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quasi-compensatory effect in emerging anode-free lithium batteries

eScience 2021年第1期1卷 3-12页

作者： Peng Li Hun Kim Jun Ming Hun-Gi Jung Ilias Belharouak Yang-Kook Sun Department of Energy Engineering Hanyang UniversitySeoul 04763Republic of Korea State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryCASChangchun 130022China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China Center for Energy Storage Research Korea Institute of Science and TechnologySeoul 02792Republic of Korea Division of Energy&Environment Technology Korea University of Science and TechnologyDaejeon 34113Republic of Korea Electrification and Energy Infrastructure Division Oak Ridge National LaboratoryOak RidgeTN 37831United States Bredesen Center for Interdisciplinary Research and Graduate Education University of TennesseeKnoxvilleTN 37996United States

As electric vehicle(EV)sales grew approximately 50%year-over-year,surpassing 3.2 million units in 2020,the“roaring era”of EV is around the *** meet the increasing demand for low cost and high energy density batteries,anode-free configuration,with no heavy and voluminous host material on the current collector,has been proposed and further ***,it always suffers from several non-negligible“bottlenecks”,such as fragile solid electrolyte interface,deteriorated cycling reversibility,and uncontrolled dendrite *** by the“compensatory effect”of some disabled people with other specific functions strengthened to make up for their inconvenience,corresponding quasi-compensatory measures after anode removal,involving dimensional compensation,SEI robustness compensation,lithio-philicity compensation,and lithium source compensation,have been carried out and achieved significant battery performance *** this review,the chemistry,challenges,and rationally designed“quasi-compensatory effect”associated with anode-free lithium-ion battery are systematically discussed with several possible R&D directions that may aid,direct,or facilitate future research on lithium storage in anode-free configuration essentially emphasized.

关键词： Lithium battery Anode free quasi-compensatory effect Battery configuration

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