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Maleimide Chemistry:Enabling the precision polymer synthesis

Chinese Journal of Chemistry 2021年第12期39卷 3177-3187页

作者： Glauber Mejia Yongquan Wang Zhihao Huang Qiunan Shi Zhengbiao Zhang Joint Engineering Laboratory for Novel Functional polymeric Materials Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationCollege of ChemistryChemical Engineering and Materials ScienceSoochow UniversitySuzhouJiangsu 215123China State Key Laboratory of Radiation Medicine and Protection Soochow UniversitySuzhouJiangsu 215123China

Herein is presented a compilation of the main characteristics of maleimide chemistry in developing the precisely controlled polymers,including the design of sequence-controlled polymers,topological polymers,and polymeric single-chain *** synthetic methods,relied on the versatilities of the maleimide moieties as a latent monomer which leads to an efficient alternative in various innovative applications,especially in self-healing material,self-reporting materials for real-time monitoring,and also in data storage and anticounterfeiting *** core of the content in this review is focused on the up-to-data advances and publications on the major of maleimide chemistry in our research group.

关键词： Maleimide chemistry precision polymer synthesis polymers Topochemistry Dendrimers

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Research progress in the living/controlled polymerization of(meth)acrylate monomers by Lewis pair

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Science China Chemistry 2023年第8期66卷 2256-2266页

作者： Wuchao Zhao Jianghua He Yuetao Zhang State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchun130012China

Lewis pair polymerization(LPP)has demonstrated its unique advantages,such as high activity,high stability,and adjustable variability,towards the polymerization of(meth)acrylate monomers in comparison with the other polymerization *** combination of Lewis acid(LA)and Lewis base(LB)to construct Lewis pairs(LPs)with appropriate Lewis basicity,Lewis acidity,and steric effects would significantly impact the polymerization process,including chain initiation,propagation,termination and chain transfer reaction,as well as polymerization manner of *** this feature article,we briefly review recent progress made by our research group towards the living/controlled polymerization of(meth)acrylate monomers,which were accomplished by a series of newly designed LPs,including monofunctional LPs,dual-initiating LPs and intramolecular tethered trifunctional *** article is divided into three parts:(1)the development of monofunctional living/controlled LP polymerization system;(2)the design and preparation of dual-initiating LPs in synthesizing thermoplastic elastomers;(3)the application of intramolecular trifunctional LP to the synthesis of cyclic *** developed LPPs have demonstrated their powerful capability in precise control over the molecular weight,molecular weight distribution,and monomer sequence as well as the topology of *** review will serve as a good resource or guideline for researchers currently working in the area of LPP and for those who are interested in synthesizing new materials by LPP.

关键词： frustrated Lewis pair living polymerization precision polymer synthesis sequence-controlled polymer

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