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Solar evaporation for simultaneous oil-water separation and electricity generation with Janus wood-based absorbers

Frontiers of Environmental Science & Engineering 2024年第2期18卷 13-23页

作者： Yue Yang Ze Fu Qi Zhang Jiangsu Key Laboratory of Chemical Pollution Control and Resources Reuse School of Environmental and Biological EngineeringNanjing University of Science&TechnologyNanjing 210094China Key Laboratory of Industrial Ecology and Environmental Engineering(Ministry of Education) School of Environmental Science and TechnologyDalian University of TechnologyDalian 116024China National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced MicrostructuresCollege of Engineering and Applied SciencesKey Laboratory of Intelligent Optical Sensing and Manipulation(Ministry of Education)Jiangsu Key Laboratory of Artificial Functional MaterialsNanjing UniversityNanjing 210093China

Oily wastewater from ocean oil spills endangers marine ecosystems and human health. Therefore, developing an effective and sustainable solution for separating oil-water mixtures is urgent. Interfacial solar photothermal evaporation is a promising approach for the complete separation of two-phase mixtures using only solar energy. Herein, we report a carbonized wood-based absorber with Janus structure of comprising a hydrophobic top-layer and an oleophobic bottom-layer for simultaneous solar-driven oil-water separation and electricity generation. Under sunlight irradiation, the rapid evaporation of seawater will induce a separation of oil-water mixtures, and cause a high salt concentration region underlying the interface, while the bottom “bulk water” maintains in a low salt concentration, thus forming a salinity gradient. Electricity can be generated by salinity gradient power. Therefore, oil-water separation efficiency of > 99% and derived extra electricity power of ~0.1 W/m2 is achieved under solar radiation, demonstrating the feasibility of oil-water separation and electricity production synchronously directly using solar energy. This work provides a green and cost-effective path for the separation of oil-water mixtures.

关键词： Oily wastewater Carbonized wood salinity gradient Electricity generation Solar irradiation

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Spatiotemporal optical properties of dissolved organic matter in a sluice-controlled coastal plain river with both salinity and trophic gradients

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Journal of Environmental Sciences 2023年第7期129卷 1-15页

作者： Yu Liu Yucheng Hu Chengxun Yu Yuqi Gao Zhenying Liu Khan M.G.Mostofa Siliang Li Yumei Hu Guanghui Yu School of Earth System Science Institute of Surface-Earth System ScienceTianjin UniversityTianjin 300072China Tianjin Hydraulic Science Research Institute Tianjin 300061China School of Environmental Science and Safety Engineering Tianjin University of TechnologyTianjin 300191China School of Mathematics Tianjin UniversityTianjin 300072China

Due to the combined effect of sluices and sea tide,the sluice-controlled coastal plain river would be characterized by both trophic state and salinity gradients,affecting the spatiotemporal optical properties of dissolved organicmatter(DOM).In this study,we investigated the spatiotemporal variation of water quality parameters and optical properties of DOM in the Haihe River,a representative sluice-controlled coastal plain river in Tianjin,China.A significant salinity gradient and four trophic states were observed in the water body of the Haihe River.Two humic-and one protein-like substances were identified from the DOM by the three-dimensional fluorescence spectra combined with the parallel factor(PARAFAC)analysis.Pearson’s correlation analysis and redundancy analysis(RDA)showed that the salinity significantly affected the abundance of chromophoric DOM(CDOM)but did not cause significant changes in the fluorescence optical characteristics.In addition,the effect of Trophic state index(TSI)on the CDOM abundance was greater than that on the fluorescence intensity of fluorescent dissolved organic matter(FDOM).In the water body with both salinity and trophic state gradients,TSI posed a greater influence than salinity on the CDOM abundance.Our results fill the research gap in spatiotemporal DOM characteristics and water quality variation in water bodies with both salinity and trophic state gradients.These results are beneficial for clarifying the joint influence of saline intrusion and sluices on the DOM characteristics and water quality in sluice-controlled coastal plain rivers.

