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surface charge Accumulation Characteristics on DC GIL Three-post Insulators Considering the Influence of Temperature Gradient

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CSEE Journal of Power and Energy Systems 2023年第5期9卷 1926-1934页

作者： Qi Hu Qingmin Li Zhipeng Liu Naifan Xue Jian Wang Manu Haddad North China Electric Power University Beijing 102206China.He is now with State Grid Jiangxi Electric Power Co.Ltd.Nanchang 330077China the State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources North China Electric Power UniversityBeijing 102206China the Advanced HV Engineering Research Centre Cardiff UniversityThe ParadeCardiff CF243AAU.K.

surface charge accumulation is considered to be a critical factor in flashover failure of three-post insulators.However,surface charge accumulation characteristics on threepost insulators with complex structures and uneven electric fields are still unclear.Furthermore,the temperature gradient field makes charge accumulation more complicated.In this presentation,surface charge profiles of DC three-post insulators under electro-thermal coupling stress are studied by establishing a multi-degree-of-freedom movement measurement system.The abdominal area of the three-post insulator accumulaftes charges of identical polarity as the DC voltage,while the leg area accumulates heteropolar charges.charge density from the bottom of the leg to the center of the abdomen presents a trimodal distribution pattern,including two homopolar charge peaks and one heteropolar charge peak.Asymmetrical surface conductance distribution arising from the temperature gradient leads to a significant increase in amplitude and distribution range of the homopolar charge peak at the legs of insulator.Increase of the temperature gradient will further magnify the homopolar charge peak at the legs.When DC voltage is 100 kV and conductive pole temperature is 70℃,surface charge density of the three-post insulator can reach 100μC/m^(2).Therefore,surface conductance regulation of the leg region is the key to charge regulation and insulation optimization design of DC three-post insulators.

关键词： charge accumulation charge measurement surface charge temperature gradient three-post insulator

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Composite laminar membranes for electricity generation from water evaporation

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Nano Research 2024年第1期17卷 307-311页

作者： Xiao Wang Gang Yuan Han Zhou Yu Jiang Shuo Wang Jiaojiao Ma Chongyang Yang Sheng Hu State Key Laboratory of Physical Chemistry of Solid surfaces Collaborative Innovation Center of Chemistry for Energy Materials(iChEM)College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province(IKKEM) Xiamen 361005China Pen-Tung Sah Institute of Micro-Nano Science and Technology Xiamen UniversityXiamen 361005China

Harvesting clean energy from water evaporation has been extensively investigated due to its sustainability.To achieve high efficiency,energy conversion materials should contain multiple features which are difficult to be simultaneously obtained from single-component materials.Here we use composite laminar membranes assembled by nanosheets of graphene oxide and mica,and find a sustained power density induced by water evaporation that is two orders of magnitude larger than that from membranes made by either of the components.The power output is attributed to selective proton transport driven by water evaporation through the interlayer nanochannels in the membranes.This process relies on the synergistic effects from negatively charged and hydrophilic mica surfaces that are important for proton selectivity and water transport,and the tunable electrical conductivity of graphene oxide that provides optimized internal resistance.The demonstrated composite membranes offer a strategy of enhancing power generation by combining the advantages from each of their components.

关键词： graphene oxide mica water evaporation electrical double layer surface charge ion selectivity

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surface charge of PLA microparticles in regulation of antigen loading,macrophage phagocytosis and activation,and immune effects in vitro

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Particuology 2014年第6期12卷 74-80页

作者： Yuying Liu Xiaoming Chen Lianyan Wang Tingyuan Yang Qipeng Yuan Guanghui Ma National Key Laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of Sciences State Key Laboratory of Chemical Resource Engineering College of Life Science and TechnologyBeijing University of Chemical Technology University of Chinese Academy of Sciences

The use of microparticles（MPs） as adjuvants has attracted increasing interest in vaccine delivery systems.Many physiochemical characteristics of MPs including hydrodynamic size,surface properties,and morphology can regulate the immune response.surface charge is an important characteristic of MPs,but how it affects their adjuvanticity remains unknown.In this study,we prepared uniform-sized polylactide MPs coated with various polymers of different positive charge,and investigated how the surface charge affected antigen loading and macrophage phagocytosis and activation in vitro.A higher surface charge greatly enhanced antigen loading and antigen internalization into macrophages,promoted the expression of MHC 11 and CD80,and increased the secretion level of TNF-a.Taken together,these results indicated that surface charge was an important parameter for improving the adjuvanticity of MPs.

关键词： Microparticle（MP） Macrophage surface charge Antigen loading Phagocytosis Activation

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Calibration Algorithm of surface charge Density on Insulating Materials Measured by Pockels Technique

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Plasma Science and Technology 2011年第6期13卷 645-650页

作者：穆海宝张冠军 School of Electrical Engineering Xi'an Jiaotong University

surface charges greatly affect the discharge/flashover development process across an insulator. The relationship between surface charge distribution on insulating materials and measurement data based on Pockels technique is discussed, and an improved algorithm is built to calculate the real surface charge density from original data. In this algorithm, two-dimensional Fourier transform technique and Wiener filter are employed to reduce the amount of numerical calculation and improve the stability of computation, Moreover, this algorithm considers not only the influence of sample＇s thickness and permittivity, but also the impact of charges at different positions. The achievement of this calibration algorithm is demonstrated in details. Compared with traditional algorithms, the improved one supplies a better solution in the calibration of surface charge distribution on different samples with different thickness.

