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Building better solid-state batteries with silicon-based anodes

Interdisciplinary Materials 2023年第4期2卷 635-663页

作者： Zhefei Sun Quanzhi Yin Haoyu Chen Miao Li Shenghui Zhou sifan Wen Jianhai Pan Qizheng Zheng Bing Jiang Haodong Liu Kangwoon Kim Jie Li Xiang Han Yan-Bing He Li Zhang Meicheng Li Qiaobao Zhang State Key Laboratory of Physical Chemistry of Solid Surfaces College of MaterialsXiamen UniversityXiamenFujianChina State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringCollaborative Innovation Center of Chemistry for Energy MaterialsTan Kah Kee Innovation LaboratoryXiamen UniversityXiamenFujianChina State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources School of New EnergyNorth China Electric Power UniversityBeijingChina Center for Memory and Recording Research Building University of California San DiegoLa JollaCaliforniaUSA Department of Energy Politecnico di MilanoMilanItaly Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and EngineeringNanjing Forestry UniversityNanjingJiangsuChina Tsinghua Shenzhen International Graduate School Shenzhen All-Solid-State Lithium Battery Electrolyte Engineering Research Center and Shenzhen Geim Graphene CenterInstitute of Materials Research(IMR)Tsinghua UniversityShenzhenChina Shenzhen Research Institute of Xiamen University ShenzhenChina

silicon(si)-based solid-state batteries(si-SSBs)are attracting tremendous attention because of their high energy density and unprecedented safety,making them become promising candidates for next-generation energy storage ***,the commercialization of si-SSBs is significantly impeded by enormous challenges including large volume variation,severe interfacial problems,elusive fundamental mechanisms,and unsatisfied electrochemical ***,some unknown electrochemical processes in si-based anode,solid-state electrolytes(SSEs),and si-based anode/SSE interfaces are still needed to be explored,while an in-depth understanding of solid–solid interfacial chemistry is insufficient in *** review aims to summarize the current scientific and technological advances and insights into tackling challenges to promote the deployment of ***,the differences between various conventional liquid electrolyte-dominated si-based lithium-ion batteries(LIBs)with si-SSBs are ***,the interfacial mechanical contact model,chemical reaction properties,and charge transfer kinetics(mechanical–chemical kinetics)between si-based anode and three different SSEs(inorganic(oxides)SSEs,organic–inorganic composite SSEs,and inorganic(sulfides)SSEs)are systemically reviewed,***,the progress for promising inorganic(sulfides)SSE-based si-SSBs on the aspects of electrode constitution,three-dimensional structured electrodes,and external stack pressure is highlighted,***,future research directions and prospects in the development of si-SSBs are proposed.

关键词： interfaces si-based anodes solid-state batteries solid-state electrolytes

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