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Carbon-containing electrospun nanofibers for lithium-sulfur battery:Current status and future directions

Journal of Energy Chemistry 2021年第3期30卷 254-273页

作者： Zhaoming Tong Liang Huang Wen Lei Haijun Zhang Shaowei Zhang The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and TechnologyWuhan 430081HubeiChina College of Engineering Mathematics and Physical SciencesUniversity of ExeterExeter EX44QFUnited Kingdom

Lithium-sulfur batteries(LSBs)have become promising next-generation energy storage technologies for electric vehicles and portable electronics,due to its excellent theoretical specific ***,the low conductivity of sulfur species,notorious lithium dendrites,the severe"shuttle effect"of polysulfides(LiPSs)and the inferior kinetic reaction for LiPSs/Li_(2)S conversion during discharge-charge have seriously hindered their practical application,and also pose potential safety *** to their superior porous architectures,high specific surface areas,excellent structural designability,functional modifiability,abundant active sites and flexibility of carbon-containing electrospun nanofibers(CENFs),they exhibited the superior characteristics that can simultaneously solve the above *** this review,we summarize the recent progress and application of CENFs in ***,we provide a brief introduction to the structure and composition controlled of carbon nanofibers by *** then review progress in recent developments of CENFs for LSBs including cathodes,anodes,separators,and *** focus on how to solve practical issues that arise when the CENFs are applied to various parts of LSBs,and the relevant working mechanisms are described,from high sulfur loading and Li dendrites suppression to LiPSs’confinement and ***,we summarize and propose the existing challenges and future prospects of CENFs,for the design and architecture of electrochemical components in Li-S energy storage systems.

关键词： Lithium-sulfur batteries Electrospinning Carbon-containing nanofibers Cathodes Anodes separators and interlayers

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