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Recent Advances in the Synthesis of Zeolites from Solid Wastes

Chemical Research in Chinese Universities 2024年第4期40卷 646-656页

作者： LIU Pei WU Qinming CHEN Zhenghai XIAO Feng-Shou Key Laboratory of Biomass Chemical Engineering of Ministry of Education and College of Chemical and Biological Engineering Zhejiang UniversityHangzhou310028P.R.China Zhejiang Provincial Innovation Center of Green Petrochemical Technology Ningbo315048P.R.China Kente Catalysts Inc. Xianju317300P.R.China

With the rapid development of industrialization,it is inevitable to produce solid wastes in the fields of energy petrochemical ***,the storage and utilization of these solid wastes have become a considerable *** to the main element composition of these solid wastes including silicon and aluminum,it has attracted extensive attention for synthesizing *** review summarized the properties of major solid wastes including coal fly ash,coal gangue,spent fluid catalytic cracking(FCC)catalyst,lithium slag,bauxite residue,and waste ***,the preparation of LTA,FAU,ZSM-5,SSZ-13,Beta,and MOR zeolites from these solid wastes were ***,the current challenges and perspectives were discussed.

关键词： Solid waste Zeolite Utilization sustainable route Application

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Solvent-Free Synthesis of ITQ-12, ITQ-13, and ITQ-17 Zeolites

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Chinese Journal of Chemistry 2017年第5期35卷 572-576页

作者： Qinming Wu Xiaolong Liu Longfeng Zhu Xiangju Meng Feng Deng Fengtao Fan Zhaochi Feng Can Li Stefan Maurer Mathias Feyen Ulrich Muller Feng-Shou Xiao Key Lab of Applied Chemistry of Zhejiang Province Department of Chemistry Zhejiang University Hangzhou Zhejiang 310007 China State Key Laboratory of Magnetic Resonance andAtomic and Molecular Physics Wuhan Center for Magnetic Resonance Wuhan Institute of Physics and Mathematics Chinese Academy of Sciences Wuhan Hubei 430071 China College of Biological Chemical Sciences and Engineering Jiaxing University Jiaxing Zhejiang 314001 China State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian Liaoning 116023 China BASF Catalysts (Shanghai) Co. Ltd. 239 Luqiao Road Jinqiao Export Process Zone Pudong New District Shanghai 201206 China Process Research and Chemical Engineering BASF SE 67056 Ludwigshafen Germany

Development of the sustainable routes for synthesis of ITQ-family zeolites is very important because of their unique structures and excellent catalytic and adsorptive *** burden of costly raw materials and low efficiency of synthesis put a strong challenge for their widespread commercial ***,we show an alternative and simple route for synthesis of ITQ-12,ITQ-13,and ITQ-17 zeolites using commercially available organic templates by a facile grinding process of anhydrous starting raw solids,followed by heating at 140-180 ℃.Compared with the conventional hydrothermal synthesis,this approach has obvious advantages such as employment of low-cost organic templates with very high effectiveness,high yield of zeolite products,short crystallization time,and relatively simple *** methodology might open a pathway to synthesize ITQ zeolites with more sustainable manner.

关键词： zeolite sustainable route solvent-free synthesis low-cost organic template ITQ-family

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