombay

To use stabilized nanoparticles（NPs） in water as disinfectants over a very long period, the amount of coating agent（for NP stabilization） needs to be optimized. To this end, silver nanoparticles（Ag-NPs） with two different coating densities of tri-sodium citrate（12.05 and46.17 molecules/nm2, respectively）, yet of very similar particle size（29 and 27 nm, respectively）were synthesized. Both sets of citrate capped NPs were then separately impregnated on plasma treated activated carbon（AC）, with similar Ag loading of 0.8 and 0.82 wt.%, respectively. On passing contaminated water（containing 10~4 CFU Escherichia coli/m L of water） through a continuous flow-column packed with Ag/AC, zero cell concentration was achieved in 22 and 39 min, with Ag-NPs（impregnated on AC, named as Ag/AC） having lower and higher coating density, respectively. Therefore, even on ensuring similar Ag-NP size and loading, there is a significant difference in antibacterial performance based on citrate coating density in Ag/AC.This is observed in lower coating density case, due to both：（i） higher Ag~＋ ion release from Ag-NP and（ii） stronger binding of individual Ag-NPs on AC. The latter ensures that, Ag-NP does not detach from the AC surface for a long duration. TGA-DSC shows that Ag-NPs with a low coating density bind to AC with 4.55 times higher adsorption energy, compared to Ag/AC with a high coating density, implying stronger binding. Therefore, coating density is an important parameter for achieving higher antibacterial efficacy, translating into a faster decontamination rate in experiments, over a long period of flow-column operation.

关键词： Silver nanoparticles Activated carbon Escherichia coliCitrate coating Coating density water disinfection

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医院消毒研讨会在北京召开

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中国消毒学杂志 1991年第4期 207-208页

作者：李荣芬

由中华预防医学会消毒学会主办的全国医院消毒研讨会于1991年11月26日～28日在北京召开。与会代表140多人,交流论文80余篇。刘育京、袁洽劻、王枢群三位专家作了有关医院消毒的专题报告。同时举办了消毒药械展览。代表们一致反映收获很... 详细信息

由中华预防医学会消毒学会主办的全国医院消毒研讨会于1991年11月26日～28日在北京召开。与会代表140多人,交流论文80余篇。刘育京、袁洽劻、王枢群三位专家作了有关医院消毒的专题报告。同时举办了消毒药械展览。代表们一致反映收获很大,希望多办这样的专题性学术会议。

关键词： Bdellovibrio bacteriovorus water disinfection total bacterial count

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