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Synthesis and enhanced piezoelectric response of CVD-grown SnSe layered nanosheets for flexible nanogenerators

Nano Research 2023年第9期16卷 11839-11845页

作者： Fumei Yang Man-Chung Wong Jianfeng Mao Zehan Wu Jianhua Hao Department of Applied Physics the Hong Kong Polytechnic UniversityHong Kong 999077China

Piezoelectricity is the electric charge which accumulates in certain materials in response to mechanical stimuli,while piezoelectric nanogenerators(PENGs)converting mechanical energy into electricity can be widely used for energy harvesting and self-powered *** group IV-VI monochalcogenides may exhibit strong piezoelectricity because of their puckered C_(2v)symmetry and electronic structure,making them promising for flexible ***,we investigated the synthesis and piezoelectric properties of multilayer SnSe nanosheets grown by chemical vapor deposition(CVD).The SnSe nanosheets exhibited high single-crystallinity,large area,and good *** strong layer-dependent in-plane piezoelectric coefficient of SnSe nanosheets showed a saturated trend to be~110 pm/V,which overcomes the weak piezoelectric response or odd-even effects in other layered nanosheets.A high energy conversion efficiency of 9.3%and a maximum power density of 538 mW/cm^(2)at 1.03%strain have been demonstrated in a SnSe-based *** on the enhanced piezoelectricity of SnSe and attractive output performance of the nanogenerator,a self-powered sensor for human motion monitoring is further *** results demonstrate the strong piezoelectricity in high quality CVD-grown SnSe nanosheets,allowing for application in flexible smart piezoelectric sensors and advanced microelectromechanical devices.

关键词： SnSe piezotronics piezoresponse force microscope piezoelectric nanogenerator self-powered device

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A self‑powered Piezoelectric Nanofibrous Membrane as Wearable Tactile Sensor for Human Body Motion Monitoring and Recognition

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Advanced Fiber Materials 2023年第4期5卷 1417-1430页

作者： Jingcheng Li Jing Yin Mei Gui Vanessa Wee Amutha Chinnappan Seeram Ramakrishna Centre for Nanotechnology and Sustainability Department of Mechanical EngineeringNational University of SingaporeSingapore 117081Singapore National Engineering Laboratory for Modern Silk College of Textile and Clothing EngineeringSoochow UniversitySuzhouChina Integrative Sciences and Engineering Program NUS Graduate SchoolNational University of SingaporeSingapore 119077Singapore

Wearable sensors have drawn vast interest for their convenience to be worn on body to monitor and track body movements or exercise activities in real ***,wearable electronics rely on powering systems to ***,a self-powered,porous,flexible,hydrophobic and breathable nanofibrous membrane based on electrospun polyvinylidene fluoride(PVDF)nanofiber has been developed as a tactile sensor with low-cost and simple fabrication for human body motion detection and ***,effects of multi-walled carbon nanotubes(CNT)and barium titanate(BTO)as additives to the fiber morphology as well as mechanical and dielectric properties of the piezoelectric nanofiber membrane were *** fabricated BTO@PVDF piezoelectric nanogenerator(PENG)exhibits the highβ-phase content and best overall electrical performances,thus selected for the flexible sensing device ***,the nanofibrous membrane demonstrated robust tactile sensing performance that the device exhibits durability over 12,000 loading test cycles,holds a fast response time of 82.7 ms,responds to a wide pressure range of 0-5 bar and shows a high relative sensitivity,especially in the small force range of 11.6 V/bar upon pressure applied perpendicular to the ***,when attached on human body,its unique fibrous and flexible structure offers the tactile sensor to present as a health care monitor in a self-powered manner by translating motions of different movements to electrical signals with various patterns or sequences.

关键词： Electrospinning Nanofiber Piezoelectric sensor PENG Wearable self-powered device

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Flexible bidirectional self-powered photodetector with significantly reduced volume and accelerated response speed based on hydrogel and lift-off GaN-based nanowires

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Fundamental Research 2024年第2期4卷 369-378页

作者： Min Jiang Yukun Zhao Penghui Zheng Jianya Zhang Wenxian Yang Min Zhou Yuanyuan Wu Renjun Pei Shulong Lu Key Lab of Nanodevices and Applications Suzhou Institute of Nano-Tech and Nano-Bionics(SINANO)Chinese Academy of Sciences(CAS)Suzhou 215123China School of Nano-Tech and Nano-Bionics University of Science and Technology of ChinaHefei 230026China CAS Key Laboratory of Nano-Bio Interface Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China Nanchang Research Institute Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesNanchang 330200China

Due to the wide range of potential applications for next-generation multi-functional devices,the flexible selfpowered photodetector(PD)with polarity-switchable behavior is essential but very challenging to be ***,a wearable bidirectional self-powered PD based on detached(Al,Ga)N and(In,Ga)N nanowires has been proposed and demonstrated *** from the photovoltage-competing dynamics across(Al,Ga)N and(In,Ga)N nanowire photoelectrodes,such PD can generate the positive(33.3 mA W−1)and negative(-0.019 mA W−1)photo-responsivity under ultraviolet(UV)and visible illumination,respectively,leading to the bidirectional photocurrent *** to the introduction of quasi solid-state hydrogel,the PD can work without the liquid-electrolyte,thus remarkably reducing the volume from about 482 cm3 to only 0.18 ***,the use of hydrogel is found to enhance response speed in the UV range by reducing the response time for more than 95%,which is mainly attributed to the increased open circuit potential and reduced ion transport *** the GaN connecting segment is pretty thin,the piezoelectric charges generated by stress are proposed to have only a limited effect on the photocurrent ***,both the stable on-off switching characteristics and photocurrent densities can still be achieved after being bent 400 *** an excellent flexibility,this work creates opportunities for technological applications of bidirectional photocurrent PDs in flexible optoelectronic devices,e.g.,wearable intelligent sensors.

关键词： Flexible photodetector Bidirectional photocurrent Lift-off GaN-based nanowires Hydrogel self-powered device

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Emerging trends in materials and devices-based electric stimulation therapy for tumors

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BMEMat(BioMedical Engineering Materials) 2023年第3期1卷 101-122页

作者： Shiwang Xie Jing Huang Andreia Trindade Pereira Lingling Xu Dan Luo Zhou Li Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijingChina School of Nanoscience and Engineering University of Chinese Academy of SciencesBeijingChina CAS Key Laboratory for Biomedical Effects of Nanomaterials and Nanosafety CAS Center for Excellence in NanoscienceNational Center for Nanoscience and Technology of ChinaBeijingChina Instituto de Investigação e Inovação em Saúde i3SUniversity of PortoPortoPortugal

Electrical stimulation(ES),as one of the physical therapy modalities for tumors,has attracted extensive attention of researchers due to its promising *** the continuous development of material science,nanotechnology,and micro/nano processing techniques,novel electroactive nanomaterials and delicately designed devices have emerged to realize innovative ES therapies,which provide more possibilities and approaches for tumor ***,exploring the molecular biological mechanisms underlying different ES modalities affecting tumor cells and their immune microenvironment is also an unresolved hotspot emerging from the current biomedical engineering *** on the above research interests,in this review,we systematically summarized the effects of different ES parameters on the subcellular structure of tumor cells and the tumor immune microenvironment(TIME)in conjunction with the involved signaling *** addition,we also reviewed the latest progress in novel self-powered devices and electroactive nanomaterials for tumor ***,the prospects for the development of electrostimulation tumor therapy are also discussed,bringing inspiration for the development of new physical therapy strategies in the future.

关键词： cancer therapy electrical stimulation electroactive materials self-powered device

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