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Recent advances in synthesis strategies and solar-to-hydrogen evolution of 1T phase MS_(2)(M=W,Mo)co-catalysts

Journal of Materials Science & Technology 2022年第6期101卷 242-263页

作者： Shuo Li Jinyan Xiong Xueteng Zhu Weijie Li Rong Chen Gang Cheng School of Chemistry and Environmental Engineering Wuhan Institute of TechnologyDonghu New&High Technology Development ZoneWuhan 430205China College of Chemistry and Chemical Engineering Hubei Key Laboratory of Biomass Fibers and Ecodyeing&FinishingWuhan Textile UniversityWuhan 430200China School of Materials Science and hydrogen Energy Foshan UniversityFoshan 528000China Institute for Superconducting and Electronic Materials Innovation CampusSquires WayUniversity of WollongongNorth WollongongNSW 2500Australia Henan Institute of Advanced Technology Zhengzhou UniversityZhengzhou 450002China

Photocatalytic water splitting is a promising strategy to produce hydrogen as a sustainable and clean energy carrier,based on abundant solar energy and semiconductor photocatalysts,and it has received extensive research and discussion over the past several *** is challenging,however,to achieve an efficient solar-to-hydrogen evolution process with a single particulate photocatalyst due to the weak solar spectrum harvest and the rapid recombination of photogenerated electron-hole pairs during the photocatalysis *** semiconductors to create different co-catalysts presents a viable solution to the above ***,semiconductor photocatalysts modified by different transition metal sulfidebased co-catalysts with designed functions,especially in light absorption enhancement and chargecarrier-separation efficiency promotion,have attracted much *** continued breakthroughs have been made in the preparation,modification,and solar-to-hydrogen evolution application of the 1T phase MS_(2)(M=W,Mo)co-catalyst-based photocatalysis system in recent years,we believe that a comprehensive review of this kind of co-catalyst would further promote its research and development to address the energy and environmental challenges that we are currently ***,recent studies and progress are summarized on the fabrication of 1T phase MS_(2)(M=W,Mo)-based co-catalyst materials,as well as their roles and functional mechanisms for photocatalytic H;***,concluding perspectives on the opportunities in and challenges for the further exploration of the 1T-MS_(2)(M=W,Mo)-based solar-tohydrogen evolution system are presented.

关键词： solar-to-hydrogen evolution Co-catalysts 1T-MS_(2)(M=W Mo) Water splitting Synthesis strategies Photocatalysis

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