关键词： Pockels effect surface charge two-dimensional fourier transform Wiener filter

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All-organic modification coating prepared with large-scale atmospheric-pressure plasma for mitigating surface charge accumulation

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Plasma Science and Technology 2023年第8期25卷 12-18页

作者：张鹏浩余亮贺大钊唐昕宇陈硕董守龙姚陈果 State Key Laboratory of Power Transmission Equipment&System Security and New Technology Chongqing UniversityChongqing 400044People's Republic of China School of Electrical Engineering Zhengzhou UniversityZhengzhou 450001People's Republic of China

The surface charge accumulation on polymers often leads to surface flashover.Current solutions are mainly based on the introduction of inorganic fillers.The high-cost process and low compatibility remain formidable challenges.Moreover,existing researches on all-organic insulation focus on capturing electrons,contrary to alleviating charge accumulation.Here,an all-organic modification coating was prepared on polystyrene(PS)with the large-scale atmospheric-pressure plasma,which exhibits outperformed function in mitigating surface charge accumulation.The surface charge dissipation rate and surface conductivity are promoted by about 1.37 and 9.45 times,respectively.Simulation and experimental results show that this all-organic modification coating has a smaller electron affinity potential compared with PS.The decrease of electron affinity potential may result in accelerated surface charge decay of PS,which has never been involved in previous works.Moreover,this coating also has good reliability in a repeated surface flashover.This facile and large-scale approach brings up a novel idea for surface charge regulation and the manufacture of advanced dielectric polymers.

关键词： atmospheric-pressure plasma polymer surface fiashover surface charge surface modification

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EFFECT OF surface charge OF POLYMERIC MICELLES ON IN VITRO CELLULAR UPTAKE

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Chinese Journal of Polymer Science 2013年第9期31卷 1299-1309页

作者： Dan-hua Zhou Jie Zhang Guan Zhang Zhi-hua Gan CAS Key Laboratory of Engineering Plastics Institute of Chemistry Chinese Academy of Sciences Novelty Research Station for SCI-TECH Beijing University of Chemical Technology Department of Urology China-Japan Friendship Hospital State Key Laboratory of Organic-inorganic Composites Beijing Laboratory of Biomedical Materials College of Life Science and Technology Beijing University of Chemical Technology

This work focuses on the interaction between polymeric micelles with different charged surfaces and cancer cells in order to study the influence of surface charge on the in vitro cellular uptake efficiency. The amphiphilic diblock copolymers poly（e-caprolaetone）-b-poly（ethylene oxide）（PCL-b-PEO） with different functional groups at the end of hydrophilic block were synthesized. The functional groups endue the micelles with different charges on the surfaces. The cellular uptake of micelles to T-24 cells （human bladder tumor cells）, HepG2 cells （human liver hepatocellular carcinoma cell line） and Hela cells （human epithelial cervical cancer cells） was studied by means of flow cytometer and confbcal laser scanning microscopy. The results indicate that the surface charges showed great influence on zeta potential of micelles at different pH values. The in vitro cellular uptake efficiency of micelles with different charged surfaces demonstrated different cellular uptake patterns to three kinds of cancer cells.

关键词： Polymeric micelles surface charge pH value Cellular uptake efficiency.

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Improved photocatalytic activity of surface charge functionalized ZnO nanoparticles using aniline

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Journal of Materials Science & Technology 2021年第17期76卷 1-10页

作者： Chatchai Rodwihok Korakot Charoensri Duangmanee Wongratanaphisan Won Mook Choi Seung Hyun Hur Hyun Jin Park Jin Suk Chung School of Chemical Engineering University of Ulsan680-749.South ICorea Department of Biotechnology College of Life Sciences andBiotechnologyKorea University145 Anam-roSeongbuk-guSeoul02841South Korea Research Center in Physics andAstronomy Faculty of ScienceChiang Mai UniversityChiang Mai50200Thailand

Functionalization of aniline molecules on zinc oxide(ZnO)nanoparticles is reported using a simple impregnation technique.Functionalized ZnO samples were systematically characterized based on morphology,surface and optical properties,and photocatalytic performance towards methyl orange(MO).Aniline functionalization increased the surface charge of the modified ZnO.Compared to pristine ZnO,the aniline-functionalized ZnO yielded faster photodegradation of MO,degrading 98.29%of MO in 60 min and superoxide radicals were the major species during the MO photodegradation reaction.These results indicate that the improvement of photocatalytic degradation could be attributed to opposite charge-induced surface adsorption.Hence,protonated amine as a positively charged molecule was expected to increase the surface adsorption of MO(as an anionic dye)on ZnO nanoparticles surfaces,thereby increasing their photocatalytic degradation performance.

