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Application of different fiber structures and arrangements by electrospinning in triboelectric nanogenerators

Chinese Journal of Chemical Engineering 2024年第5期69卷 177-191页

作者： Hebin Li Zifei Meng Dehua Wang Ye Lu Longlong Jiang Le Zhang Hanbin Wang Xiaoxiong Wang College of Physics Qingdao UniversityQingdao 266071China School of Physics and Electronic Engineering Jiangsu Normal UniversityXuzhouJiangsu 221000China Microsystem&Terahertz Research Center China Academy of Engineering Physics(CAEP)Chengdu 610200China Institute of Electronic Engineering China Academy of Engineering Physics(CAEP)Mianyang 621900China University-Industry Joint Center for Ocean Observation and Broadband Communication College of PhysicsQingdao UniversityQingdao 266071China Weihai Innovation Research Institute of Qingdao University Weihai 264200China Collaborative Innovation Center for Eco-Textiles of Shandong Province and State Key Laboratory of Bio-Fibers and Eco-TextilesQingdao UniversityQingdao 266071China

In recent years,nanogenerators(NGs)have attracted wide attention in the energy field,among which triboelectric nanogenerators(TENGs)have shown superior performance.Multiple reports of electrospinning(ES)-based TENGs have been reported,but there is a lack of deep analysis of the designing method from microstructure,limiting the creative of new ES-based TENGs.Most TENGs use polymer materials to achieve corresponding design,which requires structural design of polymer materials.The existing polymer molding design methods include macroscopic molding methods,such as injection,compression,extrusion,calendering,etc.,combined with liquid-solid changes such as soluting and melting;it also includes micro-nano molding technology,such as melt-blown method,coagulation bath method,ES method,and nanoimprint method.In fact,ES technology has good controllability of thickness dimension and rich means of nanoscale structure regulation.At present,these characteristics have not been reviewed.Therefore,in this paper,we combine recent reports with some microstructure regulation functions of ES to establish a more general TENGs design method.Based on the rich microstructure research results in the field of ES,much more new types of TENGs can be designed in the future.

关键词： triboelectric nanogenerators Electrospinning Fiber microstructure regulation Nanomaterials Membranes Global optimization

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triboelectric nanogenerators as wearable power sources and self-powered sensors

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National Science Review 2023年第1期10卷 28-48页

作者： Xiong Pu Chi Zhang Zhong Lin Wang CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-Nano Energy and Sensor Beijing Institute of Nanoenergy and NanosystemsChinese Academy of Sciences School of Nanoscience and Technology University of Chinese Academy of Sciences School of Materials Science and Engineering College of EngineeringGeorgia Institute of Technology

Smart we arable technologies are augmenting human bodies beyond our biological capabilities in communication,healthcare and recreation.Energy supply and information acquisition are essential for wearable electronics,whereas the increasing demands in multifunction are raising the requirements for energy and sensor devices.The triboelectric nanogenerator(TENG),proven to be able to convert various mechanical energies into electricity,can fulfill either of these two functions and therefore has drawn extensive attention and research efforts worldwide.The everyday life of a human body produces considerable mechanical energies and,in the meantime,the human body communicates mainly through mechanical signals,such as sound,body gestures and muscle movements.Therefore,the TENG has been intensively studied to serve as either wearable sources or wearable self-powered sensors.Herein,the recent finding on the fundamental understanding of TENGs is revisited briefly,followed by a summary of recent advancements in TENG-based wearable power sources and self-powered sensors.The challenges and prospects of this area are given as well.

关键词： triboelectric nanogenerators power sources self-powered sensors wearable electronics

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Harvesting Environment Mechanical Energy by Direct Current triboelectric nanogenerators

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Nano-Micro Letters 2023年第8期15卷 381-404页

作者： Chuncai Shan Kaixian Li Yuntao Cheng Chenguo Hu School of Physics Chongqing UniversityChongqing 400044People’s Republic of China School of Energy and Engineering Chongqing UniversityChongqing 400044People’s Republic of China

As hundreds of millions of distributed devices appear in every corner of our lives for information collection and transmission in big data era,the biggest challenge is the energy supply for these devices and the signal transmission of sensors.triboelectric nanogenerator(TENG)as a new energy technology meets the increasing demand of today’s distributed energy supply due to its ability to convert the ambient mechanical energy into electric energy.Meanwhile,TENG can also be used as a sensing system.Direct current triboelectric nanogenerator(DC-TENG)can directly supply power to electronic devices without additional rectification.It has been one of the most important developments of TENG in recent years.Herein,we review recent progress in the novel structure designs,working mechanism and corresponding method to improve the output performance for DC-TENGs from the aspect of mechanical rectifier,tribovoltaic effect,phase control,mechanical delay switch and air-discharge.The basic theory of each mode,key merits and potential development are discussed in detail.At last,we provide a guideline for future challenges of DC-TENGs,and a strategy for improving the output performance for commercial applications.