关键词： Dissolved organic matter Optical characteristics Trophic state index salinity gradient Haihe River Sluice-controlled coastal plain river

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Response of gaseous carbon emissions to low-level salinity increase in tidal marsh ecosystem of the Min River estuary,southeastern China

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Journal of Environmental Sciences 2017年第2期29卷 210-222页

作者： Minjie Hu Hongchang Ren Peng Ren Jiabing Li Benjamin J.Wilson Chuan Tong School of Geographical Sciences Fujian Normal UniversityFuzhou 350007China Key Laboratory of Humid Sub-tropical Eco-geographical Process of Ministry of Education Fujian Normal UniversityFuzhou 350007China Research Centre of Wetlands in Subtropical Region Fujian Normal UniversityFuzhou 350007China School of Environmental Sciences Fujian Normal UniversityFuzhou 35000YChina Department of Biological Sciences Florida International UniversityMiamiFL 33199USA

Although estuarine tidal marshes are important contributors to the emission of greenhouse gases into the atmosphere, the relationship between carbon dioxide（CO2）, methane（CH4）emission, and environmental factors, with respect to estuarine marshes, has not been clarified thoroughly. This study investigated the crucial factors controlling the emission of CO2 and CH4from a freshwater marsh and a brackish marsh located in a subtropical estuary in southeastern China, as well as their magnitude. The duration of the study period was November 2013 to October 2014. Relevant to both the field and incubation experiments, the CO2 and CH4emissions from the two marshes showed pronounced seasonal variations. The CO2 and CH4emissions from both marshes demonstrated significant positive correlations with the air/soil temperature（p 〈 0.01）, but negative correlations with the soil electrical conductivity and the pore water/tide water Cl-and SO42- （p 〈 0.01）. The results indicate no significant difference in the CO2 emissions between the freshwater and brackish marshes in the subtropical estuary, whereas there was a difference in the CH4 emissions between the two sites（p 〈 0.01）. Although future sea-level rise and saltwater intrusion could reduce the CH4 emissions from the estuarine freshwater marshes, these factors had little effect on the CO2 emissions with respect to an increase in salinity of less than 5‰. The findings of this study could have important implications for estimating the global warming contributions of estuarine marshes along differing salinity gradients.

关键词： Greenhouse gases salinity gradient Global warming Tidal marsh Min River estuary

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The effect of salinity on Fucus ceranoides (Ochrophyta,Phaeophyceae) in the Mondego River(Portugal)

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Journal of Oceanology and Limnology 2019年第3期37卷 881-891页

作者： COTAS Joao FIGUEIRINHA Artur PEREIRA Leonel BATISTA Teresa Department of Life Sciences University of CoimbraCoimbra 3001-456Portugal MARE-Marine and Environmental Sciences Centre Faculty of Science and TechnologyUniversity of CoimbraCoimbra 3000-548Portugal Laboratory of Pharmacognosy Faculty of PharmacyUniversity of CoimbraCoimbra 3000-548Portugal LAQV REQUIMTEFaculty of PharmacyUniversity of CoimbraCoimbra 3000-548Portugal CIEPQPF Department of Chemical EngineeringFaculty of Science and TechnologyUniversity of CoimbraCoimbra 3030-790Portugal

Algae(and their extracts)are increasingly important for pharmaceutical applications due to the diversity of useful compounds they contain.The genus Fucus contains one of the most studied species,Fucus vesiculosus.The species F.ceranoides differs from the others of the genus by presenting longitudinal air-vesicles and a capacity to survive at low salinities.It is an alga that inhabits the Mondego River estuary(Portugal),at the southern limit of its distribution,and can serve as a role model to understand the effect of a salt gradient on the production of bioactive compounds.We assessed the phenolic content and antioxidant activity of different F.ceranoides extracts(e.***.methanolic,aqueous and polysaccharide)prepared from samples harvested from two different zones to evaluate if the adaptation of F.ceranoides to different salinity levels influenced its chemical composition.The antioxidant activity of the extracts was determined using 1,2-diphenyl-picrylhydrazyl(DPPH)and 2.2-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid)(ABTS)radicals.These assays demonstrated that the methanolic extract of lyophilized F.ceranoides that grew at low salinities was the most bioactive,i.e.DPPH(IC 50=50.39μg/mL)and ABTS(TEAC=2.42).The total phenolic content(Folin-Ciocalteu method)and the methanolic extract of the lyophilized F.ceranoides collected from a low salinity habitat exhibited the highest phenolic content(PGE=49.48μg/mg of lyophilized extract)amongst those sampled.Thin layer chromatography(TLC)and Fourier transform infrared spectroscopy(FTIR)were used for the identification of compounds in the extracts.This characterization allowed confirmation that the various extracts contained almost the same compounds but with notable quantitative differences.Based on these results,we conclude that there were differences in the quantity of the compounds due to the effect of salinity.The drying methods used were also found to have influenced the quality of the extracted compounds.

关键词： Fucus ceranoides salinity gradient sequential extractions phenolic content dependent bioactivities spectroscopic analysis

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