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Wettability control in electrocatalyst: A mini review

Journal of Energy Chemistry 2022年第7期31卷 643-655,I0016页

作者： Yan Liang Yifeng Han Jing-sha Li Jun Wang Depei Liu Qi Fan Key Laboratory of Solar Energy Science and Technology in Jiangsu Province Southeast UniversityNanjing 210096JiangsuChina National Laboratory of Solid State Microstructures Jiangsu Key Laboratory for Nano TechnologySchool of PhysicsNanjing UniversityNanjing 210093JiangsuChina Power China Huadong Engineering Corporation Limited Hangzhou 311122ZhejiangChina Institute of Materials Science and Devices School of Materials Science and EngineeringSuzhou University of Science and TechnologySuzhou 215011JiangsuChina

Electrocatalysis, as a typical heterogeneous catalysis, generally occurs in the di-or tri-phase *** is an important property for describing the balance of a gas-liquid-solid system. Therefore,the wettability of reaction interface, especially hydrophilicity/hydrophobicity, plays an important role in the adsorption/desorption process of gas bubbles on the surface of the solid electrode. Herein, we present a comprehensive review of the wettability control of the electrode materials applied in electrocatalysis reactions, including hydrogen evolution reaction(HER), oxygen evolution reaction(OER), oxygen reduction reaction(ORR) and carbon dioxide reduction reaction(CO_(2) RR). Firstly, the basic theories of wettability as well as the impact on electrocatalysis were introduced in this review. Secondly, the overview of modifying methods of the wettability from electrocatalyst microstructure(structural modification, surface coating, introducing hydrophilic groups) and system design(electrode, device) were suggested. At last, the deficiencies and problems in the application of wettability control are discussed,and deeper and broader application prospects are proposed.

关键词： Electrocatalysis reaction interfaces Wettability Gas evolution reactions Gas consumption reactions

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