关键词： triboelectric nanogenerators Direct current Working mechanism

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Contact Electrification Spectrum for Performance Enhancement Mechanism Investigation of triboelectric nanogenerators based on Silicone Elastomers with Different Surface Microstructures

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高分子科学:英文版 2023年第10期41卷 1591-1598页

作者： Jianliang Gong Shenyang Ye Yan Luo Liqiong Xia Bingyu Liu Yiwang Chen National Engineering Research Center for Carbohydrate Synthesis/Key Laboratory of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education College of Chemistry and Chemical EngineeringJiangxi Normal UniversityNanchang330022China Institute of Polymers and Energy Chemistry(IPEC)/Jiangxi Provincial Key Laboratory of New Energy Chemistry Nanchang UniversityNanchang330031China

triboelectric nanogenerators(TENGs)based on conjunctive effects of contact electrification(CE)and electrostatic induction are emerging as a new mechanical energy harvesting and sensing technique for promising applications in smart wearables,Internet of Things(IoTs),etc.The surface microstructure of a flexible triboelectric material for the increase of surface area is a common strategy for performance enhancement of TENGs,but the real roles of surface microstructures on their output performance are still not explicit due to the lack of suitable analysis tool and rational experimental design.Taking advantages of the surface-sensitive characteristic of CE effect,this work exploited and developed the electric signal patterns generated by single impact of TENGs as a kind of CE spectrum to analyze and speculate the real roles of surface microstructures of flexible triboelectric materials on the output performance of TENGs.Firstly,four different kinds of surface microstructures,namely planar surface(PS)and three combinations of two basic surface microstructures,i.e.,micro lens arrays(MLAs),fabric textures(FTs),and hierarchical structures of MLAs on FTs(MLA/FTs),were elaborately designed and introduced for an identical triboelectric material(i.e.,silicone elastomer)by a(micro)molding synthesis route.Then they were used for assembly of TENGs based on vertical contact mode to conduct performance evaluation under the same triggering conditions.Through systematic analysis and comparison of their highly repeatable CE spectra by programmed machine,it was found that the surface microstructure for a flexible triboelectric material to maximally enhance the output performance of a TENG shall achieve a positive synergistic effect of increasing triboelectric charge density,effective contact area and contacting/separating velocity,rather than simple increase of its surface area.

关键词： Contact electrification spectrum Silicone elastomer Surface microstructures triboelectric nanogenerators Enhancement mechanism

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A Review of Contact Electrification at Diversified Interfaces and Related Applications on triboelectric Nanogenerator

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Nano-Micro Letters 2024年第1期16卷 106-130页

作者： Jun Hu Mitsumasa Iwamoto Xiangyu Chen CAS Center for Excellence in Nanoscience Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083People’s Republic of China School of Nanoscience and Engineering University of Chinese Academy of SciencesBeijing 100049People’s Republic of China Department of Physical Electronics Tokyo Institute of Technology2‑12‑1 S3‑33 O‑OkayamaMeguro‑KuTokyo 152‑8552Japan

The triboelectric nanogenerator(TENG)can effectively collect energy based on contact electrification(CE)at diverse interfaces,including solid–solid,liquid–solid,liquid–liquid,gas–solid,and gas–liquid.This enables energy harvesting from sources such as water,wind,and sound.In this review,we provide an overview of the coexistence of electron and ion transfer in the CE process.We elucidate the diverse dominant mechanisms observed at different interfaces and emphasize the interconnectedness and complementary nature of interface studies.The review also offers a comprehensive summary of the factors influencing charge transfer and the advancements in interfacial modification techniques.Additionally,we highlight the wide range of applications stemming from the distinctive characteristics of charge transfer at various interfaces.Finally,this review elucidates the future opportunities and challenges that interface CE may encounter.We anticipate that this review can offer valuable insights for future research on interface CE and facilitate the continued development and industrialization of TENG.