关键词： Photocatalysts surface charge ZnO Aniline Methyl orange

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Electrical modeling of dielectric barrier discharge considering surface charge on the plasma modified material

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Chinese Physics B 2020年第7期29卷 383-388页

作者：关弘路陈向荣江铁杜浩 Ashish Paramane 周浩 Zhejiang Provincial Key Laboratory of Electrical Machine Systems College of Electrical EngineeringZhejiang UniversityHangzhou 310027China ZJU-Hangzhou Global Scientific and Technological Innovation Center Hangzhou 311200China

We present the variations of electrical parameters of dielectric barrier discharge(DBD)when the DBD generator is used for the material modification,whereas the relevant physical mechanism is also elaborated.An equivalent circuit model is applied for a DBD generator working in a filament discharging mode,considering the addition of epoxy resin(EP)as the plasma modified material.The electrical parameters are calculated through the circuit model.The surface conductivity,surface potential decay,trap distributions and surface charge distributions on the EP surface before and after plasma treatments were measured and calculated.It is found that the coverage area of micro-discharge channels on the EP surface is increased with the discharging time under the same applied AC voltage.The results indicate that the plasma modified material could influence the ignition of new filaments in return during the modification process.Moreover,the surface conductivity and density of shallow traps with low trap energy of the EP samples increase after the plasma treatment.The surface charge distributions indicate that the improved surface properties accelerate the movement and redistribution of charge carriers on the EP surface.The variable electrical parameters of discharge are attributed to the redistribution of deposited surface charge on the plasma modified EP sample surface.

关键词： dielectric barrier discharge surface charge plasma treatment circuit model

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Effects of Size and surface charge of Polymeric Nanoparticles on in Vitro and in Vivo Applications

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Journal of Biomaterials and Nanobiotechnology 2016年第2期7卷 91-108页

作者： Sams M. A. Sadat Sheikh Tasnim Jahan Azita Haddadi Division of Pharmacy College of Pharmacy and Nutrition University of Saskatchewan Saskatoon Canada

Biodegradable polymeric materials are the most common carriers for use in drug delivery systems. With this trend, newer drug delivery systems using targeted and controlled release polymeric nanoparticles (NPs) are being developed to manipulate their navigation in complex in vivo environment. However, a clear understanding of the interactions between biological systems and these nanoparticulates is still unexplored. Different studies have been performed to correlate the physicochemical properties of polymeric NPs with the biological responses. Size and surface charge are the two fundamental physicochemical properties that provide a key direction to design an effective NP formulation. In this critical review, our goal is to provide a brief overview on the influences of size and surface charge of different polymeric NPs in vitro and to highlight the challenges involved with in vivo trials.

关键词： Nanoparticle Size surface charge In Vitro In Vivo

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Destructing surfactant network in nanoemulsions by positively charged magnetic nanorods to enhance oil-water separation

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Journal of Environmental Sciences 2022年第8期34卷 112-121页

作者： Yongjiao Xiong Xiangfeng Huang Lexue Li Wanqi Liu Jialu Zhang Mengfan He Jia Liu Lijun Lu Kaiming Peng College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource ReuseMinistry of Education Key Laboratory of Yangtze River Water EnvironmentTongji UniversityShanghai 200092China

The separation of ultrafine oil droplets from wasted nanoemulsions stabilized with high concentration of surfactants is precondition for oil reuse and the safe discharge of effluent.However, the double barriers of the interfacial film and network structures formed by surfactants in nanoemulsions significantly impede the oil-water separation. To destroy these surfactant protective layers, we proposed a newly-developed polyethyleneimine micelle template approach to achieve simultaneous surface charge manipulation and morphology transformation of magnetic nanospheres to magnetic nanorods. The results revealed that positively charged magnetic nanospheres exhibited limited separation performance of nanoemulsions, with a maximum chemical oxygen demand(COD) removal of 50%, whereas magnetic nanorods achieved more than 95% COD removal in less than 30 s. The magnetic nanorods were also applicable to wasted nanoemulsions from different sources and exhibited excellent resistance to wide pH changes. Owing to their unique one-dimensional structure, the interfacial dispersion of magnetic nanorods was significantly promoted, leading to the efficient capture of surfactants and widespread destruction of both the interfacial film and network structure, which facilitated droplet merging into the oil phase. The easy-toprepare and easy-to-tune strategy in this study paves a feasible avenue to simultaneously tailor surface charge and morphology of magnetic nanoparticles, and reveals the huge potential of morphology manipulation for producing high-performance nanomaterials to be applied in complex interfacial interaction process. We believe that the newly-developed magnetic-nanorods significantly contribute to hazardous oily waste remediation and advances technology evolution toward problematic oil-pollution control.

关键词： Nanoemulsions surface charge Magnetic nanorods Surfactant Interfacial film Oil-water separation

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