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Recent Progress,Challenges,and Prospects in Two‑Dimensional photo‑Catalyst Materials and Environmental Remediation

Nano-Micro Letters 2020年第12期12卷 29-105页

作者： Karim Khan Ayesha Khan Tareen Muhammad Aslam Rizwan Ur Rehman Sagar Bin Zhang Weichun Huang Asif Mahmood Nasir Mahmood Kishwar Khan Han Zhang Zhongyi Guo School of Electrical Engineering and Intelligentization Dongguan University of Technology(DGUT)Dongguan 523808GuangdongPeople’s Republic of China Institute of Microscale Optoelectronics Collaborative Innovation Centre for Optoelectronic Science and TechnologyKey Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong ProvinceCollege of Physics and Optoelectronic EngineeringShenzhen Key Laboratory of Micro‑Nano Photonic Information TechnologyGuangdong Laboratory of Artificial Intelligence and Digital Economy(SZ)Shenzhen UniversityShenzhen 518060People’s Republic of China College of Materials Science and Engineering Shenzhen UniversityShenzhen 518060People’s Republic of China Government Degree College Paharpur Gomel UniversityDera Ismail KhanK.P.KIslamic Republic of Pakistan School of Materials Science and Engineering Jiangxi University of Science and TechnologyJiangxi 341000People’s Republic of China School of Chemical and Bio‑Molecular Engineering The University of SydneySydneyNSW 2006Australia School of Engineering The Royal Melbourne Institute of Technology(RMIT)UniversityMelbourneVICAustralia Research Laboratory of Electronics(RLE) Massachusetts Institute of Technology(MIT)CambridgeMAUSA

The successful photo-catalyst library gives significant information on feature that affects photo-catalytic performance and proposes new *** is considerably significant to form multi-functional photo-catalysts with flexible *** recently,two-dimensional materials(2DMs)gained much attention from researchers,due to their unique thickness-dependent uses,mainly for photo-catalytic,outstanding chemical and physical ***-catalytic water splitting and hydrogen(H2)evolution by plentiful compounds as electron(e−)donors is estimated to participate in constructing clean method for solar *** photocatalysis received much research attention caused by their applications to tackle numerous energy and environmental *** broad review explains progress regarding 2DMs,significance in structure,and catalytic *** will discuss in detail current progresses of approaches for adjusting 2DMs-based photo-catalysts to assess their photo-activity including doping,hetero-structure scheme,and functional formation *** plans,e.g.,doping and sensitization of semiconducting 2DMs,increasing electrical conductance,improving catalytic active sites,strengthening interface coupling in semiconductors(SCs)2DMs,forming nano-structures,building multi-junction nano-composites,increasing photo-stability of SCs,and using combined results of adapted approaches,are summed ***,to further improve 2DMs photo-catalyst properties,hetero-structure design-based 2DMs’photo-catalyst basic mechanism is also reviewed.

关键词： Two-dimensional materials photo-catalysts H2O2/H2-production Pollutant degradation CO2 reduction

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