关键词： Contact electrification Interfaces triboelectric nanogenerators Diversified applications

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Fully Fabric-Based triboelectric nanogenerators as Self-Powered Human-Machine Interactive Keyboards

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Nano-Micro Letters 2021年第7期13卷 42-54页

作者： Jia Yi Kai Dong Shen Shen Yang Jiang Xiao Peng Cuiying Ye Zhong Lin Wang School of Physical Science and Technology Guangxi UniversityNanning 530004People’s Republic of China CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-Nano Energy and SensorBeijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083People’s Republic of China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049People’s Republic of China School of Material Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332-0245USA

Combination flexible and stretchable textiles with self-powered sensors bring a novel insight into wearable functional electronics and cyber security in the era of Internet of Things.This work presents a highly flexible and self-powered fully fabric-based triboelectric nanogenerator(F-TENG)with sandwiched structure for biomechanical energy harvesting and real-time biometric authentication.The prepared F-TENG can power a digital watch by low-frequency motion and respond to the pressure change by the fall of leaves.A self-powered wearable keyboard(SPWK)is also fabricated by integrating large-area F-TENG sensor arrays,which not only can trace and record electrophysiological signals,but also can identify individuals’typing characteristics by means of the Haar wavelet.Based on these merits,the SPWK has promising applications in the realm of wearable electronics,self-powered sensors,cyber security,and artificial intelligences.

关键词： triboelectric nanogenerators Self-powered keyboard Human-machine interface Wearable electronics Fully fabric-based

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triboelectric nanogenerators for clinical diagnosis and therapy:A report of recent progress

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Medicine in Novel Technology and Devices 2022年第4期16卷 390-407页

作者： Yichang Quan Xujie Wu Simian Zhu Xiangyu Zeng Zhu Zeng Qiang Zheng Key Laboratory of Infectious Immune and Antibody Engineering of Guizhou Province Engineering Research Center of Cellular Immunotherapy of Guizhou ProvinceSchool of Biology and Engineering/School of Basic Medical SciencesGuizhou Medical UniversityGuiyang550025China Immune Cells and Antibody Engineering Research Center of Guizhou Province Key Laboratory of Biology and Medical EngineeringGuizhou Medical UniversityGuiyang550025China

triboelectric nanogenerators(TENGs)are considered as an ideal platform for power harvesting for living organisms,thanks to their unique characteristics like flexibility,conversion efficient,and manufacturing cost.Recent advances in TENGs have brought innovative solutions for clinical healthcare.Particularly,TENGs offer novel solutions of continues power supply for wearable and implantable medical devices with lightweight,thinness,good biocompatibility,and excellent soft tissue conformability.In this review,we discuss(1)The working principle and representative structure of TENGs,(2)the material selection of TENGs,(3)the recent progression of application of TENG in the medical field of cardiovascular system,nervous system,respiratory system,microbial inactivation,antibiofouling,disinfection,and tissue repair,(4)challenges and future perspectives of TENG-based medical devices.The emerging TENGs and their applications in medicine cannot simply be seen as an alternative to conventional power supplies,it provides a revolutionary solution for wearable and implantable medical devices,and they will surely change the paradigm of disease diagnosis and treatment in the future.

关键词： triboelectric nanogenerators Wearable and implantable medical devices Self-powered medical services Diagnostic and therapeutic applications

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Recent Progress of Functional Fiber and Textile triboelectric nanogenerators:Towards Electricity Power Generation and Intelligent Sensing

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Advanced Fiber Materials 2021年第6期3卷 394-412页

作者： Wei Wang Aifang Yu Junyi Zhai Zhong Lin Wang CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-Nano Energy and SensorBeijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049China Center On Nanoenergy Research School of Physical Science and TechnologyGuangxi UniversityNanning 530004China School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332-0245USA

