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The development of hollow multishelled structure: from the innovation of synthetic method to the discovery of new characteristics

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Science China Chemistry 2022年第1期65卷 7-19页

作者： Jiangyan Wang Zumin Wang Dan Mao Dan Wang State Key Laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

Hollow multishelled structure(HoMS)is one of the most promising multifunctional *** high complexity of its structure makes the general and controllable synthesis of HoMS rather *** integration of multidisciplinary knowledge,a great achievement in HoMSs has been obtained in the past ***,the developed sequential templating approach has significantly boomed the progress of HoMS in composition and structure diversity and application *** implementation of the temporal-spatial ordering in HoMS makes it indispensable in solving the key scientific problems in energy conversion,catalysis and drug delivery *** development in HoMSs with novel intricate structures will bring new *** this review,we systematically introduce the development history of HoMSs,summarize the inspiration inherited from the previous research on hollow structures,and discuss the milestones in the development of HoMSs,with a focus on the sequential templating approach for HoMS fabrication,attractive temporal-spatial ordering property and dynamic smart behavior for advanced *** hope to reveal the inherent relationship between the precise synthesis of HoMS and its highly tunable compositional and structural characteristics,and point out its future direction to boost HoMS area further.

关键词： hollow multishelled structure sequential templating approach temporal-spatial ordering smart dynamic behavior

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Hollow Multi-shelled Structure Photoelectric Materials: Multiple Shells Bring Novel Properties

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Chemical Research in Chinese Universities 2024年第3期40卷 413-427页

作者： SU Fengmei WAN Jiawei WANG Dan State Key Laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190P.R.China University of Chinese Academy of Sciences Beijing 100049P.R.China Key Laboratory of Biopharmaceutical Preparation and Delivery Chinese AcademyofSciencesBeijing 100049P.R.China

Hollow multi-shelled structures(HoMSs)have made significant strides across a wide spectrum of scientific investigations since the inception of the sequential templating approach(STA)in 2009,revealing distinctive temporal-spatial ordering *** recent establishment of a mathematical model for STA has not only demystified the formation of concentration waves within the STA process but also extended its relevance to gentler solutionbased systems,thereby broadening the HoMs ***,focusing on photoelectric applications,this review first summarizes the unique temporal-spatial ordering features of ***,the greatly enhanced properties of light capture and absorption,exciton separation,and transfer are deeply ***,we conclude with a perspective on the potential challenges and burgeoning opportunities that lie ahead in the advancement of HoMs development.

关键词： Hollow multi-shelled structure Photoelectric conversion sequential templating approach Light absorption Chargetransfer

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Progress and Perspectives of Hollow Multishelled Structures

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Chinese Journal of Chemistry 2022年第10期40卷 1190-1203页

作者： Jiangyan Wang Mei Yang Dan Wang State Key Laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

Hollow multishelled structure(HoMs)has drawn tremendous attention due to its abundant attractive properties and promising ***,for a long time,the limited synthesis method hindered the development of *** sequential templating approach developed by our group,has greatly enriched its composition and'structure *** progress in HoMS synthesis promotes the discovery of its characteristics as well as widens its application ***,the recently explored temporal-spatial ordering characteristic of HoMS has shown great promise in drug delivery and cascade catalysis application ***,we summarize the current development progress of HoMS in the aspects of both synthesis and application,with a focus discussion on how to shape its application performance by manipulating its composition and structure *** addition,we discuss the current challenges and providethe future potentials holdingfor HoMs.

关键词： Hollow multishelled structure sequential templating approach Temporal-spatial ordering Catalysis Structure-activity relationships

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