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Characteristics of PM_(2.5) pollution in Beijing after the improvement of air quality

Journal of Environmental Sciences 2021年第2期33卷 1-10页

作者： Xiaojuan Huang Guiqian Tang Junke Zhang Baoxian Liu Chao Liu Jin Zhang Leilei Cong Mengtian Cheng Guangxuan Yan Wenkang Gao Yinghong Wang Yuesi Wang Plateau Atmosphere and Environment Key Laboratory of Sichuan Province School of Atmospheric SciencesChengdu University of Information TechnologyChengdu 610225China State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry(LAPC) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Faculty of Geosciences and Environmental Engineering Southiuest Jiaotong UniversityChengdu 611756China Beijing Municipal Environmental Monitoring Centre Beijing 100048China Fengtai District Ecology and Environment Bureau Beijing 100071China School of Environment Henan Normal UniuersityKey Laboratory Jor YellouRiuer and Huai Riuer Water Environment and Pollution ControlMinistry of EducationHenan Key Laboratory/or EnvironmentaI Pollution ControlXinxiang 453007China

Following the implementation of the strictest clean air policies to date in Beijing,the physicochemical characteristics and sources of PM_(2.5) have changed over the past few years.To improve pollution reduction policies and subsequent air quality further,it is necessary to explore the changes in PM_(2.5) over time.In this study,over one year(2017-2018)field study based on filter sampling(TH-150C;Wuhan Tianhong,China)was conducted in Fengtai District,Beijing,revealed that the annual average PM_(2.5) concentration(64.8±43.1μg/m^3)was significantly lower than in previous years and the highest PM_(2.5) concentration occurred in spring(84.4±59.9μg/m^3).Secondary nitrate was the largest source and accounted for 25.7%of the measured PM_(2.5).Vehicular emission,the second largest source(17.6%),deserves more attention when considering the increase in the number of motor vehicles and its contribution to gaseous pollutants.In addition,the contribution from coal combustion to PM_(2.5) decreased significantly.During weekends,the contribution from EC and NO3−increased whereas the contributions from SO4^2−,OM,and trace elements decreased,compared with weekdays.During the period of residential heating,PM_(2.5) mass decreased by 23.1%,compared with non-heating period,while the contributions from coal combustion and vehicular emission,and related species increased.With the aggravation of pollution,the contribution of vehicular emission and secondary sulfate increased and then decreased,while the contribution of NO3−and secondary nitrate continued to increase,and accounted for 34.0%and 57.5%of the PM_(2.5) during the heavily polluted days,respectively.

关键词： PM_(2.5) Seasonal variations Chemical composition Source apportionment pollution evolution

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