Rapid development in wearable electronics has brought huge convenience to human life and gradually penetrated into various indispensable felds,such as health monitoring,medical assistance,smart sports,object tracking and smart home,etc.However,the suitable energy supply system for these wearable electronics remains an important issue to address.Fiber and textile triboelectric nanogenerators(f/t-TENGs),capable of converting biomechanical energy into electricity,have promising features to act as a mobile sustainable power source for wearable electronics or directly serve as an intelligent self-powered sensing solution.Compared with the low-output piezoelectric nanogenerators,hard-to-wear electromagnetic generators and other bulk TENGs,the fber/textile TENG may be the best type of wearable human mechanical energy harvester at present.Herein,this review comprehensively introduces the recent progress of smart fbers and textiles with a highlight on triboelectric nanogenerators,including the general materials and structures of fber/textile shaped electronics,various fber and textile devices for triboelectric/triboelectric-integrated energy harvesting and self-powered smart sensing systems.Moreover,the advance of f/t-TENGs with multifunctionality and large-scale textile processing techniques is summarized as well.Finally,the challenges and perspectives of f/t-TENGs for future improvement,large-scale production and emerging applications are thoroughly discussed as well.

关键词： Smart fber and textile triboelectric nanogenerators Energy harvesting Intelligent sensing Wearable electronics

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Eutectogel-based self-powered wearable sensor for health monitoring in harsh environments

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Nano Research 2024年第6期17卷 5559-5568页

作者： Junpeng Wu Xinru Teng Lu Liu Hongzhi Cui Xiaoyi Li College of Materials Science and Engineering Ocean University of ChinaQingdao 266100China Key Lab for Special Functional Materials of Ministry of Education School of Materials Science and EngineeringHenan UniversityKaifeng 475004China

triboelectric nanogenerators(TENG)have emerged as a highly promising energy harvesting technology,attracting significant attention in recent years for their broad applications.Gel-based TENGs,with superior stretchability and sensitivity,have been widely reported as wearable sensors.However,the traditional hydrogel-based TENGs suffer from freezing at low temperatures and drying at high temperatures,resulting in malfunctions.In this study,we introduce an anti-freezing eutectogel,which uses a deep eutectic solvent(DES),to improve the stability and electrical conductivity of TENGs in harsh environmental conditions.The eutectogel-based TENG(E-TENG)produces an open-circuit voltage of 776 V,a short-circuit current of 1.54μA,and a maximum peak power of 1.1 mW.Moreover,the E-TENG exhibits exceptional mechanical properties with an elongation at a break of 476%under tension.Importantly,it maintains impressive performances across a wide temperature range from−18 to 60℃,with conductivities of 2.15 S/m at−10℃and 1.75 S/m at−18℃.Based on the excellent weight stability of the E-TENG sensor,motion sensing can be achieved in the air,and even underwater.Finally,the versatility of the E-TENG can serve as a wearable sensor,by integrating it with Bluetooth technology.The self-powered E-TENG can monitor various human motion signals in real-time and send the health signals directly to mobile phones.This research paves a new road for the applications of TENGs in harsh environments,offering wireless flexible sensors with real-time health signal monitoring capabilities.

关键词： triboelectric nanogenerators self-powered harsh environment health monitoring Eutectogel

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Self-charging power textiles integrating energy harvesting triboelectric nanogenerators with energy storage batteries/supercapacitors

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Journal of Semiconductors 2021年第10期42卷 57-70页

作者： Kai Dong Zhong Lin Wang Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 100083China College of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049China School of Material Science and Engineering Georgia Institute of TechnologyAtlantaGeorgia 30332USA

Lightweight and flexible self-charging power systems with synchronous energy harvesting and energy storage abilities are highly desired in the era of the internet of things and artificial intelligences,which can provide stable,sustainable,and autonomous power sources for ubiquitous,distributed,and low-power wearable electronics.However,there is a lack of comprehensive review and challenging discussion on the state-of-the-art of the triboelectric nanogenetor(TENG)-based self-charging power textiles,which have a great possibility to become the future energy autonomy power sources.Herein,the recent progress of the self-charging power textiles hybridizing fiber/fabric based TENGs and fiber/fabric shaped batteries/supercapacitors is comprehensively summarized from the aspect of textile structural designs.Based on the current research status,the key bottlenecks and brighter prospects of self-charging power textiles are also discussed in the end.It is hoped that the summary and prospect of the latest research of self-charging power textiles can help relevant researchers accurately grasp the research progress,focus on the key scientific and technological issues,and promote further research and practical application process.

关键词： self-charging power textiles triboelectric nanogenerators energy harvesting batteries/supercapacitors energy storage power management system

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